Standard approaches to quantum computing require significant overhead to correct for errors. The hardware size for conventional quantum processors in solids often increases linearly with the number of physical qubits, such as for transmon qubits in superconducting circuits or electron spin qubits in quantum dot arrays. While photonic circuits based on flying qubits do not suffer from decoherence or lack of potential scalability, they have encountered significant challenges to overcome photon loss in long delay circuits. Here, we propose an alternative approach that utilizes flying electronic wave packets propagating in solid-state quantum semiconductor circuits. Using a novel time-bin architecture for the electronic wave packets, hardware requirements are drastically reduced because qubits can be created on-demand and manipulated with a common hardware element, unlike the localized approach of wiring each qubit individually. The electronic Coulomb interaction enables reliable coupling and readout of qubits. Improving upon previous devices, we realize electronic interference at the level of a single quantized mode that can be used for manipulation of electronic wavepackets. This important landmark lays the foundation for fault-tolerant quantum computing with a compact and scalable architecture based on electron interferometry in semiconductors.
Pierre Hamonic, Martin Nurizzo, Jayshankar Nath, Matthieu C. Dartiailh, Victor El-Homsy, Mathis Fragnol, Biel Martinez, Pierre-Louis Julliard, Bruna Cardoso Paz, Mathilde Ouvrier-Buffet, Jean-Baptiste Filippini, Benoit Bertrand, Heimanu Niebojewski, Christopher Bäuerle, Maud Vinet, Franck Balestro, Tristan Meunier, Matias Urdampilleta Semiconductor quantum dot arrays are a promising platform to perform spin-based error-corrected quantum computation with large numbers of qubits. However, due to the diverging number of possible charge configurations combined with the limited sensitivity of large-footprint charge sensors, achieving single-spin occupancy in each dot in a growing quantum dot array is exceedingly complex. Therefore, to scale-up a spin-based architecture we must change how individual charges are readout and controlled. Here, we demonstrate single-spin occupancy of each dot in a foundry-fabricated array by combining two methods. 1/ Loading a finite number of electrons into the quantum dot array; simplifying electrostatic tuning by isolating the array from the reservoirs. 2/ Deploying multiplex gate-based reflectometry to dispersively probe charge tunneling and spin states without charge sensors or reservoirs. Our isolated arrays probed by embedded multiplex readout can be readily electrostatically tuned. They are thus a viable, scalable approach for spin-based quantum architectures.
Jashwanth Shaju, Elina Pavlovska, Ralfs Suba, Junliang Wang, Seddik Ouacel, Thomas Vasselon, Matteo Aluffi, Lucas Mazzella, Clement Geffroy, Arne Ludwig, Andreas D. Wieck, Matias Urdampiletta, Christopher Bäuerle, Vyacheslavs Kashcheyevs, Hermann Sellier Emergence of universal collective behaviour from interactions in a sufficiently large group of elementary constituents is a fundamental scientific paradigm. In physics, correlations in fluctuating microscopic observables can provide key information about collective states of matter such as deconfined quark-gluon plasma in heavy-ion collisions or expanding quantum degenerate gases. Two-particle correlations in mesoscopic colliders have provided smoking-gun evidence on the nature of exotic electronic excitations such as fractional charges, levitons and anyon statistics. Yet the gap between two-particle collisions and the emergence of collectivity as the number of interacting particles grows is hard to address at the microscopic level. Here, we demonstrate all-body correlations in the partitioning of up to $N = 5$ electron droplets driven by a moving potential well through a Y-junction in a semiconductor. We show that the measured multivariate cumulants (of order $k = 2$ to $N$) of the electron droplet are accurately described by $k$-spin correlation functions of an effective Ising model below the Néel temperature and can be interpreted as a Coulomb liquid in the thermodynamic limit. Finite size scaling of high-order correlation functions provides otherwise inaccessible fingerprints of emerging order. Our demonstration of emergence in a simple correlated electron collider opens a new way to study engineered states of matter.
Seddik Ouacel, Lucas Mazzella, Thomas Kloss, Matteo Aluffi, Thomas Vasselon, Hermann Edlbauer, Junliang Wang, Clement Geffroy, Jashwanth Shaju, Michihisa Yamamoto, David Pomaranski, Shintaro Takada, Nobu-Hisa Kaneko, Giorgos Georgiou, Xavier Waintal, Matias Urdampilleta, Arne Ludwig, Andreas D. Wieck, Hermann Sellier, Christopher Bäuerle Electronic flying qubits offer an interesting alternative to photonic qubits: electrons propagate slower, hence easier to control in real time, and Coulomb interaction enables direct entanglement between different qubits. While their coherence time is limited, picosecond-scale control would make them competitive in terms of number of possible coherent operations. The key challenge lies in achieving the dynamical regime, where the injected plasmonic pulse width is shorter than the quantum device dimensions. Here we reach this new regime in a quantum nanoelectronic system by injecting ultrashort single electron plasmonic pulses into a 14-micrometer-long Mach-Zehnder interferometer. Our findings reveal that quantum coherence is preserved for ultrashort plasmonic pulses, exhibiting enhanced contrast of coherent oscillations compared to the DC regime. Moreover, this coherence remains robust even under large bias voltages. This milestone demonstrates the feasibility of flying qubits as a promising alternative to localized qubit architectures, offering reduced hardware footprint, increased connectivity, and potential for scalable quantum information processing.
The displacement of a single electron enables exciting avenues for nanotechnology with vast application potential in quantum metrology, quantum communication and quantum computation. Surface acoustic waves (SAW) have proven itself as a surprisingly useful solution to perform this task over large distance with outstanding precision and reliability. Over the last decade, important milestones have been achieved bringing SAW-driven single-electron transport from first proof-of-principle demonstrations to accurate, highly-controlled implementations, such as coherent spin transport, charge-to-photon conversion, or antibunching of charge states. Beyond the well-established piezoelectric gallium-arsenide platform, first realisations of acousto-electronic transport have also been carried out on the surface of liquid helium. In this review article, we aim to keep track of this remarkable progress by explaining these recent achievements from basic principles, with an outlook on follow-up experiments and near-term applications.
Surface acoustic waves (SAWs) hold a vast potential in various fields such as spintronics, quantum acoustics, and electron-quantum optics, but an electromagnetic wave emanating from SAW generation circuits has often been a major hurdle. Here, we investigate a differential excitation method of interdigital transducers (IDTs) to generate SAWs while reducing the electromagnetic wave. The results show that electromagnetic waves are suppressed by more than 90% in all directions. This suppression overcomes the operating limits and improves the scalability of SAW systems. Our results promise to facilitate the development of SAW-based applications in a wide range of research fields.
Shunsuke Ota, Junliang Wang, Hermann Edlbauer, Yuma Okazaki, Shuji Nakamura, Takehiko Oe, Arne Ludwig, Andreas D. Wieck, Hermann Sellier, Christopher Bäuerle, Nobu-Hisa Kaneko, Tetsuo Kodera, Shintaro Takada Surface acoustic waves (SAWs) are a reliable solution to transport single electrons with precision in piezoelectric semiconductor devices. Recently, highly efficient single-electron transport with a strongly compressed single-cycle acoustic pulse has been demonstrated. This approach, however, requires surface gates constituting the quantum dots, their wiring, and multiple gate movements to load and unload the electrons, which is very time-consuming. Here, on the contrary, we employ such a single-cycle acoustic pulse in a much simpler way - without any quantum dot at the entrance or exit of a transport channel - to perform single-electron transport between distant electron reservoirs. We observe the transport of a solitary electron in a single-cycle acoustic pulse via the appearance of the quantized acousto-electric current. The simplicity of our approach allows for on-demand electron emission with arbitrary delays on a ns time scale. We anticipate that enhanced synthesis of the SAWs will facilitate electron-quantum-optics experiments with multiple electron flying qubits.
Victor Elhomsy, Luca Planat, David J. Niegemann, Bruna Cardoso-Paz, Ali Badreldin, Bernhard Klemt, Vivien Thiney, Renan Lethiecq, Eric Eyraud, Matthieu C. Dartiailh, Benoit Bertrand, Heimanu Niebojewski, Christopher Bäuerle, Maud Vinet, Tristan Meunier, Nicolas Roch, Matias Urdampilleta Spins in semiconductor quantum dots hold great promise as building blocks of quantum processors. Trapping them in SiMOS transistor-like devices eases future industrial scale fabrication. Among the potentially scalable readout solutions, gate-based dispersive radiofrequency reflectometry only requires the already existing transistor gates to readout a quantum dot state, relieving the need for additional elements. In this effort towards scalability, traveling-wave superconducting parametric amplifiers significantly enhance the readout signal-to-noise ratio (SNR) by reducing the noise below typical cryogenic low-noise amplifiers, while offering a broad amplification band, essential to multiplex the readout of multiple resonators. In this work, we demonstrate a 3GHz gate-based reflectometry readout of electron charge states trapped in quantum dots formed in SiMOS multi-gate devices, with SNR enhanced thanks to a Josephson traveling-wave parametric amplifier (JTWPA). The broad, tunable 2GHz amplification bandwidth combined with more than 10dB ON/OFF SNR improvement of the JTWPA enables frequency and time division multiplexed readout of interdot transitions, and noise performance near the quantum limit. In addition, owing to a design without superconducting loops and with a metallic ground plane, the JTWPA is flux insensitive and shows stable performances up to a magnetic field of 1.2T at the quantum dot device, compatible with standard SiMOS spin qubit experiments.
Bernhard Klemt, Victor El-Homsy, Martin Nurizzo, Pierre Hamonic, Biel Martinez, Bruna Cardoso Paz, Cameron spence, Matthieu Dartiailh, Baptiste Jadot, Emmanuel Chanrion, Vivien Thiney, Renan Lethiecq, Benoit Bertrand, Heimanu Niebojewski, Christopher Bäuerle, Maud Vinet, Yann-Michel Niquet, Tristan Meunier, Matias Urdampilleta For semiconductor spin qubits, complementary-metal-oxide-semiconductor (CMOS) technology is the ideal candidate for reliable and scalable fabrication. Making the direct leap from academic fabrication to qubits fabricated fully by industrial CMOS standards is difficult without intermediate solutions. With a flexible back-end-of-line (BEOL) new functionalities such as micromagnets or superconducting circuits can be added in a post-CMOS process to study the physics of these devices or achieve proof of concepts. Once the process is established it can be incorporated in the foundry-compatible process flow. Here, we study a single electron spin qubit in a CMOS device with a micromagnet integrated in the flexible BEOL. We exploit the synthetic spin orbit coupling (SOC) to control the qubit via electric field and we investigate the spin-valley physics in the presence of SOC where we show an enhancement of the Rabi frequency at the spin-valley hotspot. Finally, we probe the high frequency noise in the system using dynamical decoupling pulse sequences and demonstrate that charge noise dominates the qubit decoherence in this range.
Single-electron sources are an essential component of modern quantum nanoelectronic devices. Owing to their high accuracy and stability, they have been successfully employed for metrology applications, studying fundamental matter interactions and more recently for electron quantum optics. They are traditionally driven by state-of-the-art arbitrary waveform generators that are capable of producing single-electron pulses in the sub-100 ps timescale. In this work, we use an alternative approach for generating ultrashort electron wavepackets. By combining several harmonics provided by a frequency comb, we synthesise Lorentzian voltage pulses and then use them to generate electron wavepackets. Through this technique, we report on the generation and detection of an electron wavepacket with temporal duration of 27 ps generated on top of the Fermi sea of a 2-dimensional electron gas - the shortest reported to date. Electron pulses this short enable studies on elusive, ultrafast fundamental quantum dynamics in nanoelectronic systems and pave the way to implement flying electron qubits by means of Levitons.
We investigate experimentally the capacitive coupling between a two-electron singlet-triplet spin qubit and flying electrons propagating in quantum Hall edge channels. After calibration of the spin qubit detector, we assess its charge sensibility and demonstrate experimentally the detection of less than five flying electrons with average measurement. This experiment demonstrates that the spin qubit is an ultrasensitive and fast charge detector with the perspective of a future single shot-detection of a single flying electron. This work opens the route toward quantum electron optics experiments at the single electron level in semiconductor circuits.
Junliang Wang, Hermann Edlbauer, Aymeric Richard, Shunsuke Ota, Wanki Park, Jeongmin Shim, Arne Ludwig, Andreas Wieck, Heung-Sun Sim, Matias Urdampilleta, Tristan Meunier, Tetsuo Kodera, Nobu-Hisa Kaneko, Hermann Sellier, Xavier Waintal, Shintaro Takada, Christopher Bäuerle Electron flying qubits are envisioned as potential information link within a quantum computer, but also promise -- alike photonic approaches -- a self-standing quantum processing unit. In contrast to its photonic counterpart, electron-quantum-optics implementations are subject to Coulomb interaction, which provide a direct route to entangle the orbital or spin degree of freedom. However, the controlled interaction of flying electrons at the single particle level has not yet been established experimentally. Here we report antibunching of a pair of single electrons that is synchronously shuttled through a circuit of coupled quantum rails by means of a surface acoustic wave. The in-flight partitioning process exhibits a reciprocal gating effect which allows us to ascribe the observed repulsion predominantly to Coulomb interaction. Our single-shot experiment marks an important milestone on the route to realise a controlled-phase gate for in-flight quantum manipulations.
Cameron Spence, Bruna Cardoso-Paz, Vincent Michal, Emmanuel Chanrion, David J. Niegemann, Baptiste Jadot, Pierre-André Mortemousque, Bernhard Klemt, Vivien Thiney, Benoit Bertrand, Louis Hutin, Christopher Bäuerle, Franck Balestro, Maud Vinet, Yann-Michel Niquet, Tristan Meunier, Matias Urdampilleta Charge noise is one of the main sources of environmental decoherence for spin qubits in silicon, presenting a major obstacle in the path towards highly scalable and reproducible qubit fabrication. Here we demonstrate in-depth characterization of the charge noise environment experienced by a quantum dot in a CMOS-fabricated silicon nanowire. We probe the charge noise for different quantum dot configurations, finding that it is possible to tune the charge noise over two orders of magnitude, ranging from 1 ueV^2 to 100 ueV^2. In particular, we show that the top interface and the reservoirs are the main sources of charge noise and their effect can be mitigated by controlling the quantum dot extension. Additionally, we demonstrate a novel method for the measurement of the charge noise experienced by a quantum dot in the few electron regime. We measure a comparatively higher charge noise value of 40 ueV^2 at the first electron, and demonstrate that the charge noise is highly dependent on the electron occupancy of the quantum dot.
Martin Nurizzo, Baptiste Jadot, Pierre-André Mortemousque, Vivien Thiney, Emmanuel Chanrion, David Niegemann, Matthieu Dartiailh, Arne Ludwig, Andreas D. Wieck, Christopher Bäuerle, Matias Urdampilleta, Tristan Meunier We propose and demonstrate complete spin state readout of a two-electron system in a double quantum dot probed by an electrometer. The protocol is based on repetitive single shot measurements using Pauli spin blockade and our ability to tune on fast timescales the detuning and the interdot tunnel coupling between the GHz and sub-Hz regime. A sequence of three distinct manipulations and measurements allows establishing if the spins are in S, Tzero, Tplus or Tminus state. This work points at a procedure to reduce the overhead for spin readout, an important challenge for scaling up spin qubit platforms.
Junliang Wang, Shunsuke Ota, Hermann Edlbauer, Baptiste Jadot, Pierre-André Mortemousque, Aymeric Richard, Yuma Okazaki, Shuji Nakamura, Arne Ludwig, Andreas D. Wieck, Matias Urdampilleta, Tristan Meunier, Tetsuo Kodera, Nobu-Hisa Kaneko, Shintaro Takada, Christopher Bäuerle The synthesis of single-cycle, compressed optical and microwave pulses sparked novel areas of fundamental research. In the field of acoustics, however, such a generation has not been introduced yet. For numerous applications, the large spatial extent of surface acoustic waves (SAW) causes unwanted perturbations and limits the accuracy of physical manipulations. Particularly, this restriction applies to SAW-driven quantum experiments with single flying electrons, where extra modulation renders the exact position of the transported electron ambiguous and leads to undesired spin mixing. Here, we address this challenge by demonstrating single-shot chirp synthesis of a strongly compressed acoustic pulse. Employing this solitary SAW pulse to transport a single electron between distant quantum dots with an efficiency exceeding 99%, we show that chirp synthesis is competitive with regular transduction approaches. Performing a time-resolved investigation of the SAW-driven sending process, we outline the potential of the chirped SAW pulse to synchronize single-electron transport from many quantum-dot sources. By superimposing multiple pulses, we further point out the capability of chirp synthesis to generate arbitrary acoustic waveforms tailorable to a variety of (opto)nanomechanical applications. Our results shift the paradigm of compressed pulses to the field of acoustic phonons and pave the way for a SAW-driven platform of single-electron transport that is precise, synchronized, and scalable.
David J. Niegemann, Victor El-Homsy, Baptiste Jadot, Martin Nurizzo, Bruna Cardoso-Paz, Emmanuel Chanrion, Matthieu Dartiailh, Bernhard Klemt, Vivien Thiney, Christopher Bäuerle, Pierre-André Mortemousque, Benoit Bertrand, Heimanu Niebojewski, Maud Vinet, Franck Balestro, Tristan Meunier, Matias Urdampilleta We demonstrate singlet-triplet readout and parity readout allowing to distinguish T0 and the polarized triplet states. We achieve high fidelity spin readout with an average fidelity above $99.9\%$ for a readout time of $20~\mu$s and $99\%$ for $4~\mu$s at a temperature of $0.5~K$. We initialize a singlet state in a single dot with a fidelity higher than $99\%$ and separate the two electrons while keeping the same spin state with $a \approx 95.6\%$ fidelity.
Martin Nurizzo, Baptiste Jadot, Pierre-André Mortemousque, Vivien Thiney, Emmanuel Chanrion, Matthieu Dartiailh, Arne Ludwig, Andreas D. Wieck, Christopher Bäuerle, Matias Urdampilleta, Tristan Meunier Recent demonstrations using electron spins stored in quantum dots array as qubits are promising for developing a scalable quantum computing platform. An ongoing effort is therefore aiming at the precise control of the quantum dots parameters in larger and larger arrays which represents a complex challenge. Partitioning of the system with the help of the inter-dot tunnel barriers can lead to a simplification for tuning and offers a protection against unwanted charge displacement. In a triple quantum dot system, we demonstrate a nanosecond control of the inter-dot tunnel rate permitting to reach the two extreme regimes, large GHz tunnel coupling and sub-Hz isolation between adjacent dots. We use this novel development to isolate a sub part of the array while performing charge displacement and readout in the rest of the system. The degree of control over the tunnel coupling achieved in a unit cell should motivate future protocol development for tuning, manipulation and readout including this capability.
Hermann Edlbauer, Junliang Wang, Thierry Crozes, Pierre Perrier, Seddik Ouacel, Clément Geffroy, Giorgos Georgiou, Eleni Chatzikyriakou, Antonio Lacerda-Santos, Xavier Waintal, D. Christian Glattli, Preden Roulleau, Jayshankar Nath, Masaya Kataoka, Janine Splettstoesser, Matteo Acciai, Maria Cecilia da Silva Figueira, Kemal Öztas, Alex Trellakis, Thomas Grange, et al (3) The progress of charge manipulation in semiconductor-based nanoscale devices opened up a novel route to realise a flying qubit with a single electron. In the present review, we introduce the concept of these electron flying qubits, discuss their most promising realisations and show how numerical simulations are applicable to accelerate experimental development cycles. Addressing the technological challenges of flying qubits that are currently faced by academia and quantum enterprises, we underline the relevance of interdisciplinary cooperation to move emerging quantum industry forward. The review consists of two main sections: Pathways towards the electron flying qubit: We address three routes of single-electron transport in GaAs-based devices focusing on surface acoustic waves, hot-electron emission from quantum dot pumps and Levitons. For each approach, we discuss latest experimental results and point out how numerical simulations facilitate engineering the electron flying qubit. Numerical modelling of quantum devices: We review the full stack of numerical simulations needed for fabrication of the flying qubits. Choosing appropriate models, examples of basic quantum mechanical simulations are explained in detail. We discuss applications of open-source (KWANT) and the commercial (nextnano) platforms for modelling the flying qubits. The discussion points out the large relevance of software tools to design quantum devices tailored for efficient operation.
In quantum nanoelectronics, numerical simulations have become an ubiquitous tool. Yet the comparison with experiments is often done at a qualitative level or restricted to a single device with a handful of fitting parameters. In this work, we assess the predictive power of these simulations by comparing the results of a single model with a large experimental data set of 110 devices with 48 different geometries. The devices are quantum point contacts of various shapes and sizes made with electrostatic gates deposited on top of a high mobility GaAs/GaAlAs two dimensional electron gas. We study the pinch-off voltages applied on the gates to deplete the two-dimensional electron gas in various spatial positions. We argue that the pinch-off voltages are a very robust signature of the charge distribution in the device. The large experimental data set allows us to critically review the modeling and arrive at a robust one-parameter model that can be calibrated in situ, a crucial step for making predictive simulations.
Hermann Edlbauer, Junliang Wang, Shunsuke Ota, Americ Richard, Baptiste Jadot, Pierre-André Mortemousque, Yuma Okazaki, Shuji Nakamura, Tetsuo Kodera, Nobu-Hisa Kaneko, Arne Ludwig, Andreas D. Wieck, Matias Urdampilleta, Tristan Meunier, Christopher Bäuerle, Shintaro Takada Surface acoustic waves (SAW) have large potential to realize quantum-optics-like experiments with single flying electrons employing their spin or charge degree of freedom. For such quantum applications, highly efficient trapping of the electron in a specific moving quantum dot (QD) of a SAW train plays a key role. Probabilistic transport over multiple moving minima would cause uncertainty in synchronisation that is detrimental for coherence of entangled flying electrons and in-flight quantum operations. It is thus of central importance to identify the device parameters enabling electron transport within a single SAW minimum. A detailed experimental investigation of this aspect is so far missing. Here we fill this gap by demonstrating time-of-flight measurements for a single electron that is transported via a SAW train between distant stationary QDs. Our measurements reveal the in-flight distribution of the electron within the moving acousto-electric quantum dots of the SAW train. Increasing the acousto-electric amplitude, we observe the threshold necessary to confine the flying electron at a specific, deliberately chosen SAW minimum. Investigating the effect of a barrier along the transport channel, we also benchmark the robustness of SAW-driven electron transport against stationary potential variations. Our results pave the way for highly controlled transport of electron qubits in a SAW-driven platform for quantum experiments.
Shintaro Takada, Giorgos Georgiou, Everton Arrighi, Hermann Edlbauer, Yuma Okazaki, Shuji Nakamura, Arne Ludwig, Andreas D. Wieck, Michihisa Yamamoto, Christopher Bäuerle, Nobu-Hisa Kaneko We study the interaction between two closely spaced but electrically isolated quasi-one-dimensional electrical wires by a drag experiment. In this work we experimentally demonstrate the generation of current in an unbiased (drag) wire, which results from the interactions with a neighboring biased (drive) wire. The direction of the drag current depends on the length of the one-dimensional wire with respect to the position of the barrier in the drag wire. When we additionally form a potential barrier in the drive wire, the direction of the drag current is determined by the relative position of the two barriers. We interpret this behavior in terms of electron excitations by phonon-mediated interactions between the two wires in presence of the electron scattering inside the drive wire.
The ability to shuttle coherently individual electron spins in arrays of quantum dots is a key procedure for the development of scalable quantum information platforms. It allows the use of sparsely populated electron spin arrays, envisioned to efficiently tackle the one- and two-qubit gate challenges. When the electrons are displaced in an array, they are submitted to site-dependent environment interactions such as hyperfine coupling with substrate nuclear spins. Here, we demonstrate that the electron multi-directional displacement in a $3\times 3$ array of tunnel coupled quantum dots enhances the spin coherence time via the motional narrowing phenomenon. More specifically, up to 10 configurations are explored by the electrons to study the impact of the displacement on spin dynamics. An increase of the coherence time by a factor up to 10 is observed in case of fast and repetitive displacement. The physical mechanism responsible for the loss of coherence induced by displacement is quantitatively captured by a simple model and its implications on spin coherence properties during the electron displacement are discussed in the context of large-scale quantum circuits.
Quantum communication networks require on-chip transfer and manipulation of single particles as well as their interconversion to single photons for long-range information exchange. Flying excitons propelled by GHz surface acoustic waves (SAWs) are outstanding messengers to fulfill these requirements. Here, we demonstrate the acoustic manipulation of single exciton centers consisting of individual excitons bound to shallow impurities centers embedded in a semiconductor quantum well. Time-resolved photoluminescence studies show that the emission intensity and energy from these centers oscillate at the SAW frequency of 3.5 GHz. Furthermore, these centers can be remotely pumped via acoustic transport of flying excitons along a quantum well channel over several microns. Time correlation studies reveal that the centers emit anti-bunched light, thus acting as single-photon sources operating at GHz frequencies. Our results pave the way for the exciton-based on-demand manipulation and on-chip transfer of single excitons at microwave frequencies with a natural photonic interface.
In the quest for large-scale quantum computing, networked quantum computers offer a natural path towards scalability. Now that nearest neighbor entanglement has been demonstrated for electron spin qubits in semiconductors, on-chip long distance entanglement brings versatility to connect quantum core units. Here we realize the controlled and coherent transfer of a pair of entangled electron spins, and demonstrate their remote entanglement when separated by a distance of 6 microns. Driven by coherent spin rotations induced by the electron displacement, high-contrast spin quantum interferences are observed and are a signature of the preservation of the entanglement all along the displacement procedure. This work opens the route towards fast on-chip deterministic interconnection of remote quantum bits in semiconductor quantum circuits.
Léo Bourdet, Louis Hutin, Benoit Bertrand, Andrea Corna, Heorhii Bohuslavskyi, Anthony Amisse, Alessandro Crippa, Romain Maurand, Sylvain Barraud, Matias Urdampilleta, Christopher Bäuerle, Tristan Meunier, Marc Sanquer, Xavier Jehl, Silvano De Franceschi, Yann-Michel Niquet, Maud Vinet We fabricated Quantum Dot (QD) devices using a standard SOI CMOS process flow, and demonstrated that the spin of confined electrons could be controlled via a local electrical-field excitation, owing to inter-valley spin-orbit coupling. We discuss that modulating the confinement geometry via an additional electrode may enable switching a quantum bit (qubit) between an electrically-addressable valley configuration and a protected spin configuration. This proposed scheme bears relevance to improve the trade-off between fast operations and slow decoherence for quantum computing on a Si qubit platform. Finally, we evoke the impact of process-induced variability on the operating bias range.
L. Hutin, L. Bourdet, B. Bertrand, A. Corna, H. Bohuslavskyi, A. Amisse, A. Crippa, R. Maurand, S. Barraud, M. Urdampilleta, C. Bäuerle, T. Meunier, M. Sanquer, X. Jehl, S. De Franceschi, Y.-M. Niquet, M. Vinet We successfully demonstrated experimentally the electrical-field-mediated control of the spin of electrons confined in an SOI Quantum Dot (QD) device fabricated with a standard CMOS process flow. Furthermore, we show that the Back-Gate control in SOI devices enables switching a quantum bit (qubit) between an electrically-addressable, yet charge noise-sensitive configuration, and a protected configuration.
Shintaro Takada, Hermann Edlbauer, Hugo V. Lepage, Junliang Wang, Pierre-André Mortemousque, Giorgos Georgiou, Crispin H. W. Barnes, Chris J. B. Ford, Mingyun Yuan, Paulo V. Santos, Xavier Waintal, Arne Ludwig, Andreas D. Wieck, Matias Urdampilleta, Tristan Meunier, Christopher Bäuerle Surface acoustic waves (SAWs) strongly modulate the shallow electric potential in piezoelectric materials. In semiconductor heterostructures such as GaAs/AlGaAs, SAWs can thus be employed to transfer individual electrons between distant quantum dots. This transfer mechanism makes SAW technologies a promising candidate to convey quantum information through a circuit of quantum logic gates. Here we present two essential building blocks of such a SAW-driven quantum circuit. First, we implement a directional coupler allowing to partition a flying electron arbitrarily into two paths of transportation. Second, we demonstrate a triggered single-electron source enabling synchronisation of the SAW-driven sending process. Exceeding a single-shot transfer efficiency of 99 %, we show that a SAW-driven integrated circuit is feasible with single electrons on a large scale. Our results pave the way to perform quantum logic operations with flying electron qubits.
The ability to manipulate coherently individual quantum objects organized in arrays is a prerequisite to any scalable quantum information platform. For electron spin qubits, it requires the fine tuning of large arrays of tunnel-coupled quantum dots. The cumulated efforts in linear dot arrays have permitted the recent realization of quantum simulators and multi-electron spin coherent manipulation. However, the two-dimensional scaling of such implementations remains undemonstrated while being compulsory to resolve complex quantum matter problems or process quantum information. Here, we demonstrate the two-dimensional coherent control of individual electron spins in a 3x3 array of tunnel-coupled quantum dots. More specifically, we focus on several key quantum functionalities of such control: charge deterministic displacement, local spin readout, local coherent exchange manipulation between two electron spins trapped in adjacent dots, and coherent multi-directional spin shuttling over distances of several microns. This work lays the foundations for exploiting a two-dimensional array of electron spins for quantum simulation and information processing.
In this report we review the present state of the art of the control of propagating quantum states at the single-electron level and its potential application to quantum information processing. We give an overview of the different approaches which have been developed over the last ten years in order to gain full control over a propagating single electron in a solid state system. After a brief introduction of the basic concepts, we present experiments on flying qubit circuits for ensemble of electrons measured in the low frequency (DC) limit. We then present the basic ingredients necessary to realise such experiments at the single-electron level. This includes a review of the various single electron sources which are compatible with integrated single electron circuits. This is followed by a review of recent key experiments on electron quantum optics with single electrons. Finally we will present recent developments about the new physics that emerges using ultrashort voltage pulses. We conclude our review with an outlook and future challenges in the field.
Gregoire Roussely, Everton Arrighi, Giorgos Georgiou, Shintaro Takada, Martin Schalk, Matias Urdampilleta, Arne Ludwig, Andreas D. Wieck, Pacome Armagnat, Thomas Kloss, Xavier Waintal, Tristan Meunier, Christopher Bauerle Quantum dynamics is very sensitive to dimensionality. While two-dimensional electronic systems form Fermi liquids, one-dimensional systems -- Tomonaga-Luttinger liquids -- are described by purely bosonic excitations, even though they are initially made of fermions. With the advent of coherent single-electron sources, the quantum dynamics of such a liquid is now accessible at the single-electron level. Here, we report on time-of-flight measurements of ultrashort few-electron charge pulses injected into a quasi one-dimensional quantum conductor. By changing the confinement potential we can tune the system from the one-dimensional Tomonaga-Luttinger liquid limit to the multi-channel Fermi liquid and show that the plasmon velocity can be varied over almost an order of magnitude. These results are in quantitative agreement with a parameter-free theory and demonstrate a powerful new probe for directly investigating real-time dynamics of fractionalisation phenomena in low-dimensional conductors.
Solid-state approaches to quantum information technology are attractive because they are scalable. The coherent transport of quantum information over large distances, as required for a practical quantum computer, has been demonstrated by coupling solid-state qubits to photons1. As an alternative approach for a spin-based quantum computer, single electrons have also been transferred between distant quantum dots in times faster than their coherence time2, 3. However, there have been no demonstrations to date of techniques that can coherently transfer scalable qubits and perform quantum operations on them at the same time. The resulting so-called flying qubits are attractive because they allow for control over qubit separation and non-local entanglement with static gate voltages, which is a significant advantage over other solid-state qubits in confined systems for integration of quantum circuits. Here we report the transport and manipulation of qubits over distances of 6 microns within 40 ps, in an Aharonov-Bohm ring connected to two-channel wires that have a tunable tunnel coupling between channels. The flying qubit state is defined by the presence of a travelling electron in either channel of the wire, and can be controlled without a magnetic field. Our device has shorter quantum gates, longer coherence lengths (~86 \mum at 70 mK), and shorter operation times (~10 ps or 100 GHz) than other solid-state flying qubit implementations4, 5, which makes our solid-state flying qubit potentially scalable.
The transmission phase across a quantum dot (QD) is expected to show mesoscopic behavior, where the appearance of a phase lapse between Coulomb peaks (CPs) as a function of the gate voltage depends on the orbital parity relation between the corresponding CPs. On the other hand, such mesoscopic behavior has been observed only in a limited QD configuration (a few-electron and single-level transport regime) and universal phase lapses by $\pi$ between consecutive CPs have been reported for all the other configurations. Here, we report on the measurement of a transmission phase across a QD around the crossover between single-level and multilevel transport regimes employing an original two-path quantum interferometer. We find mesoscopic behavior for the studied QD. Our results show that the universal phase lapse, a longstanding puzzle of the phase shift, is absent for a standard QD, where several tens of successive well-separated CPs are observed.
The electron wave function experiences a phase modification at coherent transmission through a quantum dot. This transmission phase undergoes a characteristic shift of $\pi$ when scanning through a Coulomb-blockade resonance. Between successive resonances either a transmission phase lapse of $\pi$ or a phase plateau is theoretically expected to occur depending on the parity of the corresponding quantum dot states. Despite considerable experimental effort, this transmission phase behaviour has remained elusive for a large quantum dot. Here we report on transmission phase measurements across such a large quantum dot hosting hundreds of electrons. Using an original electron two-path interferometer to scan the transmission phase along fourteen successive resonances, we observe both phase lapses and plateaus. Additionally, we demonstrate that quantum dot deformation alters the sequence of transmission phase lapses and plateaus via parity modifications of the involved quantum dot states. Our findings set a milestone towards a comprehensive understanding of the transmission phase of quantum dots.
The scaling up of electron spin qubit based nanocircuits has remained challenging up to date and involves the development of efficient charge control strategies. Here we report on the experimental realization of a linear triple quantum dot in a regime isolated from the reservoir. We show how this regime can be reached with a fixed number of electrons. Charge stability diagrams of the one, two and three electron configurations where only electron exchange between the dots is allowed are observed. They are modelled with established theory based on a capacitive model of the dot systems. The advantages of the isolated regime with respect to experimental realizations of quantum simulators and qubits are discussed. We envision that the results presented here will make more manipulation schemes for existing qubit implementations possible and will ultimately allow to increase the number of tunnel coupled quantum dots which can be simultaneously controlled.
We demonstrate evidences of electronic transport via topological Dirac surface states in a thin film of strained HgTe. At high perpendicular magnetic fields, we show that the electron transport reaches the quantum Hall regime with vanishing resistance. Furthermore, quantum Hall transport spectroscopy reveals energy splittings of relativistic Landau levels specific to coupled Dirac surface states. This study provides new insights in the quantum Hall effect of topological insulator (TI) slabs, in the cross-over regime between two- and three-dimensional TIs, and in the relevance of thin TI films to explore novel circuit functionalities in spintronics and quantum nanoelectronics.
Controlling nanocircuits at the single electron spin level is a possible route for large-scale quantum information processing. In this context, individual electron spins have been identified as versatile quantum information carriers to interconnect different nodes of a spin-based semiconductor quantum circuit. Despite important experimental efforts to control the electron displacement over long distances, keeping the electron spin coherence after transfer remained up to now elusive. Here we demonstrate that individual electron spins can be displaced coherently over a distance of 5 micrometers. This displacement is realized on a closed path made of three tunnel-coupled lateral quantum dots. Using fast quantum dot control, the electrons tunnel from one dot to another at a speed approaching 100 m/s. We find that the spin coherence length is 8 times longer than expected from the electron spin coherence without displacement. Such an enhanced spin coherence points at a process similar to motional narrowing observed in nuclear magnetic resonance experiments6. The demonstrated coherent displacement will enable long-range interaction between distant spin-qubits and will open the route towards non-abelian and holonomic manipulation of a single electron spin.
We study the transmission phase shift across a Kondo correlated quantum dot in a GaAs heterostructure at temperatures below the Kondo temperature ($T < T_{\rm K}$), where the phase shift is expected to show a plateau at $\pi/2$ for an ideal Kondo singlet ground state. Our device is tuned such that the ratio $\Gamma/U$ of level width $\Gamma$ to charging energy $U$ is quite large ($\lesssim 0.5$ rather than $\ll 1$). This situation is commonly used in GaAs quantum dots to ensure Kondo temperatures large enough ($\simeq 100$ mK here) to be experimentally accessible; however it also implies that charge fluctuations are more pronounced than typically assumed in theoretical studies focusing on the regime $\Gamma/U \ll 1$ needed to ensure a well-defined local moment. Our measured phase evolves monotonically by $\pi$ across the two Coulomb peaks, but without being locked at $\pi/2$ in the Kondo valley for $T \ll T_{\rm K}$, due to a significant influence of large $\Gamma/U$. Only when $\Gamma/U$ is reduced sufficiently does the phase start to be locked around $\pi/2$ and develops into a plateau at $\pi/2$. Our observations are consistent with numerical renormalization group calculations, and can be understood as a direct consequence of the Friedel sum rule that relates the transmission phase shift to the local occupancy of the dot, and thermal average of a transmission coefficient through a resonance level near the Fermi energy.
We study the injection mechanism of a single electron from a static quantum dot into a moving quantum dot created in a long depleted channel with surface acoustic waves (SAWs). We demonstrate that such a process is characterized by an activation law with a threshold that depends on the SAW amplitude and the dot-channel potential gradient. By increasing sufficiently the SAW modulation amplitude, we can reach a regime where the transfer is unitary and potentially adiabatic. This study points at the relevant regime to use moving dots in quantum information protocols.
Transporting ensembles of electrons over long distances without losing their spin polarization is an important benchmark for spintronic devices. It requires usually to inject and to probe spin polarized electrons in conduction channels using ferromagnetic contacts or optical excitation. Parallel to this development, an important effort has been dedicated to the control of nanocircuits at the single electron level. The detection and the coherent manipulation of the spin of a single electron trapped in a quantum dot are now well established. Combined with the recent control of the displacement of individual electrons between two distant quantum dots, these achievements permit to envision the realization of spintronic protocols at the single electron level. Here, we demonstrate that spin information carried by one or two electrons can be transferred between two quantum dots separated by a distance of 4 micrometers with a classical fidelity of 65 %. We show that it is presently limited by spin flips occurring during the transfer procedure prior to and after the electron displacement. Being able to encode and control information in the spin degree of freedom of a single electron while being transferred over distances of a few microns on nanosecond timescales paves the way towards "quantum spintronics" devices where large scale spin-based quantum information processing could be implemented.
A quantum two-path interferometer allows for direct measurement of the transmission phase shift of an electron, providing useful information on coherent scattering problems. In mesoscopic systems, however, the two-path interference is easily smeared by contributions from other paths, and this makes it difficult to observe the \textittrue transmission phase shift. To eliminate this problem, multi-terminal Aharonov-Bohm (AB) interferometers have been used to derive the phase shift by assuming that the relative phase shift of the electrons between the two paths is simply obtained when a smooth shift of the AB oscillations is observed. Nevertheless the phase shifts using such a criterion have sometimes been inconsistent with theory. On the other hand, we have used an AB ring contacted to tunnel-coupled wires and acquired the phase shift consistent with theory when the two output currents through the coupled wires oscillate with well-defined anti-phase. Here, we investigate thoroughly these two criteria used to ensure a reliable phase measurement, the anti-phase relation of the two output currents and the smooth phase shift in the AB oscillation. We confirm that the well-defined anti-phase relation ensures a correct phase measurement with a quantum two-path interference. In contrast we find that even in a situation where the anti-phase relation is less well-defined, the smooth phase shift in the AB oscillation can still occur but does not give the correct transmission phase due to contributions from multiple paths. This indicates that the phase relation of the two output currents in our interferometer gives a good criterion for the measurement of the \textittrue transmission phase while the smooth phase shift in the AB oscillation itself does not.
We studied experimentally the dynamics of the exchange interaction between two antiparallel electron spins in a so-called metastable double quantum dot where coupling to the electron reservoirs can be ignored. We demonstrate that the level of control of such a double dot is higher than in conventional double dots. In particular, it allows to couple coherently two electron spins in an efficient manner following a scheme initially proposed by Loss and DiVincenzo. The present study demonstrates that metastable quantum dots are a possible route to increase the number of coherently coupled quantum dots.
We investigate experimentally the capacitive coupling between a two-electron spin qubit and flying electrons propagating in quantum Hall edge channels. We demonstrate that the qubit is an ultrasensitive and fast charge detector with the potential to allow single shot detection of a single flying electron. This work opens the route towards quantum electron optics at the single electron level above the Fermi sea.
In this work we present the fabrication and characterization of superconducting nano-mechanical resonators made from nanocrystalline boron doped diamond (BDD). The oscillators can be driven and read out in their superconducting state and show quality factors as high as 40,000 at a resonance frequency of around 10 MHz. Mechanical damping is studied for magnetic fields up to 3 T where the resonators still show superconducting properties. Due to their simple fabrication procedure, the devices can easily be coupled to other superconducting circuits and their performance is comparable with state-of-the-art technology.
We discuss an electronic interferometer recently measured by Yamamoto et al. This "flying quantum bit" experiment showed quantum oscillations between electronic trajectories of two tunnel-coupled wires connected via an Aharanov-Bohm ring. We present a simple scattering model as well as a numerical microscopic model to describe this experiment. In addition, we present new experimental data to which we confront our numerical results. While our analytical model provides basic concepts for designing the flying qubit device, we find that our numerical simulations allow to reproduce detailed features of the transport measurements such as in-phase and anti-phase oscillations of the two output currents as well as a smooth phase shift when sweeping a side gate. Furthermore, we find remarkable resemblance for the magneto conductance oscillations in both conductance and visibility between simulations and experiments within a specific parameter range.
S. Takada, C. Bäuerle, M. Yamamoto, K. Watanabe, S. Hermelin, T. Meunier, A. Alex, A. Weichselbaum, J. von Delft, A. Ludwig, A. D. Wieck, S. Tarucha We report on the direct observation of the transmission phase shift through a Kondo correlated quantum dot by employing a new type of two-path interferometer. We observed a clear $\pi/2$-phase shift, which persists up to the Kondo temperature $T_{\rm K}$. Above this temperature, the phase shifts by more than $\pi/2$ at each Coulomb peak, approaching the behavior observed for the standard Coulomb blockade regime. These observations are in remarkable agreement with 2-level numerical renormalization group calculations. The unique combination of experimental and theoretical results presented here fully elucidates the phase evolution in the Kondo regime.
We consider iron impurities in the noble metals gold and silver and compare experimental data for the resistivity and decoherence rate to numerical renormalization group results. By exploiting non-Abelian symmetries we show improved numerical data for both quantities as compared to previous calculations [Costi et al., Phys. Rev. Lett. 102, 056802 (2009)], using the discarded weight as criterion to reliably judge the quality of convergence of the numerical data. In addition we also carry out finite-temperature calculations for the magnetoresistivity of fully screened Kondo models with S = 1/2, 1 and 3/2, and compare the results with available measurements for iron in silver, finding excellent agreement between theory and experiment for the spin-3/2 three-channel Kondo model. This lends additional support to the conclusion of Costi et al. that the latter model provides a good effective description of the Kondo physics of iron impurities in gold and silver.
We observe the electron spin resonance of conduction electrons in boron doped (6400 ppm) superconducting diamond (Tc =3.8 K). We clearly identify the benchmarks of conduction electron spin resonance (CESR): the nearly temperature independent ESR signal intensity and its magnitude which is in good agreement with that expected from the density of states through the Pauli spin-susceptibility. The temperature dependent CESR linewidth weakly increases with increasing temperature which can be understood in the framework of the Elliott-Yafet theory of spin-relaxation. An anomalous and yet unexplained relation is observed between the g-factor, CESR linewidth, and the resistivity using the empirical Elliott-Yafet relation.
We have measured Universal Conductance Fluctuations in the metallic spin glass Ag:Mn as a function of temperature and magnetic field. From this measurement, we can access the phase coherence time of the electrons in the spin glass. We show that this phase coherence time increases with both the inverse of the temperature and the magnetic field. From this we deduce that decoherence mechanisms are still active even deep in the spin glass phase.
We report the realization of a quadruple quantum dot device in a square-like configuration where a single electron can be transferred on a closed path free of other electrons. By studying the stability diagrams of this system, we demonstrate that we are able to reach the few-electron regime and to control the electronic population of each quantum dot with gate voltages. This allows us to control the transfer of a single electron on a closed path inside the quadruple dot system. This work opens the route towards electron spin manipulation using spin-orbit interaction by moving an electron on complex paths free of electrons
The light scattering properties of superconducting (Tc=3.8 K) heavily boron doped nanocrystalline diamond has been investigated by Raman spectroscopy using visible excitations. Fano type interference of the zone-center phonon line and the electronic continuum was identified. Lineshape analysis reveals Fano lineshapes with a significant asymmetry (q=-2). An anomalous wavelength dependence and small value of the Raman scattering amplitude is observed in agreement with previous studies.
We report low-temperature transport measurements through a double quantum dot device in a configuration where one of the quantum dots is coupled directly to the source and drain electrodes, and a second (side-coupled) quantum dot interacts electrostatically and via tunneling to the first one. As the interdot coupling increases, a crossover from weak to strong interdot tunneling is observed in the charge stability diagrams that present a complex pattern with mergings and apparent crossings of Coulomb blockade peaks. While the weak coupling regime can be understood by considering a single level on each dot, in the intermediate and strong coupling regimes, the multi-level nature of the quantum dots needs to be taken into account. Surprisingly, both in the strong and weak coupling regimes, the double quantum dot states are mainly localized on each dot for most values of the parameters. Only in an intermediate coupling regime the device presents a single dot-like molecular behavior as the molecular wavefunctions weight is evenly distributed between the quantum dots. At temperatures larger than the interdot coupling energy scale, a loss of coherence of the molecular states is observed.
Diamond is an electrical insulator in its natural form. However, when doped with boron above a critical level (~0.25 at.%) it can be rendered superconducting at low temperatures with high critical fields. Here we present the realization of a micrometer scale superconducting quantum interference device $\mu$-SQUID made from nanocrystalline boron doped diamond (BDD) films. Our results demonstrate that $\mu$-SQUIDs made from superconducting diamond can be operated in magnetic fields as large as 4T independent on the field direction. This is a decisive step towards the detection of quantum motion in a diamond based nanomechanical oscillator.
Electrons in a metal are indistinguishable particles that strongly interact with other electrons and their environment. Isolating and detecting a single flying electron after propagation to perform quantum optics like experiments at the single electron level is therefore a challenging task. Up to date, only few experiments have been performed in a high mobility two-dimensional electron gas where the electron propagates almost ballistically. Flying electrons were detected via the current generated by an ensemble of electrons and electron correlations were encrypted in the current noise. Here we demonstrate the experimental realisation of high efficiency single electron source and single electron detector for a quantum medium where a single electron is propagating isolated from the other electrons through a one-dimensional channel. The moving potential is excited by a surface acoustic wave, which carries the single electron along the 1D-channel at a speed of 3\mum/ns. When such a quantum channel is placed between two quantum dots, a single electron can be transported from one quantum dot to the other, which is several micrometres apart, with a quantum efficiency of emission and detection of 96% and 92%, respectively. Furthermore, the transfer of the electron can be triggered on a timescale shorter than the coherence time T2* of GaAs spin qubits6. Our work opens new avenues to study the teleportation of a single electron spin and the distant interaction between spatially separated qubits in a condensed matter system.
Noise filtering is an essential part for measurement of quantum phenomena at extremely low temperatures. Here, we present the design of a filter which can be installed in space constrained cryogenic environment containing a large number of signal carrying lines. Our filters have a -3db point of 65kHz and its performance at GHz frequencies are comparable to the best available RF filters.
We have measured the low temperature electrical resistivity of Ag : Mn mesoscopic spin glasses prepared by ion implantation with a concentration of 700 ppm. As expected, we observe a clear maximum in the resistivity (T ) at a temperature in good agreement with theoretical predictions. Moreover, we observe remanence effects at very weak magnetic fields for the resistivity below the freezing temperature Tsg: upon Field Cooling (fc), we observe clear deviations of (T ) as compared with the Zero Field Cooling (zfc); such deviations appear even for very small magnetic fields, typically in the Gauss range. This onset of remanence for very weak magnetic fields is reminiscent of the typical signature on magnetic susceptibility measurements of the spin glass transition for this generic glassy system.
We report on the transport properties of nanostructures made from boron-doped superconducting diamond. Starting from nanocrystalline superconducting boron-doped diamond thin films, grown by Chemical Vapor Deposition, we pattern by electron-beam lithography devices with dimensions in the nanometer range. We show that even for such small devices, the superconducting properties of the material are well preserved: for wires of width less than $100\, nm$, we measure critical temperatures in the Kelvin range and critical field in the Tesla range.
We study the disorder dependence of the phase coherence time of quasi one-dimensional wires and two-dimensional (2D) Hall bars fabricated from a high mobility GaAs/AlGaAs heterostructure. Using an original ion implantation technique, we can tune the intrinsic disorder felt by the 2D electron gas and continuously vary the system from the semi-ballistic regime to the localized one. In the diffusive regime, the phase coherence time follows a power law as a function of diffusion coefficient as expected in the Fermi liquid theory, without any sign of low temperature saturation. Surprisingly, in the semi-ballistic regime, it becomes independent of the diffusion coefficient. In the strongly localized regime we find a diverging phase coherence time with decreasing temperature, however, with a smaller exponent compared to the weakly localized regime.
T. A. Costi, L. Bergqvist, A. Weichselbaum, J. von Delft, T. Micklitz, A. Rosch, P. Mavropoulos, P. H. Dederichs, F. Mallet, L. Saminadayar, C. Bauerle We exploit the decoherence of electrons due to magnetic impurities, studied via weak localization, to resolve a longstanding question concerning the classic Kondo systems of Fe impurities in the noble metals gold and silver: which Kondo-type model yields a realistic description of the relevant multiple bands, spin and orbital degrees of freedom? Previous studies suggest a fully screened spin $S$ Kondo model, but the value of $S$ remained ambiguous. We perform density functional theory calculations that suggest $S = 3/2$. We also compare previous and new measurements of both the resistivity and decoherence rate in quasi 1-dimensional wires to numerical renormalization group predictions for $S=1/2,1$ and 3/2, finding excellent agreement for $S=3/2$.
We present phase coherence time measurements in quasi-one-dimensional mesoscopic wires made from high mobility two-dimensional electron gas. By implanting gallium ions into a GaAs/AlGaAs heterojunction we are able to vary the diffusion coefficient over 2 orders of magnitude. We show that in the diffusive limit, the decoherence time follows a power law as a function of diffusion coefficient as expected by theory. When the disorder is low enough so that the samples are semi-ballistic, we observe a new and unexpected regime in which the phase coherence time is independent of disorder. In addition, for all samples the temperature dependence of the phase coherence time follows a power law down to the lowest temperatures without any sign of saturation and strongly suggests that the frequently observed low temperature saturation is not intrinsic.
We present phase coherence time measurements in quasi-one-dimensional Ag wires implanted with Ag$^{+}$ ions with an energy of $100 keV$. The measurements have been carried out in the temperature range from $100 mK$ up to $10 K$; this has to be compared with the Kondo temperature of iron in silver, i.e. $T_{K}^{Ag/Fe} \approx 4 K$, used in recent experiments on dephasing in Kondo systems\citemallet_prl_06,birge_prl_06. We show that the phase coherence time is not affected by the implantation procedure, clearly proving that ion implantation process by itself \emphdoes not lead to any extra dephasing at low temperature.
We review recent experimental progress on the saturation problem in metallic quantum wires. In particular, we address the influence of magnetic impurities on the electron phase coherence time. We also present new measurements of the phase coherence time in ultra-clean gold and silver wires and analyse the saturation of \tauphi in these samples, cognizant of the role of magnetic scattering. For the cleanest samples, Kondo temperatures below 1 mK and extremely-small magnetic-impurity concentration levels of less than 0.08 ppm have to be assumed to attribute the observed saturation to the presence of magnetic impurities.
Review article on equilibrium properties of mesoscopic quantum conductors.
We report on magnetoconductance measurements of metallic networks of various sizes ranging from 10 to $10^{6}$ plaquettes, with anisotropic aspect ratio. Both Altshuler-Aronov-Spivak (AAS) $h/2e$ periodic oscillations and Aharonov-Bohm (AB) $h/e$ periodic oscillations are observed for all networks. For large samples, the amplitude of both oscillations results from the incoherent superposition of contributions of phase coherent regions. When the transverse size becomes smaller than the phase coherent length $L_\phi$, one enters a new regime which is phase coherent (mesoscopic) along one direction and macroscopic along the other, leading to a new size dependence of the quantum oscillations.
F. Mallet, J. Ericsson, D. Mailly, S. Unlubayir, D. Reuter, A. Melnikov, A.D. Wieck, T. Micklitz, A. Rosch, T.A. Costi, L. Saminadayar, C. Bauerle We present phase coherence time measurements in quasi-one-dimensional Ag wires doped with Fe Kondo impurities of different concentrations $n_s$. Due to the relatively high Kondo temperature $T_{K}\approx 4.3K$ of this system, we are able to explore a temperature range from above $T_{K}$ down to below $0.01 T_{K}$. We show that the magnetic contribution to the dephasing rate $\gamma_m$ per impurity is described by a single, universal curve when plotted as a function of $(T/T_K)$. For $T>0.1 T_K$, the dephasing rate is remarkably well described by recent numerical results for spin $S=1/2$ impurities. At lower temperature, we observe deviations from this theory. Based on a comparison with theoretical calculations for $S>1/2$, we discuss possible explanations for the observed deviations.
We present measurements of the phase coherence time \tauphi in quasi one-dimensional Au/Fe Kondo wires and compare the temperature dependence of \tauphi with a recent theory of inelastic scattering from magnetic impurities (Phys. Rev. Lett. 93, 107204 (2004)). A very good agreement is obtained for temperatures down to 0.2 $T_K$. Below the Kondo temperature $T_K$, the inverse of the phase coherence time varies linearly with temperature over almost one decade in temperature.
We report on magnetotransport measurements performed on a large metallic two-dimensional $\mathcal{T}_{3}$ network. Superimposed on the conventional Altshuler-Aronov-Spivak (AAS) oscillations of period $h/2e$, we observe clear $h/e$ oscillations in magnetic fields up to $8 T$. Different interpretations of this phenomenon are proposed.
We present measurements of the magnetoresistance of long and narrow quasi one-dimensional gold wires containing magnetic iron impurities. The electron phase coherence time extracted from the weak antilocalisation shows a pronounced plateau in a temperature region of 300 mK - 800 mK, associated with the phase breaking due to the Kondo effect. Below the Kondo temperature, the phase coherence time increases, as expected in the framework of Kondo physics. At much lower temperatures, the phase coherence time saturates again, in contradiction with standard Fermi liquid theory. In the same temperature regime, the resistivity curve displays a characteristic maximum at zero magnetic field, associated with the formation of a spin glass state. We argue that the interactions between the magnetic moments are responsible for the low temperature saturation of the phase coherence time.
We present measurements of the magnetoconductance of long and narrow quasi one-dimensional gold wires containing magnetic iron impurities in a temperature range extending from $15 $mK to $4.2 $K. The dephasing rate extracted from the weak antilocalisation shows a pronounced plateau in a temperature region of $300 $mK - $800 $mK, associated with the phase breaking due to the Kondo effect. Below the Kondo temperature the dephasing rate decreases linearly with temperature, in contradiction with standard Fermi-liquid theory. Our data suggest that the formation of a spin glass due to the interactions between the magnetic moments are responsible for the observed anomalous temperature dependence.