Terahertz lies at the juncture between RF and optical electromagnetism, serving as a transition from mm-Wave to infrared photonics. Terahertz technology has been used for industrial quality control, security imaging, and high-speed communications, and often generated through optoelectronic solutions by using photoconductive antennas. In this paper, Multiphysics simulations on semi insulating GaAs, grapheneenhanced photoconductive antennas are conducted to effectively decouple optical responses of semiconductor carrier generation/drift from Terahertz radiation computation, which provides a comprehensive and integrated platform for future terahertz photoconductive antenna designs
X-ray diffraction (XRD) is an essential technique to determine a material's crystal structure in high-throughput experimentation, and has recently been incorporated in artificially intelligent agents in autonomous scientific discovery processes. However, rapid, automated and reliable analysis method of XRD data matching the incoming data rate remains a major challenge. To address these issues, we present CrystalShift, an efficient algorithm for probabilistic XRD phase labeling that employs symmetry-constrained pseudo-refinement optimization, best-first tree search, and Bayesian model comparison to estimate probabilities for phase combinations without requiring phase space information or training. We demonstrate that CrystalShift provides robust probability estimates, outperforming existing methods on synthetic and experimental datasets, and can be readily integrated into high-throughput experimental workflows. In addition to efficient phase-mapping, CrystalShift offers quantitative insights into materials' structural parameters, which facilitate both expert evaluation and AI-based modeling of the phase space, ultimately accelerating materials identification and discovery.
Recent experimental realizations of the lattice Schwinger model [Nature 587, 392 (2020) and Science 367, 1128 (2020)] open a door for quantum simulation of elementary particles and their interactions using ultracold atoms, in which the matter and gauge fields are constrained by a local U(1) gauge invariance known as the Gauss's law. Stimulated by such exciting progress, we propose a new scenario in simulating the lattice Schwinger model in a spin-1 Bose-Einstein condensate. It is shown that our model naturally contains an interaction of the matter fields which respects the U(1) gauge symmetry but has no counterpart in the conventional Schwinger model. In addition to the Z2-ordered phase identified in the previous work, this additional interaction leads to a new Z3-ordered phase. We map out a rich phase diagram and identify that the continuous phase transitions from the disordered to the Z2-ordered and the Z3-ordered phases belong to the Ising and the 3-state Potts universality classes, respectively. Furthermore, the two ordered phases each possess a set of quantum scars which give rise to anomalous quantum dynamics when quenched to a special point in the phase diagram. Our proposal provides a novel platform for extracting emergent physics in cold-atom-based quantum simulators with gauge symmetries.
Autonomous experimentation enabled by artificial intelligence (AI) offers a new paradigm for accelerating scientific discovery. Non-equilibrium materials synthesis is emblematic of complex, resource-intensive experimentation whose acceleration would be a watershed for materials discovery and development. The mapping of non-equilibrium synthesis phase diagrams has recently been accelerated via high throughput experimentation but still limits materials research because the parameter space is too vast to be exhaustively explored. We demonstrate accelerated synthesis and exploration of metastable materials through hierarchical autonomous experimentation governed by the Scientific Autonomous Reasoning Agent (SARA). SARA integrates robotic materials synthesis and characterization along with a hierarchy of AI methods that efficiently reveal the structure of processing phase diagrams. SARA designs lateral gradient laser spike annealing (lg-LSA) experiments for parallel materials synthesis and employs optical spectroscopy to rapidly identify phase transitions. Efficient exploration of the multi-dimensional parameter space is achieved with nested active learning (AL) cycles built upon advanced machine learning models that incorporate the underlying physics of the experiments as well as end-to-end uncertainty quantification. With this, and the coordination of AL at multiple scales, SARA embodies AI harnessing of complex scientific tasks. We demonstrate its performance by autonomously mapping synthesis phase boundaries for the Bi$_2$O$_3$ system, leading to orders-of-magnitude acceleration in establishment of a synthesis phase diagram that includes conditions for kinetically stabilizing $\delta$-Bi$_2$O$_3$ at room temperature, a critical development for electrochemical technologies such as solid oxide fuel cells.
Duncan R. Sutherland, Aine Boyer Connolly, Maximilian Amsler, Ming-Chiang Chang, Katie Rose Gann, Vidit Gupta, Sebastian Ament, Dan Guevarra, John M. Gregoire, Carla P. Gomes, R. B. van Dover, Michael O. Thompson Recent advances in high-throughput experimentation for combinatorial studies have accelerated the discovery and analysis of materials across a wide range of compositions and synthesis conditions. However, many of the more powerful characterization methods are limited by speed, cost, availability, and/or resolution. To make efficient use of these methods, there is value in developing approaches for identifying critical compositions and conditions to be used as a-priori knowledge for follow-up characterization with high-precision techniques, such as micron-scale synchrotron based X-ray diffraction (XRD). Here we demonstrate the use of optical microscopy and reflectance spectroscopy to identify likely phase-change boundaries in thin film libraries. These methods are used to delineate possible metastable phase boundaries following lateral-gradient Laser Spike Annealing (lg-LSA) of oxide materials. The set of boundaries are then compared with definitive determinations of structural transformations obtained using high-resolution XRD. We demonstrate that the optical methods detect more than 95% of the structural transformations in a composition-gradient La-Mn-O library and a Ga$_2$O$_3$ sample, both subject to an extensive set of lg-LSA anneals. Our results provide quantitative support for the value of optically-detected transformations as a priori data to guide subsequent structural characterization, ultimately accelerating and enhancing the efficient implementation of $\mu$m-resolution XRD experiments.
Fei Jiao, Jingfeng Wang, Xianyu Wang, Meixia Chang, Lingbo Cai, Shu Zhu, Di Zhang, Qing Lu, Cao Wang, Shugang Tan, Yunlong Li, Jiayuan Hu, Qiang Jing, Bo Liu, Dong Qian The antiferromagnetic topological insulator has attracted lots of attention recently, as its intrinsic magnetism and topological property makes it a potential material to realize the quantum anomalous Hall effect (QAHE) at relative high temperature. Until now, only MnBi$_2$Te$_4$ is predicted and grown successfully. The other MB$_2$T$_4$-family materials predicted (MB$_2$T$_4$:M=transition-metal or rare-earth element, B=Bi or Sb, T=Te, Se, or S) with not only antiferromagnetic topological property but also rich and exotic topological quantum states and dynamically stable (or metastable) structure have not been realized on experiment completely. Here, MnBi$_2$Te$_4$ single crystals have been grown successfully and tested. It shows typical antiferromagnetic character, with Neel temperature of 24.5K and a spin-flop transition at H$\thickapprox$35000 Oe, 1.8K. After obtaining MnBi$_2$Te$_4$ single crystals, we have tried to synthesize the other members of MB$_2$T$_4$-family materials, but things are not going so well. Then it inspires us to discuss the growth mechanism of MnBi$_2$Te$_4$. The growth mode may be the layer-inserting growth mode based on symmetry, which is supported by our X-ray photoelectron spectroscopy (XPS) measurement. The XPS measurement combing with the $Ar^+$ ion sputtering is done to investigate the chemical state of MnBi$_2$Te$_4$. Binding energies (BE) of the MnBi$_2$Te$_4$-related contributions to Mn2p and Te3d spectra agree well with those of inserting material $\alpha$-MnTe. Rising intensity of the Mn2p satellite for divalent Mn (bound to chalcogen) with atomic number of ligand (from MnO to MnBi$_2$Te$_4$) has been observed, thus suggesting classification of MnBi$_2$Te$_4$ as the charge-transfer compound. Understanding the growth mode of MnBi$_2$Te$_4$ can help us to grow the other members of MB$_2$T$_4$-family materials.
Quantum anomalous Hall effect (QAHE) has been experimentally realized in magnetically-doped topological insulators or intrinsic magnetic topological insulator MnBi$_2$Te$_4$ by applying an external magnetic field. However, either the low observation temperature or the unexpected external magnetic field (tuning all MnBi$_2$Te$_4$ layers to be ferromagnetic) still hinders further application of QAHE. Here, we theoretically demonstrate that proper stacking of MnBi$_2$Te$_4$ and Sb$_2$Te$_3$ layers is able to produce intrinsically ferromagnetic van der Waals heterostructures to realize the high-temperature QAHE. We find that interlayer ferromagnetic transition can happen at $T_{\rm C}=42~\rm K$ when a five-quintuple-layer Sb$_2$Te$_3$ topological insulator is inserted into two septuple-layer MnBi$_2$Te$_4$ with interlayer antiferromagnetic coupling. Band structure and topological property calculations show that MnBi$_2$Te$_4$/Sb$_2$Te$_3$/MnBi$_2$Te$_4$ heterostructure exhibits a topologically nontrivial band gap around 26 meV, that hosts a QAHE with a Chern number of $\mathcal{C}=1$. In addition, our proposed materials system should be considered as an ideal platform to explore high-temperature QAHE due to the fact of natural charge-compensation, originating from the intrinsic n-type defects in MnBi$_2$Te$_4$ and p-type defects in Sb$_2$Te$_3$.
Quantum anomalous Hall effect (QAHE) has been experimentally observed in magnetically doped topological insulators. However, ultra-low temperature (usually below 300 mK), which is mainly attributed to inhomogeneous magnetic doping, becomes a daunting challenge for potential applications. Here, a \textitnonmagnetic-doping strategy is proposed to produce ferromagnetism and realize QAHE in topological insulators. We numerically demonstrated that magnetic moments can be induced by nitrogen or carbon substitution in Bi$_2$Se$_3$, Bi$_2$Te$_3$, and Sb$_2$Te$_3$, but only nitrogen-doped Sb$_2$Te$_3$ exhibits long-range ferromagnetism and preserve large bulk band gap. We further show that its corresponding thin-film can harbor QAHE at temperatures of 17-29 Kelvin, which is two orders of magnitude higher than the typical temperatures in similar systems. Our proposed \textitnonmagnetic doping scheme may shed new light in experimental realization of high-temperature QAHE in topological insulators.
We theoretically investigate the subradiance dynamics in a nonreciprocal chiral-coupled atomic chain, in which infinite-range dipole-dipole interaction emerges in the dissipation. We find that super- and subradiance are both present in the dissipation process following single photon excitation, and the decay dynamics shows burst emissions from uniform initial excitations, which reflects the influence of atomic ordering on the propagation of light-induced atom-atom correlations. By tuning the nonreciprocal couplings in the chiral-coupled atomic system, we show that the subradiance dynamics can be greatly modified. We further study the effect of atomic local disorder, and find occurrence of plateaus on the decay curve dependent on the defect locations, as well as persistent localized excitations induced by disorders. We also discuss the effect of imperfections of systems on the subradiance dynamics. Our results show rich opportunities in the chiral-coupled system toward photon storage and routing.
We demonstrate synthetic azimuthal gauge potentials for Bose-Einstein condensates from engineering atom-light couplings. The gauge potential is created by adiabatically loading the condensate into the lowest energy Raman-dressed state, achieving a coreless vortex state. The azimuthal gauge potentials act as effective rotations and are tunable by the Raman coupling and detuning. We characterize the spin textures of the dressed states, in agreements with the theory. The lowest energy dressed state is stable with a 4.5-s half-atom-number-fraction lifetime. In addition, we exploit the azimuthal gauge potential to demonstrate the Hess-Fairbank effect, the analogue of Meissner effect in superconductors. The atoms in the absolute ground state has a zero quasi-angular momentum and transits into a polar-core vortex when the synthetic magnetic flux is tuned to exceed a critical value. Our demonstration serves as a paradigm to create topological excitations by tailoring atom-light interactions where both types of SO(3) vortices in the $|\langle \vec{F}\rangle|=1$ manifold, coreless vortices and polar-core vortices, are created in our experiment. The gauge field in the stationary Hamiltonian opens a path to investigating rotation properties of atomic superfluids under thermal equilibrium.
We present a model to show that heat propagation away from a local source depends strongly on dimensionality, leading to dramatic localization in low-dimensional systems. An example of such a system is a carbon nanotube array. We further show that this localization is amplified due to a runaway mechanism if thermal conductivity declines rapidly with temperature. Extremely high temperatures of thousands of Kelvins and gradients of hundreds of K/\mum may thus be obtained in a conductor using a modest local power source such as a laser pointer. This is of fundamental importance for high-efficiency energy conversion through thermoelectric and thermionic mechanisms, as well as various other applications.
We theoretically investigate the light scattering of the super- and subradiant states which can be prepared by the excitation of a single photon which carries an orbital angular momentum (OAM).\ With this helical phase imprinted on the stacked ring of atomic arrays, the subradiant modes show directional side scattering in the far-field, allowing for light collimation and quantum storage of light with OAM.\ For the excitations with linear polarizations, we find a discrete $C_4$ rotational symmetry in scattering for the number of atoms $N$ $=$ $4n $ with integers $n$, while for circular polarizations with arbitrary $N$, the azimuthal and $C_N$ symmetries emerge for the super- and subradiant modes respectively.\ When the radial and azimuthal polarizations are considered, a mode shift can happen in the scattering pattern.\ The forward scattering of the superradiant modes can be enhanced as we stack up the rings along the excitation direction, and for the subradiant modes, we find the narrowing effects on the scattering in the azimuthal and the polar angles when more concentric rings are added in the radial direction.\ By designing the atomic spatial distributions and excitation polarizations, helical-phase-imprinted subradiant states can tailor and modify the radiation properties, which is detectable in the directional super- and subradiant emissions and is potentially useful in quantum information manipulations.
We show that Weyl points with topological charges 1 and 2 can be found in very simple chiral woodpile photonic crystals, which can be fabricated using current techniques down to the nano-scale. The sign of the topological charges can be tuned by changing the material parameters of the crystal, keeping the structure and the symmetry unchanged. The underlying physics can be understood using a tight binding model, which shows that the sign of the charge depends on the hopping range. Gapless surface states and their back-scattering immune properties are also demonstrated in these systems.
It has been a general trend to develop low-voltage electron microscopes due to their high imaging contrast of the sample and low radiation damage. Atom-resolved transmission electron microscopes with voltages as low as 15-40 kV have been demonstrated. However, achieving atomic resolution at voltages lower than 10 kV is extremely difficult. An alternative approach is coherent imaging or phase retrieval imaging, which requires a sufficiently coherent source and an adequately small detection area on the sample as well as the detection of high-angle diffracted patterns with a sufficient resolution. In this work, we propose several transmission-type schemes to achieve coherent imaging of thin materials (less than 5 nm thick) with atomic resolution at voltages lower than 10 kV. Experimental schemes of both lens-less and lens-containing designs are presented and the advantages and challenges of these schemes are discussed. Preliminary results based on a highly coherent single-atom electron source are presented. The image plate is designed to be retractable to record the transmission patterns at different positions along the beam propagation direction. In addition, reflection-type coherent electron imaging schemes are also proposed as novel methods for characterizing surface atomic and electronic structures of materials.
The nodal points in a Weyl semimetal are generally considered as the causes of the chiral anomaly and the chiral magnetic effect (CME). Employing a linear-response analysis of a two-band lattice model, we show that the Weyl nodes and thus the chirality are not required for the CME, while they remain crucial for the chiral anomaly. Similar to the anomalous Hall effect, the CME results directly from the Berry curvature of energy bands, even when there is no monopole source from the Weyl nodes. Therefore, the phenomenon of the CME could be observed in a wider class of materials. Motivated by this result, we suggest that the nodeless CME may appear in three-dimensional quantum anomalous Hall insulators, but after they become metallic due to the band deformation caused by inversion symmetry breaking.
Employing a two-band model of Weyl semimetal, the existence of the chiral magnetic effect (CME) is established within the linear-response theory. The crucial role played by the limiting procedure in deriving correct transport properties is clarified. Besides, in contrast to the prediction based on linearized effective models, the value of the CME coefficient in the uniform limit shows nontrivial dependence on various model parameters. Even when these parameters are away from the region of the linearized models, such that the concept of chirality may not be appropriate, this effect still exists. This implies that the Berry curvature, rather than the chiral anomaly, provides a better understanding of this effect.
We show that the five possible ordered states in a quantum spin-1/2 system with long-range exchange interactions: Neel, ladder, Peierls, coincidence, and domain states, can be realized in a binary Rydberg-dressed BEC system in the supersolid phase. In such a system, blockade phenomenon is shown to also occur for pairs of different excited-state atoms, which results in similar intra- and inter-species long-range interactions between ground-state atoms. It suggests that a pseudo spin-1/2 system can be possibly formed in the ground state of ultracold rudibium.
We present our proposals for generating total hyperfine spin zero state for two f=1 or two f=2 particles, starting from initial unentangled states. We show that our goal can be achieved by exploiting spin changing dynamics and quadratic Zeeman shifts with realistic choices of external magnetic fields and evolution time intervals.
Keng-Ku Liu, Wenjing Zhang, Yi-Hsien Lee, Yu-Chuan Lin, Mu-Tung Chang, Ching-Yuan Su, Chia-Seng Chang, Hai Li, Yumeng Shi, Hua Zhang, Chao-Sung Lai, Lain-Jong Li The two-dimensional layer of molybdenum disulfide (MoS2) has recently attracted much interest due to its direct-gap property and potential applications in optoelectronics and energy harvesting. However, the synthetic approach to obtain high quality and large-area MoS2 atomic thin layers is still rare. Here we report that the high temperature annealing of a thermally decomposed ammonium thiomolybdate layer in the presence of sulfur can produce large-area MoS2 thin layers with superior electrical performance on insulating substrates. Spectroscopic and microscopic results reveal that the synthesized MoS2 sheets are highly crystalline. The electron mobility of the bottom-gate transistor devices made of the synthesized MoS2 layer is comparable with those of the micromechanically exfoliated thin sheets from MoS2 crystals. This synthetic approach is simple, scalable and applicable to other transition metal dichalcogenides. Meanwhile, the obtained MoS2 films are transferable to arbitrary substrates, providing great opportunities to make layered composites by stacking various atomically thin layers.
Yi-Hsien Lee, Xin-Quan Zhang, Wenjing Zhang, Mu-Tung Chang, Cheng-Te Lin, Kai-Di Chang, Ya-Chu Yu, Jacob Tse-Wei Wang, Chia-Seng Chang, Lain-Jong Li, Tsung-Wu Lin Large-area MoS2 atomic layers are synthesized on SiO2 substrates by chemical vapor deposition using MoO3 and S powders as the reactants. Optical, microscopic and electrical measurements suggest that the synthetic process leads to the growth of MoS2 monolayer. The TEM images verify that the synthesized MoS2 sheets are highly crystalline.
A graphene nano-ribbon with armchair edges is known to have no edge state. However, if the nano-ribbon is in the quantum spin Hall (QSH) state, then there must be helical edge states. By folding a graphene ribbon to a ring and threading it by a magnetic flux, we study the persistent charge and spin currents in the tight-binding limit. It is found that, for a broad ribbon, the edge spin current approaches a finite value independent of the radius of the ring. For a narrow ribbon, inter-edge coupling between the edge states could open the Dirac gap and reduce the overall persistent currents. Furthermore, by enhancing the Rashba coupling, we find that the persistent spin current gradually reduces to zero at a critical value, beyond which the graphene is no longer a QSH insulator.
The density of states near zero energy in a graphene due to strong point defects with random positions are computed. Instead of focusing on density of states directly, we analyze eigenfunctions of inverse T-matrix in the unitary limit. Based on numerical simulations, we find that the squared magnitudes of eigenfunctions for the inverse T-matrix show random-walk behavior on defect positions. As a result, squared magnitudes of eigenfunctions have equal \it a priori probabilities, which further implies that the density of states is characterized by the well-known Thomas-Porter type distribution. The numerical findings of Thomas-Porter type distribution is further derived in the saddle-point limit of the corresponding replica field theory of inverse T-matrix. Furthermore, the influences of the Thomas-Porter distribution on magnetic and transport properties of a graphene, due to its divergence near zero energy, are also examined.
A semiclassical theory of spin dynamics and transport is formulated using the Dirac electron model. This is done by constructing a wavepacket from the positive-energy electron band, and studying its structure and center of mass motion. The wavepacket has a minimal size equal to the Compton wavelength, and has self-rotation about the average spin angular momentum, which gives rise to the spin magnetic moment. Geometric gauge structure in the center of mass motion provides a natural explanation of the spin-orbit coupling and various Yafet terms. Applications of the spin-Hall and spin-Nernst effects are discussed.
Ever since its discovery, the Berry phase has permeated through all branches of physics. Over the last three decades, it was gradually realized that the Berry phase of the electronic wave function can have a profound effect on material properties and is responsible for a spectrum of phenomena, such as ferroelectricity, orbital magnetism, various (quantum/anomalous/spin) Hall effects, and quantum charge pumping. This progress is summarized in a pedagogical manner in this review. We start with a brief summary of necessary background, followed by a detailed discussion of the Berry phase effect in a variety of solid state applications. A common thread of the review is the semiclassical formulation of electron dynamics, which is a versatile tool in the study of electron dynamics in the presence of electromagnetic fields and more general perturbations. Finally, we demonstrate a re-quantization method that converts a semiclassical theory to an effective quantum theory. It is clear that the Berry phase should be added as a basic ingredient to our understanding of basic material properties.
We study the magnetization for the classical antiferromagnetic Ising model on the Shastry-Sutherland lattice using the tensor renormalization group approach. With this method, one can probe large spin systems with little finite-size effect. For a range of temperature and coupling constant, a single magnetization plateau at one third of the saturation value is found. We investigate the dependence of the plateau width on temperature and on the strength of magnetic frustration. Furthermore, the spin configuration of the plateau state at zero temperature is determined.
Density Matrix Renormalization Group (DMRG) calculations on 4-leg t-J and Hubbard ladders have found a phase exhibiting "stripes" at intermediate doping. Such behavior can be viewed as generalized Friedel oscillations, with wavelength equal to the inverse hole density, induced by the open boundary conditions. So far, this phase has not been understood using the conventional weak coupling bosonization approach. Based on studies from a general bosonization proof, finite size spectrum, an improved analysis of weak coupling renormalization group equations and the decoupled 2-leg ladders limit, we here find new types of phases of 4-leg ladders which exhibit "stripes". They also inevitably exhibit "bipairing", meaning that there is a gap to add 1 or 2 electrons (but not 4) and that both single electron and electron pair correlation functions decay exponentially while correlation functions of charge 4 operators exhibit power-law decay. Whether or not bipairing occurs in the stripe phase found in DMRG is an important open question.
Entanglement in J_1-J_2, S=1/2 quantum spin chains with an impurity is studied using analytic methods as well as large scale numerical density matrix renormalization group methods. The entanglement is investigated in terms of the von Neumann entropy, S=-Tr rho_A log rho_A, for a sub-system A of size r of the chain. The impurity contribution to the uniform part of the entanglement entropy, S_imp, is defined and analyzed in detail in both the gapless, J_2 <= J_2^c, as well as the dimerized phase, J_2>J_2^c, of the model. This quantum impurity model is in the universality class of the single channel Kondo model and it is shown that in a quite universal way the presence of the impurity in the gapless phase, J_2 <= J_2^c, gives rise to a large length scale, xi_K, associated with the screening of the impurity, the size of the Kondo screening cloud. The universality of Kondo physics then implies scaling of the form S_imp(r/xi_K,r/R) for a system of size R. Numerical results are presented clearly demonstrating this scaling. At the critical point, J_2^c, an analytic Fermi liquid picture is developed and analytic results are obtained both at T=0 and T>0. In the dimerized phase an appealing picure of the entanglement is developed in terms of a thin soliton (TS) ansatz and the notions of impurity valence bonds (IVB) and single particle entanglement (SPE) are introduced. The TS-ansatz permits a variational calculation of the complete entanglement in the dimerized phase that appears to be exact in the thermodynamic limit at the Majumdar-Ghosh point, J_2=J_1/2, and surprisingly precise even close to the critical point J_2^c. In appendices the relation between the finite temperature entanglement entropy, S(T), and the thermal entropy, S_th(T), is discussed and <S^z_r> and <S_r S_r+1> calculated at the MG-point using the TS-ansatz.
Electrons with spin-orbit coupling moving in mesoscopic structures can often exhibit local spin polarization. In this paper, we study the influence of the Rashba coupling on the scattering of two-dimensional electrons from a circular disk. It is observed that spin-polarized regions exist, even if the incident electrons are unpolarized. In addition to the distributions of charge and spin current in the near-field region, we also analyze the symmetry and the differential cross-section of the scattering.
The non-equilibrium transportation of two-dimensional electrons through a narrow channel is investigated under the influence of the Rashba interaction. By introducing suitable lifetime in the Green's function, the average spin values can be calculated from the ballistic regime to the diffusive regime. It is shown that the spin accumulation is a combined effect of the spin current and disorders. In the diffusive regime, disorders offer a mechanism to stop the spin current and generate the spin accumulation. In the ballistic regime, spins are more spread out and do not have definite signs. Further consideration indicates that the inclusion of ferromagnetic spin-spin interaction increases the spin accumulation near the edge.
The screening of an impurity spin by conduction electrons is associated with the formation of a large Kondo screening cloud, of size xi_K. We study the quantum entanglement between a region of size r surrounding the impurity and the rest of the sample, (of total size R) using Density Matrix Renormalization Group and analytic methods. The corresponding "impurity entanglement entropy", S_imp, is shown to be a universal scaling function of r/xi_K and r/R. We calculate this universal function using Fermi liquid theory in the regime xi_K << r.
We present exact diagonalization and density matrix renormalization group results for the entanglement entropy of critical spin-1/2 XXZ chains. We find that open boundary conditions induce an alternating term in both the energy density and the entanglement entropy which are approximately proportional, decaying away from the boundary with a power-law. The power varies with anisotropy along the XXZ critical line and is corrected by a logarithmic factor, which we calculate analytically, at the isotropic point. A heuristic resonating valence bond explanation is suggested.
We interpret the recently observed spatial domain formation in spin-1 atomic condensates as a result of dynamical instability. Within the mean field theory, a homogeneous condensate is dynamically unstable (stable) for ferromagnetic (antiferromagnetic) atomic interactions. We find this dynamical instability naturally leads to spontaneous domain formation as observed in several recent experiments for condensates with rather small numbers of atoms. For trapped condensates, our numerical simulations compare quantitatively to the experimental results, thus largely confirming the physical insight from our analysis of the homogeneous case.
A generalized Streda formula is derived for the spin transport in spin-orbit coupled systems. As compared with the original Streda formula for charge transport, there is an extra contribution of the spin Hall conductance whenever the spin is not conserved. For recently studied systems with quantum spin Hall effect in which the z-component spin is conserved, this extra contribution vanishes and the quantized value of spin Hall conductivity can be reproduced in the present approach. However, as spin is not conserved in general, this extra contribution can not be neglected, and the quantization is not exact.
Collisions in a thermal gas are perceived as random or incoherent as a consequence of the large numbers of initial and final quantum states accessible to the system. In a quantum gas, e.g. a Bose-Einstein condensate or a degenerate Fermi gas, the phase space accessible to low energy collisions is so restricted that collisions be-come coherent and reversible. Here, we report the observation of coherent spin-changing collisions in a gas of spin-1 bosons. Starting with condensates occupying two spin states, a condensate in the third spin state is coherently and reversibly created by atomic collisions. The observed dynamics are analogous to Josephson oscillations in weakly connected superconductors and represent a type of matter-wave four-wave mixing. The spin-dependent scattering length is determined from these oscillations to be -1.45(18) Bohr. Finally, we demonstrate coherent control of the evolution of the system by applying differential phase shifts to the spin states using magnetic fields.
We studied the correlated quasi-one-dimensional systems by one-loop renormalization group techniques in weak coupling. In contrast to conventional g-ology approach, we formulate the theory in terms of bilinear currents and obtain all possible interaction vertices. Furthermore, the one-loop renormalization group equations are derived by operator product expansions of these currents at short length scale. It is rather remarkable that these coupled non-linear equations, after appropriate rescaling, can be casted into potential flows. The existence of what we nicknamed "RG potential" provides a natural explanation of the emergent symmetry enhancement in ladder systems. Further implications arisen from the RG potential are also discussed at the end.
Using a semiclassical approach, we study the persistent magnetization current of a mesoscopic ferrimagnetic ring in a nonuniform magnetic field. At zero temperature, there exists persistent spin current because of the quantum fluctuation of magnons, similar to the case of an antiferromagnetic spin ring. At low temperature, the current shows activation behavior because of the field-induced gap. At higher temperature, the magnitude of the spin current is proportional to temperature T, similar to the reported result of a ferromagnetic spin ring.
We study the coherent off-equilibrium spin mixing inside an atomic condensate. Using mean field theory and adopting the single spatial mode approximation (SMA), the condensate spin dynamics is found to be well described by that of a nonrigid pendulum, and displays a variety of periodic oscillations in an external magnetic field. Our results illuminate several recent experimental observations and provide critical insights into the observation of coherent interaction-driven oscillations in a spin-1 condensate.
In a two-dimensional electron gas with Rashba and Dresselhaus spin-orbit couplings, there are two spin-split energy surfaces connected with a degenerate point. Both the energy surfaces and the topology of the Fermi surfaces can be varied by an in-plane magnetic field. We find that, if the chemical potential falls between the bottom of the upper band and the degenerate point, then simply by changing the direction of the magnetic field, the magnitude of the spin Hall conductivity can be varied by about 100 percent. Once the chemical potential is above the degenerate point, the spin Hall conductivity becomes the constant $e/8\pi$, independent of the magnitude and direction of the magnetic field. In addition, we find that the in-plane magnetic field exerts no influence on the charge Hall conductivity.
We measure spin mixing of F=1 and F=2 spinor condensates of 87Rb atoms confined in an optical trap. We determine the spin mixing time to be typically less than 600 ms and observe spin population oscillations. The equilibrium spin configuration in the F=1 manifold is measured for different magnetic fields and found to show ferromagnetic behavior for low field gradients. An F=2 condensate is created by microwave excitation from F=1 manifold, and this spin-2 condensate is observed to decay exponentially with time constant 250 ms. Despite the short lifetime in the F=2 manifold, spin mixing of the condensate is observed within 50 ms.
Two-dimensional Bloch electrons in a uniform magnetic field exhibit complex energy spectrum. When static electric and magnetic modulations with a checkerboard pattern are superimposed on the uniform magnetic field, more structures and symmetries of the spectra are found, due to the additional adjustable parameters from the modulations. We give a comprehensive report on these new symmetries. We have also found an electric-modulation induced energy gap, whose magnitude is independent of the strength of either the uniform or the modulated magnetic field. This study is applicable to experimentally accessible systems and is related to the investigations on frustrated antiferromagnetism.
We address the issue why the phase diagrams for quasi-one-dimensional systems are rather simple, while the renormalization group equations behind the scene are non-linear and messy looking. The puzzle is answered in two steps -- we first demonstrate that the complicated coupled flow equations are simply described by a potential $V(h_i)$, in an appropriate basis for the interaction couplings $h_i$. The renormalization-group potential is explicitly constructed by introducing the Majorana fermion representation. The existence of the potential prevents chaotic behaviors and other exotic possibilities such as limit cycles. Once the potential is obtained, the ultimate fate of the flows are described by a special set of fixed-ray solutions and the phase diagram is determined by Abelian bosonization. Extension to strong coupling regime and comparison with the Zamolodchikov c-theorem are discussed at the end.
The magnetization curve of the two-dimensional spin-1/2 $J_1$-$J_2$ Heisenberg model is investigated by using the Chern-Simons theory under a uniform mean-field approximation. We find that the magnetization curve is monotonically increasing for $J_2/J_1 < 0.267949$, where the system under zero external field is in the antiferromagnetic Néel phase. For larger ratios of $J_2/J_1$, various plateaus will appear in the magnetization curve. In particular, in the disordered phase, our result supports the existence of the $M/M_{\rm sat}=1/2$ plateau and predicts a new plateau at $M/M_{\rm sat}=1/3$. By identifying the onset ratio $J_2/J_1$ for the appearance of the 1/2-plateau with the boundary between the Néel and the spin-disordered phases in zero field, we can determine this phase boundary accurately by this mean-field calculation. Verification of these interesting results would indicate a strong connection between the frustrated antiferromagnetic system and the quantum Hall system.
The effect of a one-dimensional periodic electrostatic modulation on quantum Hall systems with filling factor \nu=1 is studied. We propose that, either when the amplitude of the modulation potential or the tilt angle of the magnetic field is varied, the system can undergo a first-order phase transition from a fully spin-polarized homogeneous state to a partially spin-polarized charge-density-wave state, and show hysteresis behavior of the spin polarization. This is confirmed by our self-consistent numerical calculations within the Hartree-Fock approximation. Finally we suggest that the \nu=1/3 fractional quantum Hall state may also show similar hysteresis behavior in the presence of a periodic potential modulation.
In this comment, we emphasize that the self-consistent spin wave theory in a recent paper [J. K"onig, H.-H. Lin, and A. H. MacDonald, Phys. Rev. Lett. 84, 5628 (2000)] leads to incorrect results both at low temperatures and near T_c. Thus we suggest another self-consistent spin wave approximation to remedy these flaws.
In this paper, the influence of an in-plane magnetic field B_∥on the finite-temperature phase transitions in nu=2 bilayer quantum Hall systems are examined. It is found that there can exist two types of finite-temperature phase transitions. The first is the Kosterlitz-Thouless (KT) transitions, which can have an unusual non-monotonic dependence on B_∥; the second type originates from the crossing of energy levels and always increases with B_∥. Based on these results, we point out that the threshold temperature observed in the inelastic light scattering experiments cannot be the KT transition temperature, because the latter shows a totally different B_∥-dependence as compared with the experimental observation. Instead, it should be the level-crossing temperature, which we found agrees with the B_∥-dependence observed. Moreover, combining the knowledge of these two transition temperatures, a complete finite-temperature phase diagram is presented.
By using the effective bosonic spin theory, which is recently proposed by Demler and Das Sarma [ Phys. Rev. Lett. 82, 3895 (1999) ], we analyze the effect of an external in-plane magnetic field on the magnetic phase transitions of the bilayer quantum Hall system at filling factor nu=2. It is found that the quantum phase diagram is modified by the in-plane magnetic field. Therefore, quantum phase transitions can be induced simply by tilting the magnetic field. The general behavior of the critical tilted angle for different layer separations and interlayer tunneling amplitudes is shown. We find that the critical tilted angles being calculated agree very well with the reported values. Moreover, a universal critical exponent for the transition from the canted antiferromagnetic phase to the ferromagnetic phase is found to be equal to 1/2 within the present effective theory.
The energy spectra of spin-1/2 electrons under two-dimensional magnetic field modulations are calculated beyond the one-band approximation. Our formulation is generally applicable to a modulation field with a rectangular lattice symmetry. The field distribution within a plaquette is otherwise arbitrary. The spectra being obtained are qualitatively different from their electric modulated counterparts. Peculiar features of the spectra are that, for an electron with a g factor precisely being equal to two, no matter how strong the modulation is, the zero-energy level seems to be unaffected by the modulation and is separated from higher energy levels with a nonzero energy gap. Moreover, there is a two-fold degenerancy for all states with positive energies with respect to spin flip. These features agree with earlier analytical studies of the periodically magnetic modulated systems.
Jul 04 1997
cond-mat arXiv:cond-mat/9707031v1
When the energy of a pump wave is in resonance with the exciton creation energy, the electric susceptibility of a conjugated polymer in response to the probe wave is altered by the exciton gas. In this paper, we calculate the dependence of this change on the the exciton populations by the equation of motion (EOM) method. The magnitude of optical nonlinearity is also influenced by ambient temperature, by the extent of exciton wave functions, and by the strength of electron-electron interaction. All of these factors can be easily incorporated in the EOM approach systematically. Using the material parameters for polydiacetylene (PDA), the optical Kerr coefficient $n_2$ obtained is about $10^{-8} cm^2/W$, which is close to experimental value, and is four orders of magnitude larger than the value in nonresonant pump experiments.
An effective Hamiltonian approach is used to study the effect of Landau-level mixing on the energy spectrum of electrons in a smooth but random magnetic field B(r) with a finite uniform component B_0. It is found that, as opposed to electrostatic disorder, the energy levels of localized electrons shift upward with a rate of order O(1/B_0) when B_0 is decreased, while the extended states remain static at the same order. Therefore, there is no indication that the extended states will float out of the Fermi energy and induce a metal-insulator transition as the magnetic disorder is increased. We also find that the Zeeman term may have significant effect on the spectral shift of low-lying Landau levels.
Nov 04 1995
cond-mat arXiv:cond-mat/9511014v1
We have derived a new set of semiclassical equations for electrons in magnetic Bloch bands. The velocity and energy of magnetic Bloch electrons are found to be modified by the Berry phase and magnetization. This semiclassical approach is used to study general electron transport in a DC or AC electric field. We also find a close connection between the cyclotron orbits in magnetic Bloch bands and the energy subbands in the Hofstadter spectrum. Based on this formalism, the pattern of band splitting, the distribution of Hall conduct- ivities, and the positions of energy subbands in the Hofstadter spectrum can be understood in a simple and unified picture.
May 06 1995
cond-mat arXiv:cond-mat/9505021v1
We develop a semiclassical theory for the dynamics of electrons in a magnetic Bloch band, where the Berry phase plays an important role. This theory, together with the Boltzmann equation, provides a framework for studying transport problems in high magnetic fields. We also derive an Onsager-like formula for the quantization of cyclotron orbits, and we find a connection between the number of orbits and Hall conductivity. This connection is employed to explain the clustering structure of the Hofstadter spectrum. The advantage of this theory is its generality and conceptual simplicity.
Jul 21 1994
cond-mat arXiv:cond-mat/9407083v1
In this paper we study the energy spectrum of a two dimensional electron gas (2DEG) in a two dimensional periodic magnetic field. Both a square magnetic lattice and a triangular one are considered. We consider the general case where the magnetic field in a cell can be of any shape. A general feature of the band structure is bandwidth oscillation as a function of the Landau index. A triangular magnetic lattice on a 2DEG can be realized by the vortex lattice of a superconductor film coated on top of a heterojunction. Our calculation indicates a way of relating the energy spectrum of the 2DEG to the vortex structure. We have also derived conditions under which the effects of a weak magnetic modulation, periodic or not, may be reproduced by an electric potential modulation, and vice versa.
May 16 1994
cond-mat arXiv:cond-mat/9405036v2
We explore the possibility of using a double-tip STM to probe the single electron Green function of a sample surface, and describe a few important applications: (1) Probing constant energy surfaces in $\k$-space by ballistic transport; (2) Measuring scattering phase shifts of defects; (3) Observing the transition from ballistic to diffusive transport to localization; and (4) Measuring inelastic mean free paths.
Jul 22 1993
cond-mat arXiv:cond-mat/9307049v1
The local density of states \rho(x,E) is calculated for a Bloch electron in an electric field. Depending on the system size, we can see one or more sequences of Wannier-Stark ladders in \rho(x,E), with Lorentz type level widths and apparent spatial localization of the states. Our model is a chain of delta function potential barriers plus a step-like electric potential, with open boundary condition at both ends of the system. Using a wave tunneling picture, we find that the level widths shrink to zero as an inverse power as the system size approaches infinity, confirming an earlier result.