Laboratory for Multiscale materials eXperiments (LMX)

Quantum critical points (QCPs), zero-temperature phase transitions, are win- dows to fundamental quantum-mechanical phenomena associated with universal behaviour. Magnetic QCPs have been extensively investigated in the vicinity of antiferromagnetic order. However, QCPs are rare in metallic ferromagnets due to the coupling of the order parameter to electronic soft modes. Recently, antisymmetric spin-orbit coupling in noncentrosymmetric systems was suggested to protect ferromagnetic QCPs. Nonetheless, multiple centrosymmetric materials ...

Frustrated magnets with ordered magnetic spiral phases that spontaneously break inversion symmetry have received significant attention from both fundamental and applied sciences communities due to the experimental demonstration that some of these materials can couple to the lattice and induce electric polarization. In these materials, the common origin of the electric and magnetic orders guarantees substantial coupling between them, which is highly desirable for applications ...

The recent discovery of superconductivity in infinite layer thin films and bulk Ruddlesden–Popper nickelates has stimulated the investigation of other predicted properties of these materials. Among them, the existence of magnetism-driven ferroelectricity in the parent compounds RNiO₃ (R = 4f lanthanide and Y) at the onset of the Néel order, T_N, has remained particularly elusive. Using diffraction techniques, we reveal here the existence of magnetostriction at T_N in bulk YNiO₃ single crystals. Interestingly, the associated lattice anomalies ...