Electrical current pulses can be used to manipulate magnetization efficiently via spin-orbit torques (SOTs). Pulse durations as short as a few picoseconds have been used to switch the magnetization of ferromagnetic films, reaching the THz regime. However, little is known about the reversal mechanisms and energy requirements in the ultrafast switching regime. In this work, we quantify the energy cost for magnetization reversal over 7 orders of magnitude in pulse duration, in both ferromagnetic and ferrimagnetic samples, bridging quasi-static spintronics and femtomagnetism. To this end, we develop a method to stretch picosecond pulses generated by a photoconductive switch by an order of magnitude. Thereby, we can create current pulses from picoseconds to durations approaching pulse width available with commercial instruments. We show that the energy cost for SOT switching decreases by more than an order of magnitude in all samples when the pulse duration enters the picosecond range. We project an energy cost of 9 fJ for a 100 x 100 nm 2 ferrimagnetic device. Micromagnetic and macrospin simulations unveil a transition from a non-coherent to a coherent magnetization reversal with a strong modification of the magnetization dynamical trajectories as pulse duration is reduced. Our results cement the potential for high-speed magnetic spin-orbit torque memories and highlights alternative magnetization reversal pathways at fast time scales.
C. Xiang, E. R. Cardozo de Oliveira, S. Sandeep, K. Papatryfonos, M. Morassi, L. Le Gratiet, A. Harouri, I. Sagnes, A. Lemaitre, O. Ortiz, M. Esmann, N. D. Lanzillotti-Kimura The generation of propagating acoustic waves is essential for telecommunication applications, quantum technologies, and sensing. Up to now, the electrical generation has been at the core of most implementations, but is technologically limited to a few gigahertz. Overcoming this frequency limit holds the prospect of faster modulators, quantum acoustics at higher working temperatures, nanoacoustic sensing from smaller volumes. Alternatively, the optical excitation of acoustic resonators has unlocked frequencies up to 1 THz, but in most cases, the acoustic energy cannot be efficiently extracted from the resonator into a propagating wave. Here, we demonstrate a quasi-continuous and coherent source of 20 GHz acoustic phonons, based on a ridge waveguide, structured in the vertical direction as a high-Q acousto-optic resonator. The high frequency phonons propagate up to 20 $\mu$m away from the source, with a decay rate of $\sim$1.14 dB/$\mu$m. We demonstrate the coherence between acoustic phonons generated from two distant sources through spatio-temporal interference. This concept could be scaled up to a larger number of sources, which enable a new generation of optically programmed, reconfigurable nanoacoustic devices and applications.
Harnessing high-dimensional entangled states of light presents a frontier for advancing quantum information technologies, from fundamental tests of quantum mechanics to enhanced computation and communication protocols. In this context, the spatial degree of freedom stands out as particularly suited for on-chip integration. But while traditional demonstrations produce and manipulate path-entangled states sequentially with discrete optical elements, continuously-coupled nonlinear waveguide systems offer a promising alternative where photons can be generated and interfere along the entire propagation length, unveiling novel capabilities within a reduced footprint. Here we exploit this concept to implement a compact and reconfigurable source of spatially entangled photon pairs based on parametric down-conversion in AlGaAs nonlinear waveguides arrays. We use a double-pump configuration to engineer the output quantum state and implement various types of spatial correlations, exploiting a quantum interference effect between the biphoton state generated in each pumped waveguide. This demonstration, at room temperature and telecom wavelength, illustrates the potential of continuously-coupled systems as a promising alternative to discrete multi-component quantum circuits for leveraging the high-dimensional spatial degree of freedom of photons.
We explore the contributions of adiabatic and non-adiabatic spin-transfer torques (STT) of a spin-polarized current to the thermally activated creep motion of domain-walls in a thin (Ga,Mn)(As,P) film with perpendicular anisotropy. For a domain-wall transverse to current, the non-adiabatic STT is found to act as an external magnetic field. Close to the compensation between these two terms, the adiabatic contribution is strongly enhanced. The domain-wall velocity may be both increased or reduced by the adiabatic STT, which we associate to variations of creep pinning energy barrier with domain-wall magnetic texture. Far from compensation, the contribution of adiabatic STT is negligible. Field and current driven domain-wall motion present common universal behaviors described by the quenched Edwards Wilkinson universality class.
Thibaut Divoux, Elisabeth Agoritsas, Stefano Aime, Catherine Barentin, Jean-Louis Barrat, Roberto Benzi, Ludovic Berthier, Dapeng Bi, Giulio Biroli, Daniel Bonn, Philippe Bourrianne, Mehdi Bouzid, Emanuela Del Gado, Hélène Delanoë-Ayari, Kasra Farain, Suzanne Fielding, Matthias Fuchs, Jasper van der Gucht, Silke Henkes, Maziyar Jalaal, et al (20) Soft amorphous materials are viscoelastic solids ubiquitously found around us, from clays and cementitious pastes to emulsions and physical gels encountered in food or biomedical engineering. Under an external deformation, these materials undergo a noteworthy transition from a solid to a liquid state that reshapes the material microstructure. This yielding transition was the main theme of a workshop held from January 9 to 13, 2023 at the Lorentz Center in Leiden. The manuscript presented here offers a critical perspective on the subject, synthesizing insights from the various brainstorming sessions and informal discussions that unfolded during this week of vibrant exchange of ideas. The result of these exchanges takes the form of a series of open questions that represent outstanding experimental, numerical, and theoretical challenges to be tackled in the near future.
J. Schuhmann, L. Lazzari, M. Morassi, A. Lemaitre, I. Sagnes, G. Beaudoin, M.I. Amanti, F. Boeuf, F. Raineri, F. Baboux, S. Ducci The demand for integrated photonic chips combining the generation and manipulation of quantum states of light is steadily increasing, driven by the need for compact and scalable platforms for quantum information technologies. While photonic circuits with diverse functionalities are being developed in different single material platforms, it has become crucial to realize hybrid photonic circuits that harness the advantages of multiple materials while mitigating their respective weaknesses, resulting in enhanced capabilities. Here, we demonstrate a hybrid III-V/Silicon quantum photonic device combining the strong second-order nonlinearity and compliance with electrical pumping of the III-V semiconductor platform with the high maturity and CMOS compatibility of the silicon photonic platform. Our device embeds the spontaneous parametric down-conversion (SPDC) of photon pairs into an AlGaAs source and their subsequent routing to a silicon-on-insulator circuitry, within an evanescent coupling scheme managing both polarization states. This enables the on-chip generation of broadband telecom photons by type 0 and type 2 SPDC from the hybrid device, at room temperature and with internal pair generation rates exceeding $10^5$ $s^{-1}$ for both types, while the pump beam is strongly rejected. Two-photon interference with 92% visibility (and up to 99% upon 5 nm spectral filtering) proves the high energy-time entanglement quality characterizing the produced quantum state, thereby enabling a wide range of quantum information applications on-chip, within an hybrid architecture merging the assets of two mature and highly complementary platforms in view of out-of-the-lab deployment of quantum technologies.
Coherent acoustic phonon generation and detection assisted by optical resonances are at the core of efficient optophononic transduction processes. However, when dealing with a single optical resonance, the optimum generation and detection conditions take place at different laser wavelengths, i.e. different detunings from the cavity mode. In this work, we theoretically propose and experimentally demonstrate the use of elliptical micropillars to reach these conditions simultaneously at a single wavelength. Elliptical micropillar optophononic resonators present two optical modes with orthogonal polarizations at different wavelengths. By employing a cross-polarized scheme pump-probe experiment, we exploit the mode splitting and couple the pump beam to one mode while the probe is detuned from the other one. In this way, at a particular micropillar ellipticity, both phonon generation and detection processes are enhanced. We report an enhancement of a factor of ~3.1 when comparing the signals from elliptical and circular micropillars. Our findings constitute a step forward in tailoring the light-matter interaction for more efficient ultrahigh-frequency optophononic devices.
P.-J. Wang, A. Huynh, T.-C. Hung, J.-K. Sheu, X. Lafosse, A. Lemaitre, B. Perrin, B. Rufflé, R. Vacher, C.-K. Sun, M. Foret Many theories predict a quartic acoustic attenuation increase at sub-THz frequencies in glassy media for the excess vibrational modes known as the boson peak anomaly. Here by introducing phase-sensitive acoustic spectroscopy techniques with a THz bandwidth, we investigate the acoustic properties of vitreous silica at 15 and 300K in the crucial but unexplored sub-THz gap region below the boson peak. Our results indicate a strong negative dispersion starting at \SI500GHz and the onset of an athermal quartic-frequency-scaling acoustic attenuation term, which emerges above all other thermal losses.
Despite appealing high-symmetry properties that enable high quality factor and strong confinement, whispering gallery modes of spherical and circular resonators have been absent from the field of quantum-well exciton polaritons. Here we observe whispering gallery exciton polaritons in a Gallium Arsenide microdisk cavity filled with Indium Gallium Arsenide quantum wells, the testbed materials of polaritonics. Strong coupling is evidenced in photoluminescence and resonant spectroscopy, accessed through concomitant confocal microscopy and near-field optical techniques. Excitonic and optical resonances are tuned by varying temperature and disk radius, revealing Rabi splittings between 5 and 10 meV. A dedicated analytical quantum model for such circular polaritons is developed, which reproduces the measured values. At high power, lasing is observed and accompanied by a blueshift of the emission that points to the regime of polariton lasing.
Agostino Di Francescantonio, Attilio Zilli, Davide Rocco, Laure Coudrat, Fabrizio Conti, Paolo Biagioni, Lamberto Duò, Aristide Lemaître, Costantino De Angelis, Giuseppe Leo, Marco Finazzi, Michele Celebrano All-optical modulation yields the promise of high-speed information processing. In this frame, metasurfaces are rapidly gaining traction as ultrathin multifunctional platforms for light management. Among the featured functionalities, they enable light wavefront manipulation and, more recently, demonstrated the ability to perform light-by-light manipulation through nonlinear optical processes. Here, by employing a nonlinear periodic metasurface, we demonstrate all-optical routing of telecom photons upconverted to the visible range. This is achieved via the interference between two frequency-degenerate upconversion processes, namely third-harmonic and sum-frequency generation, stemming from the interaction of a pump pulse with its frequency-doubled replica. By tuning the relative phase and polarization between these two pump beams, and concurrently engineering the nonlinear emission of the individual elements of the metasurfaces (meta-atoms) along with its pitch, we route the upconverted signal among the diffraction orders of the metasurface with a modulation efficiency up to 90%. Thanks to the phase control and the ultrafast dynamics of the underlying nonlinear processes, free-space all-optical routing could be potentially performed at rates close to the employed optical frequencies divided by the quality factor of the optical resonances at play. Our approach adds a further twist to optical interferometry, which is a key-enabling technique in a wide range of applications, such as homodyne detection, radar interferometry, LiDAR technology, gravitational waves detection, and molecular photometry. In particular, the nonlinear character of light upconversion combined with phase sensitivity is extremely appealing for enhanced imaging and biosensing.
In this work, optical profilometry and finite-element simulations are applied on buckled micro-machined membranes for the stress analysis of ion-beam-sputtered $\mathrm{Ta_{2}O_{5}}$ and $\mathrm{SiO_{2}}$ thin films. Layers with different thicknesses are grown on silicon substrates, then several membranes with different geometries are manufactured with standard micro-system technologies; due to a high level of the films' compressive stress, buckled membranes are obtained. Thermally-grown silica membranes are also produced, for comparison. The residual stress values are determined by comparing the measured and simulated deflections of the membranes. The average stress state of the $\mathrm{Ta_{2}O_{5}}$ thin films is found to be $-209$ MPa. The $\mathrm{SiO_{2}}$ thin films are in a higher compressive stress state whose average value is $-576$ MPa. The average stress in thermal $\mathrm{SiO_{2}}$ thin layers grown at 1130 $^{\circ}$C is found equal to $-321$ MPa, in good agreement with the literature.
The elementary excitations in weakly interacting quantum fluids have a non-trivial nature which is at the basis of defining quantum phenomena such as superfluidity. These excitations and the physics they lead to have been explored in closed quantum systems at thermal equilibrium both theoretically within the celebrated Bogoliubov framework, and experimentally in quantum fluids of ultracold atoms. Over the past decade, the relevance of Bogoliubov excitations has become essential to understand quantum fluids of interacting photons. Their driven-dissipative character leads to distinct properties with respect to their equilibrium counterparts. For instance, the condensate coupling to the photonic vacuum environment leads to a non-zero generation rate of elementary excitations with many striking implications. In this work, considering that quantum fluids of light are often hosted in solid-state systems, we show within a joint theory-experiment analysis that the vibrations of the crystal constitute another environment that the condensate is fundamentally coupled to. This coupling leads to a unique heat transfer mechanism, resulting in a large generation rate of elementary excitations in typical experimental conditions, and to a fundamental non-zero contribution at vanishing temperatures. Our work provides a complete framework for solid-embedded quantum fluids of light, which is invaluable in view of achieving a regime dominated by photon vacuum fluctuations.
E. Rongione, L. Baringthon, D. She, G. Patriarche, R. Lebrun, A. Lemaitre, M. Morassi, N. Reyren, M. Micica, J. Mangeney, J. Tignon, F. Bertran, S. Dhillon, P. Le Fevre, H. Jaffres, J.-M. George The helicity of 3D topological insulator surface states has drawn significant attention in spintronics owing to spin-momentum locking where the carriers' spin is oriented perpendicular to their momentum. This property can provide an efficient method to convert charge currents into spin currents, and vice-versa, through the Rashba-Edelstein effect. However, experimental signatures of these surface states to the spin-charge conversion are extremely difficult to disentangle from bulk state contributions. Here, we combine spin- and angle-resolved photo-emission spectroscopy, and time-resolved THz emission spectroscopy to categorically demonstrate that spin-charge conversion arises mainly from the surface state in Bi$_{1-x}$Sb$_x$ ultrathin films, down to few nanometers where confinement effects emerge. We correlate this large conversion efficiency, typically at the level of the bulk spin Hall effect from heavy metals, to the complex Fermi surface obtained from theoretical calculations of the inverse Rashba-Edelstein response. %We demonstrate this for film thickness down to a few nanometers, Both surface state robustness and sizeable conversion efficiency in epitaxial Bi$_{1-x}$Sb$_x$ thin films bring new perspectives for ultra-low power magnetic random-access memories and broadband THz generation.
Electronic resonances can significantly enhance the photon-phonon coupling in cavity optomechanics, but are normally avoided due to absorption losses and dephasing by inhomogeneous broadening. We experimentally demonstrate that exciton-polaritons in semiconductor microcavities enable GHz optomechanics with single-particle resonant couplings reaching record values in the 10s of MHz range. Moreover, this resonant enhancement is protected from inhomogeneous broadening by the Rabi gap. Single-polariton non-linearities and the optomechanical strong-coupling regime become accessible in this platform.
Elham Mehdi, Manuel Gundin-Martinez, Clément Millet, Niccolo Somaschi, Aristide Lemaître, Isabelle Sagnes, Luc Le Gratiet, Dario Fioretto, Nadia Belabas, Olivier Krebs, Pascale Senellart, Loïc Lanco In the framework of optical quantum computing and communications, a major objective consists in building receiving nodes that implement conditional operations on incoming photons, using the interaction with a single stationary qubit. In particular, the quest for scalable nodes motivated the development of cavity-enhanced spin-photon interfaces with solid-state emitters. An important challenge remains, however, to produce a stable, controllable, spin-dependant photon state, in a deterministic way. Here we use a pillar-based high-Q cavity, embedding a singly-charged semiconductor quantum dot, to demonstrate the control of giant polarisation rotations induced by a single electron spin. A complete tomography approach is used to deduce the output polarisation Stokes vector, conditioned by a single spin state. We experimentally demonstrate rotation amplitudes such as $\pm \frac{\pi}{2}$ and $\pi$ in the Poincaré sphere, as required for applications based on spin-polarisation mapping and spin-mediated photon-photon gates. In agreement with our modeling, we observe that the environmental noise does not limit the amplitude of the spin-induced rotation, yet slightly degrades the polarisation purity of the output states. We find that the polarisation state of the reflected photons can be manipulated in most of the Poincaré sphere, through controlled spin-induced rotations, thanks to moderate cavity birefringence and limited noise. This control allows the operation of spin-photon interfaces in various configurations, including at zero or low magnetic fields, which ensures compatibility with key protocols for photonic cluster state generation.
Electrically controllable non-volatile magnetic memories show great potential for the replacement of semiconductor-based technologies. Recently there has been strong interest in spin-orbit torque (SOT) induced magnetization reversal due to the device's increased lifetime and speed of operation. However, recent SOT switching studies reveal an incubation delay in the ~ns range due to stochasticity in the nucleation of a magnetic domain during reversal. Here, we experimentally demonstrate ultrafast SOT-induced magnetization switching dynamics of a ferromagnet with no incubation delay by avoiding the nucleation process and driving the magnetization coherently. We employ an ultrafast photo-conducting switch and a co-planar strip line to generate and guide ~ps current pulses into the heavy metal/ferromagnet layer stack and induce ultrafast SOT. We use magneto-optical probing to investigate the magnetization switching dynamics with sub-picosecond time resolution. Depending on the relative current pulse and in-plane magnetic field polarities, we observe either an ultrafast demagnetization and subsequent recovery along with a SOT-induced precessional oscillation, or ultrafast SOT switching. The magnetization zero-crossing occurs in ~70 ps, which is approximately an order of magnitude faster than previous studies. Complete switching needs ~250 ps and is limited by the heat diffusion to the substrate. We use a macro-magnetic simulation coupled with an ultrafast heating model to analyze the effect of ultrafast thermal anisotropy torque and current-induced torque in the observed dynamics. Good agreement between our experimental results and the macro-spin model shows that the switching dynamics are coherent and present no noticeable incubation delay. Our work suggests a potential pathway toward dramatically increasing the writing speed of SOT magnetic random-access memory devices.
Anne Rodriguez, Priya Priya, Edson Cardozo de Oliveira, Luc Le Gratiet, Isabelle Sagnes, Martina Morassi, Aristide Lemaître, Florian Pastier, Loïc Lanco, Martin Esmann, Norberto Daniel Lanzillotti-Kimura The selection rules governing spontaneous Brillouin scattering in crystalline solids are usually taken as intrinsic material properties, locking the relative polarization of excitation and signal in bulk. In this work, we independently manipulate these polarization states by means of optical resonances in elliptical micropillars and demonstrate a polarization-based filtering scheme for Brillouin spectroscopy in the 20-100 GHz range, important for telecom applications. This strong modification of selection rules using elliptical micropillars can be extended to any optical system with localized, polarization-sensitive modes, such as plasmonic resonators, photonic crystals, birefringent micro-, and nanostructures. Our polarization control protocol will thus find applications in the engineering of light-matter interactions in optomechanical, optoelectronic and quantum optics devices.
We demonstrate that surface morphogenesis in compressed thin films may result from spatially correlated plastic activity. A soft glassy film strongly adhering to a smooth and rigid substrate and subjected to uniaxial compression, indeed, does not undergo any global elastic pattern-forming instability, but responds plastically via localized burst events that self-organize, leading to the emergence of a series of parallel ridges transverse to the compression axis. This phenomenon has been completely overlooked, but results from common features of the plastic response of glasses, hence should be highly generic for compressed glassy thin films.
Alex Amato, Diana Lumaca, Elisabetta Cesarini, Massimo Granata, Anaël Lemaître, Matteo Lorenzini, Christophe Malhaire, Christophe Michel, Francesco Piergiovanni, Laurent Pinard, Nikita Shcheblanov, Gianpietro Cagnoli Low internal friction coatings are key components of advanced technologies such as optical atomic clocks and high-finesse optical cavity and often lie at the forefront of the most advanced experiments in Physics. Notably, increasing the sensitivity of gravitational-wave detectors depends in a very large part on developing new coatings, which entails developing more suitable methods and models to investigate their loss angle. In fact, the most sensitive region of the detection band in such detectors is limited by the coating thermal noise, which is related to the loss angle of the coating. Until now, models which describe only ideal physical properties have been adopted, wondering about the use of one or more loss angles to describe the mechanical properties of coatings. Here we show the presence of a systematic error ascribed to inhomogeneity of the sample at its edges in measuring the coating loss angle. We present a model for disk-shaped resonators, largely used in loss angle measurements, and we compare the theory with measurements showing how this systematic error impacts on the accuracy with which the loss model parameters are known.
Amorphous mixed titania-tantala coatings are key components of Bragg reflectors in the gravitational wave detectors (GWDs). Attaining the lowest possible values of optical absorption and mechanical losses in the coatings is of paramount importance for GWDs, and this requires a complex optimization of the coating deposition and post-deposition annealing. We present here a systematic investigation of the optical properties and internal friction of amorphous mixed titania-tantala coatings grown by ion beam sputtering. We consider coatings with six different cation mixing ratios and we study them both in the as-deposited and annealed state. By exploiting spectroscopic ellipsometry data and modelling, along with ancillary techniques, we retrieved the dielectric function of the coatings in a wide spectral range. When varying the mixing ratio and performing the annealing we find monotonic trends for most of the aforementioned properties. Remakably, the post-annealing Urbach energy displays a definite minimum for a mixing ratio around 20%, very close to the composition of the coatings showing the lowest optical absorption for GWDs applications. We suggest that the observed minimum in the Urbach energy depends not only on the mixing ratio, but also on the annealing parameters. On the other hand, the minimum coating loss angle was found to be weakly dependent on the considered measurement frequency and to lie within a rather broad range of Ti content, suggesting that the search for an absolute minimum following post-deposition annealing should be rather sought in the study of the best annealing parameters for each specific cation ratio considered. This work constitutes a reference for the optical properties of the amorphous mixed titania-tantala coatings, and highlights the relevance of the Urbach energy in the optimization process of materials for high-performing Bragg reflectors.
We demonstrate a chip-integrated semiconductor source that combines polarization and frequency entanglement, allowing the generation of entangled biphoton states in a hybrid degree of freedom without postmanipulation. Our AlGaAs device is based on type-II spontaneous parametric down-conversion (SPDC) in a counterpropagating phase-matching scheme, in which the modal birefringence lifts the degeneracy between the two possible nonlinear interactions. This allows the direct generation of polarization-frequency entangled photons, at room temperature and telecom wavelength, and in two distinct spatial modes, offering enhanced flexibility for quantum information protocols. The state entanglement is quantified by a combined measurement of the joint spectrum and Hong-ou-Mandel interference of the biphotons, allowing to reconstruct a restricted density matrix in the hybrid polarization-frequency space.
N. Coste, M. Gundin, D. Fioretto, S. E. Thomas, C. Millet, E. Medhi, M. Gundin, N. Somaschi, M. Morassi, M. Pont, A. Lemaitre, N. Belabas, O. Krebs, L. Lanco, P. Senellart Spins in semiconductor quantum dots are promising local quantum memories to generate polarization-encoded photonic cluster states, as proposed in the pioneering Rudolph-Lindner scheme [1]. However, harnessing the polarization degree of freedom of the optical transitions is hindered by resonant excitation schemes that are widely used to obtain high photon indistinguishability. Here we show that acoustic phonon-assisted excitation, a scheme that preserves high indistinguishability, also allows to fully exploit the polarization selective optical transitions to initialise and measure single spin states. We access the coherence of hole spin systems in a low transverse magnetic field and directly monitor the spin Larmor precession both during the radiative emission process of an excited state or in the quantum dot ground state. We report a spin state detection fidelity of $94.7 \pm 0.2 \%$ granted by the optical selection rules and a $20\pm5$~ns hole spin coherence time, demonstrating the potential of this scheme and system to generate linear cluster states with a dozen of photons
Patrick Quach, Arnaud Jollivet, Andrey Babichev, Nathalie Isac, Martina Morassi, Aristide Lemaitre, Pavel Yunin, Eric Frayssinet, Philippe de Mierry, Mathieu Jeannin, Adel Bousseksou, Raffaele Colombelli, Maria Tchernycheva, Yvon Cordier, François Julien We report on a GaN/AlGaN quantum cascade detector operating in the terahertz spectral range. The device was grown by metal organic chemical vapor deposition on a c-sapphire substrate and relies on polar GaN/AlGaN step quantum wells. The active region thickness is in micrometer range. The structural, electrical and optical investigations attest of high structural quality of the synthetized nitride material. The detector exhibits a peak photocurrent at 5.7 THz (23.6 meV) with a responsivity of 0.1 mA/W at 10 K under surface normal irradiation through a 10 um period grating. The photocurrent persists up to 20 K.
Quentin Fontaine, Davide Squizzato, Florent Baboux, Ivan Amelio, Aristide Lemaître, Marina Morassi, Isabelle Sagnes, Luc Le Gratiet, Abdelmounaim Harouri, Michiel Wouters, Iacopo Carusotto, Alberto Amo, Maxime Richard, Anna Minguzzi, Léonie Canet, Sylvain Ravets, Jacqueline Bloch Revealing universal behaviors is a hallmark of statistical physics. Phenomena such as the stochastic growth of crystalline surfaces, of interfaces in bacterial colonies, and spin transport in quantum magnets all belong to the same universality class, despite the great plurality of physical mechanisms they involve at the microscopic level. This universality stems from a common underlying effective dynamics governed by the non-linear stochastic Kardar-Parisi-Zhang (KPZ) equation. Recent theoretical works suggest that this dynamics also emerges in the phase of out-of-equilibrium systems displaying macroscopic spontaneous coherence. Here, we experimentally demonstrate that the evolution of the phase in a driven-dissipative one-dimensional polariton condensate falls in the KPZ universality class. Our demonstration relies on a direct measurement of KPZ space-time scaling laws, combined with a theoretical microscopic analysis that consistently reveals the other key signatures of this universality class, together with the possible resilience of KPZ dynamics to the presence of space-time vortices. Our results highlight fundamental physical differences between out-of-equilibrium condensates and their equilibrium counterparts, and open a new paradigm for exploring universal behaviors in open systems.
O. Jamadi, B. Real, K. Sawicki, C. Hainaut, A. Gonzalez-Tudela, N. Pernet, I. Sagnes, M. Morassi, A. Lemaitre, L. Le Gratiet, A. Harouri, S. Ravets, J. Bloch, A. Amo The engineering of localised modes in photonic structures is one of the main targets of modern photonics. An efficient strategy to design these modes is to use the interplay of constructive and destructive interference in periodic photonic lattices. This mechanism is at the origin of defect modes in photonic bandgaps, bound states in the continuum and compact localised states in flat bands. Here we show that in lattices of lossy resonators, the addition of external optical drives with controlled phase enlarges the possibilities of manipulating interference effects and allows designing novel types of localised modes. Using a honeycomb lattice of coupled micropillars resonantly driven with several laser spots at energies within its photonic bands we demonstrate the localisation of light in at-will geometries down to a single site. These localised modes can be seen as fully reconfigurable optical cavities with the potentiality of enhancing nonlinear effects and of controlling light-matter interactions with single site resolution.
Heat capacity of the nuclear spin system (NSS) in GaAs-based microstructures has been shown to be much greater than expected from dipolar coupling between nuclei, thus limiting the efficiency of NSS cooling by adiabatic demagnetization. It was suggested that quadrupole interaction induced by some small residual strain could provide this additional reservoir for the heat storage. We check and validate this hypothesis by combining nuclear spin relaxation measurements with adiabatic remagnetization and nuclear magnetic resonance experiments, using electron spin noise spectroscopy as a unique tool for detection of nuclear magnetization. Our results confirm and quantify the role of the quadrupole splitting in the heat storage within NSS and provide additional insight into fundamental, but still actively debated relation between a mechanical strain and the resulting electric field gradients in GaAs.
The excitonic fine structure plays a key role for the quantum light generated by semiconductor quantum dots, both for entangled photon pairs and single photons. Controlling the excitonic fine structure has been demonstrated using electric, magnetic, or strain fields, but not for quantum dots in optical cavities, a key requirement to obtain high source efficiency and near-unity photon indistinguishability. Here, we demonstrate the control of the fine structure splitting for quantum dots embedded in micropillar cavities. We propose a scheme based on remote electrical contacts connected to the pillar cavity through narrow ridges. Numerical simulations show that such a geometry allows for a three-dimensional control of the electrical field. We experimentally demonstrate tuning and reproducible canceling of the fine structure, a crucial step for the reproducibility of quantum light source technology.
We investigate the origin of yield stress aging in semi-dense, saline, and turbid suspensions in which structural evolution is rapidly arrested by the formation of thermally irreversible roll-resisting interparticle contacts. By performing optical tweezer (OT) three-point bending tests on particle rods, we show that these contacts yield by overcoming a rolling threshold, the critical bending moment of which grows logarithmically with time. We demonstrate that this time-dependent contact-scale rolling threshold controls the suspension yield stress and its aging kinetics. We identify a simple constitutive relation between the contact-scale flexural rigidity and rolling threshold, which transfers to macroscopic scales. This leads us to establishing a constitutive relation between macroscopic shear modulus and yield stress that is generic for an array of colloidal systems.
The low sensitivity of photons to external magnetic fields is one of the major challenges for the engineering of photonic lattices with broken time-reversal symmetry. Here we show that time-reversal symmetry can be broken for microcavity polaritons in the absence of any external magnetic field thanks to polarization dependent polariton interactions. Circularly polarized excitation of carriers in a micropillar induces a Zeeman-like energy splitting between polaritons of opposite polarizations. In combination with optical spin-orbit coupling inherent to semiconductor microstructures, the interaction induced Zeeman splitting results in emission of vortical beams with a well-defined chirality. Our experimental findings can be extended to lattices of coupled micropillars opening the possibility of controling optically the topological properties of polariton Chern insulators.
Tintu Kuriakose, Paul M. Walker, Toby Dowling, Oleksandr Kyriienko, Ivan A. Shelykh, Phillipe St-Jean, Nicola Carlon Zambon, Aristide Lemaître, Isabelle Sagnes, Luc Legratiet, Abdelmounaim Harouri, Sylvain Ravets, Maurice S. Skolnick, Alberto Amo, Jacqueline Bloch, Dmitry N. Krizhanovskii Photonic platforms are an excellent setting for quantum technologies because weak photon-environment coupling ensures long coherence times. The second key ingredient for quantum photonics is interactions between photons, which can be provided by optical nonlinearities in the form of cross-phase-modulation (XPM). This approach underpins many proposed applications in quantum optics and information processing, but achieving its potential requires strong single-photon-level nonlinear phase shifts and also scalable nonlinear elements. In this work we show that the required nonlinearity can be provided by exciton-polaritons in micropillars with embedded quantum wells. These combine the strong interactions of excitons with the scalability of micrometer-sized emitters. We observe XPM up to $3 \pm 1$ mrad per particle using laser beams attenuated to below single photon average intensity. With our work serving as a first stepping stone, we lay down a route for quantum information processing in polaritonic lattices.
Amorphous solids appear to react elastically to small external strains, but in contrast to ideal elastic media, plastic responses abound immediately, at any value of the strain. Such plastic responses are quasi-localized in nature, with the ``cheapest" one being a quadrupolar source. The existence of such plastic responses results in \em screened elasticity in which strains and stresses can either quantitatively or qualitatively differ from the un-screened theory, depending on the specific screening mechanism. Here we offer a theory of such screening effects by plastic quadrupoles, dipoles and monopoles, explain their natural appearance, and point out the analogy to electrostatic screening by electric charges and dipoles. For low density of quadrupoles the effect is to normalize the elastic moduli without a qualitative change compared to pure elasticity theory; for higher density of quadrupoles the screening effects result in qualitative changes. Predictions for the spatial dependence of displacement fields caused by local sources of strains are provided and compared to numerical simulations. We find that anomalous elasticity is richer than electrostatics in having a screening mode that does not appear in the electrostatic analog
Quantum communication networks enable applications ranging from highly secure communication to clock synchronization and distributed quantum computing. Miniaturized, flexible, and cost-efficient resources will be key elements for ensuring the scalability of such networks as they progress towards large-scale deployed infrastructures. Here, we bring these elements together by combining an on-chip, telecom-wavelength, broadband entangled photon source with industry-grade flexible-grid wavelength division multiplexing techniques, to demonstrate reconfigurable entanglement distribution between up to 8 users in a resource-optimized quantum network topology. As a benchmark application we use quantum key distribution, and show low error and high secret key generation rates across several frequency channels, over both symmetric and asymmetric metropolitan-distance optical fibered links and including finite-size effects. By adapting the bandwidth allocation to specific network constraints, we also illustrate the flexible networking capability of our configuration. Together with the potential of our semiconductor source for distributing secret keys over a 60 nm bandwidth with commercial multiplexing technology, these results offer a promising route to the deployment of scalable quantum network architectures.
N. Pernet, P. St-Jean, D. D. Solnyshkov, G. Malpuech, N. Carlon Zambon, B. Real, O. Jamadi, A. Lemaître, M. Morassi, L. Le Gratiet, T. Baptiste, A. Harouri, I. Sagnes, A. Amo, S. Ravets, J. Bloch Nonlinear topological photonics is an emerging field aiming at extending the fascinating properties of topological states to the realm where interactions between the system constituents cannot be neglected. Interactions can indeed trigger topological phase transitions, induce symmetry protection and robustness properties for the many-body system. Moreover when coupling to the environment via drive and dissipation is also considered, novel collective phenomena are expected to emerge. Here, we report the nonlinear response of a polariton lattice implementing a non-Hermitian version of the Su-Schrieffer-Heeger model. We trigger the formation of solitons in the topological gap of the band structure, and show that these solitons demonstrate robust nonlinear properties with respect to defects, because of the underlying sub-lattice symmetry. Leveraging on the system non-Hermiticity, we engineer the drive phase pattern and unveil bulk solitons that have no counterpart in conservative systems. They are localized on a single sub-lattice with a spatial profile alike a topological edge state. Our results demonstrate a tool to stabilize the nonlinear response of driven dissipative topological systems, which may constitute a powerful resource for nonlinear topological photonics.
Brillouin spectroscopy emerges as a promising non-invasive tool for nanoscale imaging and sensing. One-dimensional semiconductor superlattice structures are eminently used for selectively enhancing the generation or detection of phonons at few GHz. While commercially available Brillouin spectrometers provide high-resolution spectra, they consist of complex experimental techniques and are not suitable for semiconductor cavities operating at a wide range of optical wavelengths. We develop a pragmatic experimental approach for conventional Brillouin spectroscopy integrating a widely tunable excitation-source. Our setup combines a fibered-based angular filtering and a spectral filtering based on a single etalon and a double grating spectrometer. This configuration allows probing confined acoustic phonon modes in the 20-300 GHz frequency range with excellent laser rejection and high spectral resolution. Remarkably, our scheme based on the excitation and collection of the enhanced Brillouin scattering signals through the optical cavity, allows for better angular filtering for low phonon frequency. It can be implemented for the study of cavity optomechanics and stimulated Brillouin scattering over broadband optical and acoustic frequency ranges.
Theoretical treatments of frictional granular matter often assume that it is legitimate to invoke classical elastic theory to describe its coarse-grained mechanical properties. Here we show, based on experiments and numerical simulations, that this is generically not the case since stress auto-correlation functions decay more slowly than the elastic Green's function. It was shown theoretically that standard elastic decay demands pressure and torque density fluctuations to be normal, with possibly one of them being hyperuniform. Generic compressed frictional assemblies exhibit however abnormal pressure fluctuations, failing to conform with the central limit theorem. The physics of this failure is linked to correlations built in the material during compression from a dilute configuration prior to jamming. By changing the protocol of compression one can observe different pressure fluctuations and stress auto-correlations decay at large scales.
Laser engineered exciton-polariton networks could lead to dynamically configurable integrated optical circuitry and quantum devices. Combining cavity optomechanics with electrodynamics in laser configurable hybrid designs constitutes a platform for the vibrational control, conversion, and transport of signals. With this aim we investigate 3D optical traps laser-induced in quantum-well embedded semiconductor planar microcavities. We show that the laser generated and controlled discrete states of the traps dramatically modify the interaction between photons and phonons confined in the resonators, accessing through coupling of photoelastic origin $g_\mathrm{0}/2\pi\sim 1.7$ MHz an optomechanical cooperativity $C>1$ for mW excitation. The quenching of Stokes processes and double-resonant enhancement of anti-Stokes ones involving pairs of discrete optical states in the side-band resolved regime, allows the optomechanical cooling of 180 GHz bulk acoustic waves, starting from room temperature down to $\sim120$ K. These results pave the way for dynamical tailoring of optomechanical actuation in the extremely-high-frequency range (30-300 GHz) for future network and quantum technologies.
This paper investigates whether in frictional granular packings, like in Hamiltonian amorphous elastic solids, the stress autocorrelation matrix presents long range anisotropic contributions just as elastic Green's functions. We find that in a standard model of frictional granular packing this is not the case. We prove quite generally that mechanical balance and material isotropy constrain the stress auto-correlation matrix to be fully determined by two spatially isotropic functions: the pressure and torque auto-correlations. The pressure and torque fluctuations being respectively normal and hyperuniform force the stress autocorrelation to decay as the elastic Green's function. Since we find the torque fluctuations to be hyper-uniform, the culprit is the pressure whose fluctuations decay slower than normally as a function of the system's size. Investigating the reason for these abnormal pressure fluctuations we discover that anomalous correlations build up already during the compression of the dilute system before jamming. Once jammed these correlations remain frozen. Whether this is true for frictional matter in general or is it the consequence of the model properties is a question that must await experimental scrutiny and possible alternative models.
Interface modes have been widely explored in the field of electronics, optics, acoustics and nanophononics. One strategy to generate them is band inversion in one-dimensional superlattices. Most realizations of this type of topological states have so far been explored for a single kind of excitation. Despite its potential in the manipulation and engineering of interactions, platforms for the simultaneous topological confinement of multiple excitations remain an open challenge. GaAs/AlAs heterostructures exhibit enhanced optomechanical interactions due to the intrinsic colocalization of light and sound. In this work, we designed, fabricated, and experimentally studied a multilayered structure based on GaAs/AlAs. Due to the simultaneously inverted band structures for light and phonons, colocalized interface modes for both 1.34 eV photons and 18 GHz phonons appear. We experimentally validated the concept by optical reflectivity and coherent phonon generation and detection. Furthermore, we theoretically analyzed the performance of different topological designs presenting colocalized states in time-domain Brillouin scattering and deduce engineering rules. Potential future applications include the engineering of robust optomechanical resonators, compatible with the incorporation of active media such as quantum wells and quantum dots.
Multidimensional coherent spectroscopy directly unravels multiply excited states that overlap in a linear spectrum. We report multidimensional coherent optical photocurrent spectroscopy in a semiconductor polariton diode and explore the excitation ladder of cavity polaritons. We measure doubly and triply avoided crossings for pairs and triplets of exciton-polaritons, demonstrating the strong coupling between light and dressed doublet and triplet semiconductor excitations. These results demonstrate that multiply excited excitonic states strongly coupled to a microcavity can be described as two coupled quantum-anharmonic ladders.
B. Real, O. Jamadi, M. Milićević, N. Pernet, P. St-Jean, T. Ozawa, G. Montambaux, I. Sagnes, A. Lemaître, L. Le Gratiet, A. Harouri, S. Ravets, J. Bloch, A. Amo Compression dramatically changes the transport and localization properties of graphene. This is intimately related to the change of symmetry of the Dirac cone when the particle hopping is different along different directions of the lattice. In particular, for a critical compression, a semi-Dirac cone is formed with massless and massive dispersions along perpendicular directions. Here we show direct evidence of the highly anisotropic transport of polaritons in a honeycomb lattice of coupled micropillars implementing a semi-Dirac cone. If we optically induce a vacancy-like defect in the lattice, we observe an anisotropically localized polariton distribution in a single sublattice, a consequence of the semi-Dirac dispersion. Our work opens up new horizons for the study of transport and localization in lattices with chiral symmetry and exotic Dirac dispersions.
P. St-Jean, A. Dauphin, P. Massignan, B. Real, O. Jamadi, M. Milićević, A. Lemaître, A. Harouri, L. Le Gratiet, I. Sagnes, S. Ravets, J. Bloch, A. Amo Topological materials rely on engineering global properties of their bulk energy bands called topological invariants. These invariants, usually defined over the entire Brillouin zone, are related to the existence of protected edge states. However, for an important class of Hamiltonians corresponding to 2D lattices with time-reversal and chiral symmetry (e.g. graphene), the existence of edge states is linked to invariants that are not defined over the full 2D Brillouin zone, but on reduced 1D sub-spaces. Here, we demonstrate a novel scheme based on a combined real- and momentum-space measurement to directly access these 1D topological invariants in lattices of semiconductor microcavities confining exciton-polaritons. We extract these invariants in arrays emulating the physics of regular and critically compressed graphene sucht that Dirac cones have merged. Our scheme provides a direct evidence of the bulk-edge correspondence in these systems, and opens the door to the exploration of more complex topological effects, for example involving disorder and interactions.
O. Jamadi, E. Rozas, G. Salerno, M. Milićević, T. Ozawa, I. Sagnes, A. Lemaître, L. Le Gratiet, A. Harouri, I. Carusotto, J. Bloch, A. Amo We report the realization of a synthetic magnetic field for photons and polaritons in a honeycomb lattice of coupled semiconductor micropillars. A strong synthetic field is induced in both the s and p orbital bands by engineering a uniaxial hopping gradient in the lattice, giving rise to the formation of Landau levels at the Dirac points. We provide direct evidence of the sublattice symmetry breaking of the lowest-order Landau level wavefunction, a distinctive feature of synthetic magnetic fields. Our realization implements helical edge states in the gap between n=0 and n=1 Landau levels, experimentally demonstrating a novel way of engineering propagating edge states in photonic lattices. In light of recent advances in the enhancement of polariton-polariton nonlinearities, the Landau levels reported here are promising for the study of the interplay between pseudomagnetism and interactions in a photonic system.
Kaushalya Jhuria, Julius Hohlfeld, Akshay Pattabi, Elodie Martin, Aldo Ygnacio Arriola Córdova, Xinping Shi, Roberto Lo Conte, Sebastien Petit-Watelot, Juan Carlos Rojas-Sanchez, Gregory Malinowski, Stéphane Mangin, Aristide Lemaître, Michel Hehn, Jeffrey Bokor, Richard B. Wilson, Jon Gorchon Reducing energy dissipation while increasing speed in computation and memory is a long-standing challenge for spintronics research. In the last 20 years, femtosecond lasers have emerged as a tool to control the magnetization in specific magnetic materials at the picosecond timescale. However, the use of ultrafast optics in integrated circuits and memories would require a major paradigm shift. An ultrafast electrical control of the magnetization is far preferable for integrated systems. Here we demonstrate reliable and deterministic control of the out-of-plane magnetization of a 1 nm-thick Co layer with single 6 ps-wide electrical pulses that induce spin-orbit torques on the magnetization. We can monitor the ultrafast magnetization dynamics due to the spin-orbit torques on sub-picosecond timescales, thus far accessible only by numerical simulations. Due to the short duration of our pulses, we enter a counter-intuitive regime of switching where heat dissipation assists the reversal. Moreover, we estimate a low energy cost to switch the magnetization, projecting to below 1fJ for a (20 nm)^3 cell. These experiments prove that spintronic phenomena can be exploited on picosecond time-scales for full magnetic control and should launch a new regime of ultrafast spin torque studies and applications.
V. Goblot, A. Štrkalj, N. Pernet, J. L. Lado, C. Dorow, A. Lemaître, L. Le Gratiet, A. Harouri, I. Sagnes, S. Ravets, A. Amo, J. Bloch, O. Zilberberg Conduction through materials crucially depends on how ordered they are. Periodically ordered systems exhibit extended Bloch waves that generate metallic bands, whereas disorder is known to limit conduction and localize the motion of particles in a medium. In this context, quasiperiodic systems, which are neither periodic nor disordered, reveal exotic conduction properties, self-similar wavefunctions, and critical phenomena. Here, we explore the localization properties of waves in a novel family of quasiperiodic chains obtained when continuously interpolating between two paradigmatic limits: the Aubry-André model, famous for its metal-to-insulator transition, and the Fibonacci chain, known for its critical nature. Using both theoretical analysis and experiments on cavity-polariton devices, we discover that the Aubry-André model evolves into criticality through a cascade of band-selective localization/delocalization transitions that iteratively shape the self-similar critical wavefunctions of the Fibonacci chain. Our findings offer (i) a unique new insight into understanding the criticality of quasiperiodic chains, (ii) a controllable knob by which to engineer band-selective pass filters, and (iii) a versatile experimental platform with which to further study the interplay of many-body interactions and dissipation in a wide range of quasiperiodic models.
We report the observation of a parametric instability in the out-of-equilibrium steady state of two coupled Kerr microresonators coherently driven by a laser. Using a resonant excitation, we drive the system into an unstable regime, where we observe the appearance of intense and well resolved sideband modes in the emission spectrum. This feature is a characteristic signature of self-sustained oscillations of the intracavity field. We comprehensively model our findings using semiclassical Langevin equations for the cavity field dynamics combined with a linear stability analysis. The inherent scalability of our semiconductor platform, enriched with a strong Kerr nonlinearity, is promising for the realization of integrated optical parametric oscillator networks operating in a few-photon regime.
Hélène Ollivier, Ilse Maillette de Buy Wenniger, Sarah Thomas, Stephen Wein, Guillaume Coppola, Abdelmounaim Harouri, Paul Hilaire, Clément Millet, Aristide Lemaître, Isabelle Sagnes, Olivier Krebs, Loïc Lanco, Juan Carlos Loredo, Carlos Antón, Niccolo Somaschi, Pascale Senellart Single-photon sources based on semiconductor quantum dots have emerged as an excellent platform for high efficiency quantum light generation. However, scalability remains a challenge since quantum dots generally present inhomogeneous characteristics. Here we benchmark the performance of fifteen deterministically fabricated single-photon sources. They display an average indistinguishability of 90.6 +/- 2.8 % with a single-photon purity of 95.4 +/- 1.5 % and high homogeneity in operation wavelength and temporal profile. Each source also has state-of-the-art brightness with an average first lens brightness value of 13.6 +/- 4.4 %. Whilst the highest brightness is obtained with a charged quantum dot, the highest quantum purity is obtained with neutral ones. We also introduce various techniques to identify the nature of the emitting state. Our study sets the groundwork for large-scale fabrication of identical sources by identifying the remaining challenges and outlining solutions.
Doping is a fundamental property of semiconductors and constitutes the basis of modern microelectronic and optoelectronic devices. Their miniaturization requires contactless characterization of doping with nanometer scale resolution. Here, we use low- and room-temperature cathodoluminescence (CL) measurements to analyze p-type and n-type GaAs thin films over a wide range of carrier densities ($2\times 10^{17}$ to $1\times 10^{19}$ cm$^{-3}$). The spectral shift and broadening of CL spectra induced by shallow dopant states and band filling are the signature doping. We fit the whole spectral lineshapes with the generalized Planck's law and refined absorption models to extract the bandgap narrowing (BGN) and the band tail for both doping types, and the electron Fermi level for n doping. This work provides a rigorous method for the quantitative assessment of p-type and n-type carrier density using CL. Taking advantage of the high spatial resolution of CL, it can be used to map the doping in GaAs nanostructures, and it could be extended to other semiconductor materials.
Developing future quantum communication may rely on the ability to engineer cavity-mediated interactions between photons and solid-state artificial atoms, in a deterministic way. Here, we report a set of technological and experimental developments for the deterministic coupling between the optical mode of a micropillar cavity and a quantum dot trion transition. We first identify a charged transition through in-plane magnetic field spectroscopy, and then tune the optical cavity mode to its energy via in-situ lithography. In addition, we design an asymmetric tunneling barrier to allow the optical trapping of the charge, assisted by a quasi-resonant pumping scheme, in order to control its occupation probability. We evaluate the generation of a positively-charged quantum dot through second order auto-correlation measurements of its resonance fluorescence, and the quality of light-matter interaction for these spin-photon interfaces is assessed by measuring the performance of the device as a single-photon source.
In this work we present a tight-binding model that allows to describe with a minimal amount of parameters the band structure of exciton-polariton lattices. This model based on $s$ and $p$ non-orthogonal photonic orbitals faithfully reproduces experimental results reported for polariton graphene ribbons. We analyze in particular the influence of the non-orthogonality, the inter-orbitals interaction and the photonic spin-orbit coupling on the polarization and dispersion of bulk bands and edge states.
High-dimensional entangled states of light provide novel possibilities for quantum information, from fundamental tests of quantum mechanics to enhanced computation and communication protocols. In this context, the frequency degree of freedom combines the assets of robustness to propagation and easy handling with standard telecommunication components. Here we use an integrated semiconductor chip to engineer the wavefunction and exchange statistics of frequency-entangled photon pairs directly at the generation stage, without post-manipulation. Tuning the spatial properties of the pump beam allows to generate frequency-anticorrelated, correlated and separable states, and to control the symmetry of the spectral wavefunction to induce either bosonic or fermionic behaviors. These results, supported by analytical and numerical calculations, open promising perspectives for the quantum simulation of fermionic problems with photons on an integrated platform, as well as for communication and computation protocols exploiting antisymmetric high-dimensional quantum states.
We measure the local yield stress, at the scale of small atomic regions, in a deeply quenched two-dimensional glass model undergoing shear banding in response to athermal quasistatic (AQS) deformation. We find that the occurrence of essentially a single plastic event suffices to bring the local yield stress distribution to a well-defined value for all strain orientations, thus essentially erasing the memory of the initial structure. It follows that in a well-relaxed sample, plastic events cause the abrupt (nucleation-like) emergence of a local softness contrast and thus precipitate the formation of a band, which, in its early stages, is measurably softer than the steady-state flow. Moreover, this postevent yield stress ensemble presents a mean value comparable to that of the inherent states of a supercooled liquid around the mode-coupling temperature $T_{\rm MCT}$. This, we argue, explains that the transition between brittle and ductile yielding in amorphous materials occurs around a comparable parent temperature. Our data also permit to capture quantitatively the contributions of pressure and density changes and demonstrate unambiguously that they are negligible compared with the changes of softness caused by structural rejuvenation.
We study the structural origin of the Bauschinger effect by accessing numerically the local plastic thresholds in the steady state flow of a two-dimensional model glass under athermal quasistatic deformation. More specifically, we compute the local residual strength, $\Delta\tau^{c}$, for arbitrary loading orientations and find that plastic deformation generically induces material polarization, i.e., a forward-backward asymmetry in the $\Delta\tau^{c}$ distribution. In steady plastic flow, local packings are on average closer to forward (rather than backward) instabilities, due to the stress-induced bias of barriers. However, presumably due to mechanical noise, a significant fraction of zones lie close to reverse (backward) yielding, as the distribution of $\Delta\tau^{c}$ for reverse shearing extends quasilinearly down to zero local residual strength. By constructing an elementary model of the early plastic response, we then show that unloading causes reverse plasticity of a growing amplitude, i.e., reverse softening, while it shifts away forward-yielding barriers. This result in an inversion of polarization in the low-$\Delta\tau^{c}$ region and, consequently, in the Bauschinger effect. This scenario is quite generic, which explains the pervasiveness of the effect.
V. Goblot, B. Rauer, F. Vicentini, A. Le Boité, E. Galopin, A. Lemaître, L. Le Gratiet, A. Harouri, I. Sagnes, S. Ravets, C. Ciuti, A. Amo, J. Bloch Phase frustration in periodic lattices is responsible for the formation of dispersionless flat bands. The absence of any kinetic energy scale makes flat band physics critically sensitive to perturbations and interactions. We report here on the experimental investigation of the nonlinear dynamics of cavity polaritons in the gapped flat band of a one-dimensional Lieb lattice. We observe the formation of gap solitons with quantized size and very abrupt edges, signature of the frozen propagation of switching fronts. This type of gap solitons belongs to the class of truncated Bloch waves, and had only been observed in closed systems up to now. Here the driven-dissipative character of the system gives rise to a complex multistability of the nonlinear domains generated in the flat band. These results open up interesting perspective regarding more complex 2D lattices and the generation of correlated photon phases.
C. Antón, J. C. Loredo, G. Coppola, H. Ollivier, N. Viggianiello, A. Harouri, N. Somaschi, A. Crespi, I. Sagnes, A. Lemaître, L. Lanco, R. Osellame, F. Sciarrino, P. Senellart Scaling-up optical quantum technologies requires to combine highly efficient multi-photon sources and integrated waveguide components. Here, we interface these scalable platforms: a quantum dot based multi-photon source and a reconfigurable photonic chip on glass are combined to demonstrate high-rate three-photon interference. The temporal train of single-photons obtained from a quantum emitter is actively demultiplexed to generate a 3.8 kHz three-photon source, which is then sent to the input of a tuneable tritter circuit, demonstrating the on-chip quantum interference of three indistinguishable single-photons. Pseudo number-resolving photon detection characterising the output distribution shows that this first combination of scalable sources and reconfigurable photonic circuits compares favourably in performance with respect to previous implementations. A detailed loss-budget shows that merging solid-state based multi-photon sources and reconfigurable photonic chips could allow ten-photon experiments on chip at ${\sim}40$ Hz rate in a foreseeable future.
We explore universal behaviors of magnetic domain wall driven by the spin-transfer of an electrical current, in a ferromagnetic (Ga,Mn)(As,P) thin film with perpendicular magnetic anisotropy. For a current direction transverse to domain wall, the dynamics of the thermally activated creep regime and the depinning transition are found to be compatible with a self-consistent universal description of magnetic field induced domain wall dynamics. This common universal behavior, characteristic of the so-called quenched Edwards-Wilkinson universality class, is confirmed by a complementary and independent analysis of domain wall roughness. However, the tilting of domain walls and the formation of facets is produced by the directionality of interaction with the current, which acts as a magnetic field only in the direction transverse to domain wall.
Light's orbital angular momentum (OAM) is an unbounded degree of freedom emerging in helical beams that appears very advantageous technologically. Using a chiral microlaser, i.e. an integrated device that allows generating an emission carrying a net OAM, we demonstrate a regime of bistability involving two modes presenting distinct OAM (L = 0 and L = 2). Furthermore, thanks to an engineered spin-orbit coupling of light in the device, these modes also exhibit distinct polarization patterns, i.e. cirular and azimuthal polarizations. Using a dynamical model of rate euqations, we show that this bistability arises from polarization-dependent saturation of the gain medium. Such a bistable regime appears very promising for implementing ultrafast optical switches based on the OAM of light. As well, it paves the way to the exploration of dynamical processes involving phase and polarization vortices.
M. Esmann, F. R. Lamberti, A. Harouri, L. Lanco, I. Sagnes, I. Favero, G. Aubin, C. Gomez-Carbonell, A. Lemaitre, O. Krebs, P. Senellart, N. D. Lanzillotti-Kimura We introduce a monolithic Brillouin generator based on a semiconductor micropillar cavity embedding a high frequency nanoacoustic resonator operating in the hundreds of GHz range. The concept of two nested resonators allows an independent design of the ultrahigh frequency Brillouin spectrum and of the optical device. We develop an optical free-space technique to characterize spontaneous Brillouin scattering in this monolithic device and propose a measurement protocol that maximizes the Brillouin generation efficiency in the presence of optically induced thermal effects. The compact and versatile Brillouin generator studied here could be readily integrated into fibered and on-chip architectures.
Inspired by concepts developed for fermionic systems in the framework of condensed matter physics, topology and topological states are recently being explored also in bosonic systems. The possibility of engineering systems with unidirectional wave propagation and protected against disorder is at the heart of this growing interest. Topogical acoustic effects have been observed in a variety of systems, most of them based on kHz-MHz sound waves, with typical wavelength of the order of the centimeter. Recently, some of these concepts have been successfully transferred to acoustic phonons in nanoscaled multilayered systems. The reported demonstration of confined topological phononic modes was based on Raman scattering spectroscopy, yet the resolution did not suffice to determine lifetimes and to identify other acoustic modes in the system. Here, we use time-resolved pump-probe measurements using an asynchronous optical sampling (ASOPS) technique to overcome these resolution limitations. By means of one-dimensional GaAs/AlAs distributed Bragg reflectors (DBRs) as building blocks, we engineer high frequency ($\sim$ 200 GHz) topological acoustic interface states. We are able to clearly distinguish confined topological states from stationary band edge modes. The detection scheme reflects the symmetry of the modes directly through the selection rules, evidencing the topological nature of the measured confined state. These experiments enable a new tool in the study of the more complex topology-driven phonon dynamics such as phonon nonlinearities and optomechanical systems with simultaneous confinement of light and sound.
The magnetic domain wall motion driven by a magnetic field is studied in (Ga,Mn)As and (Ga,Mn)(As,P) films of different thicknesses. In the thermally activated creep regime, a kink in the velocity curves and a jump of the roughness exponent evidence a dimensional crossover in the domain wall dynamics. The measured values of the roughness exponent zeta_1d = 0.62 +/- 0.02 and zeta_2d = 0.45 +/- 0.04 are compatible with theoretical predictions for the motion of elastic line (d = 1) and surface (d = 2) in two and three dimensional media, respectively.
Exciton-polaritons in semiconductor microcavities constitute the archetypal realization of a quantum fluid of light. Under coherent optical drive, remarkable effects such as superfluidity, dark solitons or the nucleation of hydrodynamic vortices have been observed. These phenomena can be all understood as a specific manifestation of collective excitations forming on top of the polariton condensate. In this work, we performed a Brillouin scattering experiment to measure their dispersion relation $\omega(\mathbf{k})$ directly. The result, such as a speed of sound which is apparently twice too low, cannot be explained upon considering the polariton condensate alone. In a combined theoretical and experimental analysis, we demonstrate that the presence of a reservoir of long-lived excitons interacting with polaritons has a dramatic influence on the nature and characteristic of the quantum fluid, and that it explains our measurement quantitatively. This work clarifies the role of such a reservoir in the different polariton hydrodynamics phenomena occurring under resonant optical drive. It also provides an unambiguous tool to determine the condensate-to-reservoir fraction in the quantum fluid, and sets an accurate framework to approach novel ideas for polariton-based quantum-optical applications.
We rigorously establish that, in disordered three-dimensional (3D) isotropic solids, the stress autocorrelation function presents anisotropic terms that decay as $1/r^3$ at long-range, with $r$ the distance, as soon as either pressure or shear stress fluctuations are normal. By normal, we mean that the fluctuations of stress, as averaged over spherical domains, decay as the inverse domain volume. Since this property is required for macroscopic stress to be self-averaging, it is expected to hold generically in all glasses and we thus conclude that the presence of $1/r^3$ stress correlation tails is the rule in these systems. Our proof follows from the observation that, in an infinite medium, when both material isotropy and mechanical balance hold, (i) the stress autocorrelation matrix is completely fixed by just two radial functions: the pressure autocorrelation and the trace of the autocorrelation of stress deviators; furthermore, these two functions (ii) fix the decay of the fluctuations of sphere-averaged pressure and deviatoric stresses for windows of increasing volume. Our conclusion is reached because, due to the precise analytic relation (i) fixed by isotropy and mechanical balance, the constraints arising via (ii) from the normality of stress fluctuations demand the spatially anisotropic stress correlation terms to decay as $1/r^3$ at long-range. For the sake of generality, we also examine situations when stress fluctuations are not normal.
Quentin Barbedienne, Julien Varignon, Nicolas Reyren, Alain Marty, Celine Vergnaud, Matthieu Jamet, Carmen Gomez-Carbonell, Aristide Lemaître, Patrick Le Fèvre, François Bertran, Amina Taleb-Ibrahimi, Henri Jaffrès, Jean-Marie George, Albert Fert Gray tin, also known as $\alpha$-Sn, can be turned into a three-dimensional topological insulator (3D-TI) by strain and finite size effects. Such room temperature 3D-TI is peculiarly interesting for spintronics due to the spin-momentum locking along the Dirac cone (linear dispersion) of the surface states. Angle resolved photoemission spectroscopy (ARPES) has been used to investigate the dispersion close to the Fermi level in thin (0\u20090\u20091)-oriented epitaxially strained films of $\alpha$-Sn, for different film thicknesses as well as for different capping layers (Al, AlO$_x$ and MgO). Indeed a proper capping layer is necessary to be able to use $\alpha$-Sn surface states for spintronics applications. In contrast with free surfaces or surfaces coated with Ag, coating the $\alpha$-Sn surface with Al or AlO$_x$ leads to a drop of the Fermi level below the Dirac point, an important consequence for transport is the presence of bulk states at the Fermi level. $\alpha$-Sn films coated by AlO$_x$ are studied by electrical magnetotransport: despite clear evidence of surface states revealed by Shubnikov-de Haas oscillations, an important part of the magneto-transport properties is governed by "bulk" electronic states attributed to the $\Gamma 8$ band, as suggested by \it ab-initio calculations.
The extraordinary electronic properties of Dirac materials, the two-dimensional partners of Weyl semimetals, arise from the linear crossings in their band structure. When the dispersion around the Dirac points is tilted, the emergence of intricate transport phenomena has been predicted, such as modified Klein tunnelling, intrinsic anomalous Hall effects and ferrimagnetism. However, Dirac materials are rare, particularly with tilted Dirac cones. Recently, artificial materials whose building blocks present orbital degrees of freedom have appeared as promising candidates for the engineering of exotic Dirac dispersions. Here we take advantage of the orbital structure of photonic resonators arranged in a honeycomb lattice to implement photonic lattices with semi-Dirac, tilted and, most interestingly, type-III Dirac cones that combine flat and linear dispersions. The tilted cones emerge from the touching of a flat and a parabolic band with a non-trivial topological charge. These results open the way to the synthesis of orbital Dirac matter with unconventional transport properties and, in combination with polariton nonlinearities, to the study of topological and Dirac superfluids in photonic lattices.
The resonant interaction of electrically excited travelling surface acoustic waves and magnetization has been hitherto probed through the acoustic component. In this work it is investigated using time-resolved magneto-optical detection of magnetization dynamics. To that end, we develop an experimental scheme where laser pulses are used both to generate the acoustic wave frequency and to probe magnetization dynamics thus ensuring perfect phase locking. The light polarization dependence of the signal enables to disentangle elasto-optic and magneto-optic contributions and to obtain the in-plane and out-of-plane dynamic magnetization components. Magnetization precession is proved to be driven solely by the acoustic wave. Its amplitude is shown to resonate at the same field at which we detect piezo-electrically the resonant attenuation of the acoustic wave, clearly evidencing the magneto-acoustic resonance with high sensitivity.
Nicola Carlon Zambon, Philippe St-Jean, Marijana Milićević, Aristide Lemaître, Abdelmounaim Harouri, Luc LeGratiet, Olivier Bleu, Dmitry Solnyshkov, Guillaume Malpuech, Isabelle Sagnes, Sylvain Ravets, Alberto Amo, Jacqueline Bloch Orbital angular momentum (OAM) carried by helical light beams is an unbounded degree of freedom of photons that offers a promising playground in modern photonics. So far, integrated sources of coherent light carrying OAM are based on resonators whose design imposes a single, non-tailorable chirality of the wavefront (i.e. clockwise or counter clockwise vortices). Here, we propose and demonstrate the realization of an integrated microlaser where the chirality of the wavefront can be optically controlled. Importantly, the scheme that we use, based on an effective spin-orbit coupling of photons in a semiconductor microcavity, can be extended to different laser architectures, thus paving the way to the realization of a new generation of OAM microlasers with tunable chirality.
We report polariton lasing in localised gap states in a honeycomb lattice of coupled micropillars. Localisation of the modes is induced by the optical potential created by the excitation beam, requiring no additional engineering of the otherwise homogeneous polariton lattice. The spatial shape of the gap states arises from the interplay of the orbital angular momentum eigenmodes of the cylindrical potential created by the excitation beam and the hexagonal symmetry of the underlying lattice. Our results provide insights into the engineering of defect states in two-dimensional lattices.
We study ultra-cold dipolar excitons confined in a 10$\mu$m trap of a double GaAs quantum well. Based on the local density approximation, we unveil for the first time the equation of state of excitons at pure thermodynamic equilibrium. In this regime we show that, below a critical temperature of about $1$ Kelvin, a superfluid forms in the inner region of the trap at a local exciton density $n \sim 2-3 \, 10^{10} \text{cm}^{-2}$, encircled by a more dilute and normal component in the outer rim of the trap. Remarkably, this spatial arrangement correlates directly with the concentration of defects in the exciton density which exhibits a sudden decrease at the onset of superfluidity, thus pointing towards an underlying Berezinskii-Kosterlitz-Thouless mechanism.
The Su-Schrieffer-Heeger (SSH) model is likely the simplest one-dimensional concept to study non-trivial topological phases and topological excitations. Originally developed to explain the electric conductivity of polyacetylene, it has become a platform for the study of topological effects in electronics, photonics and ultra-cold atomic systems. Here, we propose an experimentally feasible implementation of the SSH model based on coupled one-dimensional acoustic nanoresonators working in the GHz-THz range. In this simulator it is possible to implement different signs in the nearest neighbor interaction terms, showing full tunability of all parameters in the SSH model. Based on this concept we construct topological transition points generating nanophononic edge and interface states and propose an easy scheme to experimentally probe their spatial complex amplitude distribution directly by well-established optical pump-probe techniques.
We show on in-plane magnetized thin films that magnetization can be switched efficiently by 180 degrees using large amplitude Rayleigh waves travelling along the hard or easy magnetic axis. Large characteristic filament-like domains are formed in the latter case. Micromagnetic simulations clearly confirm that this multi-domain configuration is compatible with a resonant precessional mechanism. The reversed domains are in both geometries several hundreds of \mu m^2, much larger than has been shown using spin transfer torque- or field-driven precessional switching. We show that surface acoustic waves can travel at least 1mm before addressing a given area, and can interfere to create magnetic stripes that can be positionned with a sub-micronic precision.
Pillar microcavities are excellent light-matter interfaces providing an electromagnetic confinement in small mode volumes with high quality factors. They also allow the efficient injection and extraction of photons, into and from the cavity, with potentially near-unity input and output-coupling efficiencies. Optimizing the input and output coupling is essential, in particular, in the development of solid-state quantum networks where artificial atoms are manipulated with single incoming photons. Here we propose a technique to accurately measure input and output coupling efficiencies using polarization tomography of the light reflected by the cavity. We use the residual birefringence of pillar microcavities to distinguish the light coupled to the cavity from the uncoupled light: the former participates to rotating the polarization of the reflected beam, while the latter decreases the polarization purity. Applying this technique to a micropillar cavity, we measure a $53 \pm2 \% $ output coupling and a $96 \pm 1\%$ input coupling with unprecedented precision.