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Biphoton frequency comb (BFC), which encompasses multiple discrete frequency modes and represents high-dimensional frequency entanglement, is crucial in quantum information processing due to its high information capacity and error resilience. It also holds significant potential for enhancing timing precision in quantum metrology. Here, we examine quantum metrology timing limits using the BFC as a probe state and derive a quantum Cramér-Rao bound that scales quadratically with the number of frequency modes. Under ideal conditions (zero loss and perfect visibility), this bound can be saturated by both spectrally non-resolved Hong-Ou-Mandel (HOM) interferometry at zero delay and spectrally resolved HOM interferometry at arbitrary delays. In particular, under imperfect experimental conditions, Fisher information rapidly increases up to its maximum as the mode number increases for a fixed time delay close to zero, indicating that increasing the mode number is an optimal strategy for improving the timing precision in practice. Furthermore, compared with spectrally non-resolved measurement, spectrally resolved measurement is a better strategy due to its higher Fisher information, shorter measurement times, and ambiguity-free dynamic range.

It is thought that schemes for quantum imaging are fragile against realistic environments in which the background noise is often stronger than the nonclassical signal of the imaging photons. Unfortunately, it is unfeasible to produce brighter quantum light sources to alleviate this problem. Here, we overcome this paradigmatic limitation by developing a quantum imaging scheme that relies on the use of natural sources of light. This is achieved by performing conditional detection on the photon number of the thermal light field scattered by a remote object. Specifically, the conditional measurements in our scheme enable us to extract quantum features of the detected thermal photons to produce quantum images with improved signal-to-noise ratios. This technique shows a remarkable exponential enhancement in the contrast of quantum images. Surprisingly, this measurement scheme enables the possibility of producing images from the vacuum fluctuations of the light field. This is experimentally demonstrated through the implementation of a single-pixel camera with photon-number-resolving capabilities. As such, we believe that our scheme opens a new paradigm in the field of quantum imaging. It also unveils the potential of combining natural light sources with nonclassical detection schemes for the development of robust quantum technologies.

We theoretically propose a multiparameter cascaded quantum interferometer in which a two-input and two-output setup is obtained by concatenating 50:50 beam splitters with n independent and adjustable time delays. A general method for deriving the coincidence probability of such an interferometer is given based on the linear transformation of the matrix of beam splitters. As examples, we analyze the interference characteristics of one-, two- and three-parameter cascaded quantum interferometers with different frequency correlations and input states. Some typical interferograms of such interferometers are provided to reveal more rich and complicated two-photon interference phenomena. In principle, arbitrary two-input and two-output experimental setups can be designed with the proposal. This work offers a toolbox for designing versatile quantum interferometers and provides a convenient method for deriving the coincidence probabilities involved. Potential applications can be found in the complete spectral characterization of two-photon states, multiparameter estimation, and quantum metrology.

Entangled photon pairs are crucial resources for quantum information processing protocols. Via the process of spontaneous parametric down-conversion (SPDC), we can generate these photon pairs using bulk nonlinear crystals. Traditionally, the crystal is designed to satisfy specific type of phase-matching condition. Here, we report controllable transitions among different types of phase-matching in a single periodically poled potassium titanyl phosphate (PPKTP) crystal. By carefully selecting pump conditions, we can satisfy different phase-matching conditions. This allows us to observe first-order type-II, fifth-order type-I, third-order type-0, and fifth-order type-II SPDCs. The temperature-dependent spectra of our source were also analyzed in detail. Finally, we discussed the possibility of observing more than nine SPDCs in this crystal. Our work not only deepens the understanding of the physics behind phase-matching conditions, but also offers the potential for a highly versatile entangled biphoton source for quantum information research.

Entangled photons (biphotons) in the time-frequency degree of freedom play a crucial role in both foundational physics and advanced quantum technologies. Fully characterizing them poses a key scientific challenge. Here, we propose a theoretical approach to achieving the complete tomography of biphotons by introducing a frequency shift in one arm of the combination interferometer. Our method, a generalized combination interferometer, enables the reconstruction of the full complex joint spectral amplitude associated with both frequency sum and difference in a single interferometer. In contrast, the generalized Hong-Ou-Mandel and N00N state interferometers only allow for the partial tomography of biphotons, either in frequency difference or frequency sum. This provides an alternative method for full characterization of an arbitrary two-photon state with exchange symmetry and holds potential for applications in high-dimensional quantum information processing.

Interference, which refers to the phenomenon associated with the superposition of waves, has played a crucial role in the advancement of physics and finds a wide range of applications in physical and engineering measurements. Interferometers are experimental setups designed to observe and manipulate interference. With the development of technology, many quantum interferometers have been discovered and have become cornerstone tools in the field of quantum physics. Quantum interferometers not only explore the nature of the quantum world but also have extensive applications in quantum information technology, such as quantum communication, quantum computing, and quantum measurement. In this review, we analyze and summarize three typical quantum interferometers: the Hong-Ou-Mandel (HOM) interferometer, the N00N state interferometer, and the Franson interferometer. We focus on the principles and applications of these three interferometers. In the principles section, we present the theoretical models for these interferometers, including single-mode theory and multi-mode theory. In the applications section, we review the applications of these interferometers in quantum communication, computation, and measurement. We hope that this review article will promote the development of quantum interference in both fundamental science and practical engineering applications.

Franson interference can be used to test the nonlocal features of energy-time entanglement and has become a standard in quantum physics. However, most of the previous Franson interference experiments were demonstrated in the time domain, and the spectral properties of Franson interference have not been fully explored. Here, we theoretically and experimentally demonstrate spectrally resolved Franson interference using biphotons with different correlations, including positive correlation, negative correlation, and non-correlation. It is found that the joint spectral intensities of the biphotons can be modulated along both the signal and idler directions, which has potential applications in generating high-dimensional frequency entanglement and time-frequency grid states. This work may provide a new perspective for understanding the spectral-temporal properties of the Franson interferometer.

Entangled qudits, the high-dimensional entangled states, play an important role in the study of quantum information. How to prepare entangled qudits in an efficient and easy-to-operate manner is still a challenge in quantum technology. Here, we demonstrate a method to engineer frequency entangled qudits in a spontaneous parametric downconversion process. The proposal employs an angle-dependent phase-matching condition in a nonlinear crystal, which forms a classical-quantum mapping between the spatial (pump) and spectral (biphotons) degrees of freedom. In particular, the pump profile is separated into several bins in the spatial domain, and thus shapes the down-converted biphotons into discrete frequency modes in the joint spectral space. Our approach provides a feasible and efficient method to prepare a high-dimensional frequency entangled state. As an experimental demonstration, we generate a three-dimensional entangled state by using a homemade variable slit mask.

We theoretically propose a novel quantum interferometer in which the NOON state interferometer (NOONI) is combined with the Hong-Ou-Mandel interferometer (HOMI). This interferometer combined the advantages of both the NOONI that depends on biphoton frequency sum, and the HOMI that depends on biphoton frequency difference into a single interferometer. It can thus simultaneously obtain the spectral correlation information of biphotons in both frequency sum and difference by taking the Fourier transform from a single time-domain quantum interferogram, which provides a method for complete spectral characterization of an arbitrary two-photon state with exchange symmetry. A direct application of such an interferometer can be found in quantum Fourier-transform spectroscopy where direct spectral measurement is difficult. Furthermore, as it can realize the measurement of time intervals on three scales at the same time, we expect that it can provide a new method in quantum metrology. Finally, we discuss another potential application of such an interferometer in the generation and characterization of high-dimensional and phase-controlled frequency entanglement.

We theoretically investigate the preparation of pure-state single-photon source from 14 birefringent crystals (CMTC, THI, LiIO$_3$, AAS, HGS, CGA, TAS, AGS, AGSe, GaSe, LIS, LISe, LGS, and LGSe) and 8 periodic poling crystals (LT, LN, KTP, KN, BaTiO$_3$, MgBaF$_4$, PMN-0.38PT, and OP-ZnSe) in a wavelength range from 1224 nm to 11650 nm. The three kinds of group-velocity-matching (GVM) conditions, the phase matching conditions, the spectral purity, and the Hong-Ou-Mandel interference are calculated for each crystal. This study may provide high-quality single-photon sources for quantum sensing, quantum imaging, and quantum communication applications at the mid-infrared wavelength range.

The mid-infrared (MIR) band entangled photon source is vital for the next generation of quantum communication, quantum imaging, and quantum sensing. However, the current entangled states are mainly prepared in visible or near-infrared bands. It is still lack of high-quality entangled photon sources in the MIR band. In this work, we optimize the poling sequence of lithium niobate to prepare two kinds of typical entangled states, the Hermit-Gaussian state and the comb-like entangled state at 3.2 $\mu$m. We have also calculated the photon pair rates and estimated the effect of fabrication resolution in the schemes. Our approach will provide entangled photon sources with excellent performance for the study of quantum information in the MIR band.

Recent investigations suggest that the use of non-classical states of light, such as entangled photon pairs, may open new and exciting avenues in experimental two-photon absorption spectroscopy. Despite several experimental studies of entangled two-photon absorption (eTPA), there is still a heated debate on whether eTPA has truly been observed. This interesting debate has arisen, mainly because it has been recently argued that single-photon-loss mechanisms, such as scattering or hot-band absorption may mimic the expected entangled-photon linear absorption behavior. In this work, we focus on transmission measurements of eTPA, and explore three different two-photon quantum interferometers in the context of assessing eTPA. We demonstrate that the so-called N00N-state configuration is the only one amongst those considered insensitive to linear (single-photon) losses. Remarkably, our results show that N00N states may become a potentially powerful tool for quantum spectroscopy, and place them as a strong candidate for the certification of eTPA in an arbitrary sample.

The Hilbert hotel is an old mathematical paradox about sets of infinite numbers. This paradox deals with the accommodation of a new guest in a hotel with an infinite number of occupied rooms. Over the past decade, there have been many attempts to implement these ideas in photonic systems. In addition to the fundamental interest that this paradox has attracted, this research is motivated by the implications that the Hilbert hotel has for quantum communication and sensing. In this work, we experimentally demonstrate the fractional vortex Hilbert's hotel scheme proposed by G. Gbur [Optica 3, 222-225 (2016)]. More specifically, we performed an interference experiment using the fractional orbital angular momentum of light to verify the Hilbert's infinite hotel paradox. In our implementation, the reallocation of a guest in new rooms is mapped to interference fringes that are controlled through the topological charge of an optical beam.

A modified Hong--Ou--Mandel (HOM) interference reveals that the two-photon interference phenomenon can be explained only by the concept of a two-photon wave packet rather than a single-photon one. However, the temporal interferogram in the modified HOM interferometer becomes flat in some cases so that no useful information can be extracted from time-domain measurement. Here, we theoretically explore such temporal interferogram from the frequency domain and obtain the spectrally resolved interference with high visibility. The result represents a modulation of the joint spectral intensity along both the frequency sum and the frequency difference directions. This is quite different from the cases of the spectrally resolved HOM interference and N00N state interference where the modulations happened only in one direction. Moreover, we have shown that such modulations have a potential application in the generation and characterization of high-dimensional frequency entanglement.

Quantum light sources in the mid-infrared (MIR) band play an important role in many applications, such as quantum sensing, quantum imaging, and quantum communication. However, there is still a lack of high-quality quantum light sources in the MIR band, such as the spectrally pure single-photon source. In this work, we present the generation of spectrally-pure state in an optimized poled lithium niobate crystal using a metaheuristic algorithm. In particular, we adopt the particle swarm optimization algorithm to optimize the duty cycle of the poling period of the lithium niobate crystal. With our approach, the spectral purity can be improved from 0.820 to 0.998 under the third group-velocity-matched condition, and the wavelength-tunable range is from 3.0 $\mu$m to 4.0 $\mu$m for the degenerate case and 3.0 $\mu$m to 3.7 $\mu$m for the nondegenerate case. Our work paves the way for developing quantum photonic technologies at the MIR wavelength band.

Highly efficient terahertz (THz) wave sources based on difference frequency generation (DFG) process in nonlinear optical crystals play an important role for the applications of THz wave. In order to find more novel nonlinear crystals, here we theoretically investigate the generation of THz wave using the isomorphs of periodically poled $\mathrm{KTiOPO_4}$ (PPKTP), including periodically poled RTP, KTA, RTA and CTA. By solving the cascaded difference frequency coupled wave equations, it is found that the intensities of the THz wave generated from the cascaded difference frequency processes are improved by 5.27, 2.87, 2.82, 3.03, and 2.76 times from the non-cascaded cases for KTP, RTP, KTA, RTA and CTA, respectively. The effects of the crystal absorption, the phase mismatch and the pump intensity are also analyzed in detail. This study might help to provide a stronger THz radiation source based on the nonlinear crystals.

We experimentally demonstrate a polarization-entangled photon source at 810 nm using a type-II phase-matched PPKTP crystal pumped by a low-cost, broadband laser diode with a central wavelength of 405 nm and a typical bandwidth of 0.53 nm. The PPKTP crystal is placed in a Sagnac-loop to realize the compact size and high stability. The downconverted biphotons, the signal and the idler, have typical bandwidths of 5.57 nm and 7.32 nm. We prepare two Bell states |Psi+> and |Psi-> with the fidelities of 0.948+-0.004 and 0.963+-0.002. In polarization correlation measurement, the visibilities are all higher than 96.2%, and in the Bell inequality test, the S value can achieve 2.78+-0.01. To our knowledge, this experiment is the first to combine a multi-mode pump laser with a Sagnac-loop configuration. This high-quality and low-cost entangled photon source may have many practical applications in quantum information processing.

We theoretically investigate the preparation of mid-infrared (MIR) spectrally-uncorrelated biphotons from a spontaneous parametric down-conversion process using doped LN crystals, including MgO doped LN, ZnO doped LN, and In2O3 doped ZnLN with doping ratio from 0 to 7 mol%. The tilt angle of the phase-matching function and the corresponding poling period are calculated under type-II, type-I, and type-0 phase-matching conditions. We also calculate the thermal properties of the doped LN crystals and their performance in Hong-Ou-Mandel interference. It is found that the doping ratio has a substantial impact on the group-velocity-matching (GVM) wavelengths. Especially, the GVM2 wavelength of co-doped InZnLN crystal has a tunable range of 678.7 nm, which is much broader than the tunable range of less than 100 nm achieved by the conventional method of adjusting the temperature. It can be concluded that the doping ratio can be utilized as a degree of freedom to manipulate the biphoton state. The spectrally uncorrelated biphotons can be used to prepare pure single-photon source and entangled photon source, which may have promising applications for quantum-enhanced sensing, imaging, and communications at the MIR range.

We present the positive-partial-transpose squared conjecture introduced by M. Christandl at Banff International Research Station Workshop: Operator Structures in Quantum Information Theory (Banff International Research Station, Alberta, 2012). We investigate the conjecture in higher dimensions and offer two novel approaches (decomposition and composition of quantum channels) and correspondingly, several schemes for finding counterexamples to this conjecture. One of the schemes involving the composition of PPT quantum channels in unsolved dimensions yields a potential counterexample.

We theoretically investigated spectrally uncorrelated biphotons generated in a counter-propagating spontaneous parametric downconversion (CP-SPDC) from periodically poled MTiOXO4 (M = K, Rb, Cs; X = P, As) crystals. By numerical calculation, it was found that the five crystals from the KTP family can be used to generate heralded single photons with high spectral purity and wide tunability. Under the type-0 phase-matching condition, the purity at 1550 nm was between 0.91 and 0.92, and the purity can be maintained over 0.90 from 1500 nm to 2000 nm wavelength. Under the type-II phase-matching condition, the purity at 1550 nm was 0.96, 0.97, 0.97, 0.98, and 0.98 for PPKTP, PPRTP, PPKTA, PPRTA, and PPCTA, respectively; furthermore, the purity can be kept over 0.96 for more than 600 nm wavelength range. We also simulated the Hong-Ou-Mandel interference between independent photon sources for PPRTP crystals at 1550 nm, and interference visibility was 92% (97%) under type-0 (type-II) phase-matching condition. This study may provide spectrally pure narrowband single-photon sources for quantum memories and quantum networks at telecom wavelengths.

Spectrally intrinsically uncorrelated biphoton states generated from nonlinear crystals are very important but rare resources for quantum photonics and quantum information applications. Previously, such biphoton states were generated from several kinds of crystals, however, their wavelength ranges and nonlinear efficiencies were still limited for various applications. In order to explore new crystal for wider wavelength range and higher nonlinear efficiency, here we theoretically study the generation of spectrally uncorrelated biphoton states from 14 crystals in the `BBO family', including BBO, CLBO, KABO, KBBF, RBBF, CBBF, BABF, BiBO, LBO, CBO, LRB4, LCB, YCOB, and GdCOB. They satisfy three kinds of group-velocity matching condition from near-infrared to telecom wavelengths. Furthermore, heralded single photons can be generated with a purity as high as 0.98, which is achieved without any narrow filtering. The indistinguishability of photons from independent sources is examined by the Hong-Ou-Mandel interference, which results in a visibility of 98% also without any further filtering, i.e., photons from different heralded single-photon sources are highly indistinguishable. Our study may provide single-photon sources with good performance for quantum information processing at near-infrared and telecom wavelengths.

Spectrally uncorrelated biphoton state generated from the spontaneous nonlinear optical process is an important resource for quantum information. Currently such spectrally uncorrelated biphoton state can only be prepared from limited kinds of nonlinear media, thus limiting their wavelengths. In order to explore wider wavelength range, here we theoretically study the generation of spectrally uncorrelated biphoton state from 14 isomorphs of potassium dihydrogen phosphate (KDP) crystal. We find that 11 crystals from the `KDP family' still maintain similar nonlinear optical properties of KDP, such as KDP, DKDP, ADP, DADP, ADA, DADA, RDA, DRDA, RDP, DRDP and KDA, which satisfy 3 kinds of the group-velocity matching conditions for spectrally uncorrelated biphoton state generation from near-infrared to telecom wavelengths. Based on the uncorrelated biphoton state, we investigate the generation of heralded pure-state single photon by detecting one member of the biphoton state to herald the output of the other. The purity of the heralded single photon is as high as 0.98 without using a narrow-band filter; the Hong-Ou-Mandel interference from independent sources can also achieve a visibility of 98%. This study may provide more and better single-photon sources for quantum information processing at near-infrared and telecom wavelengths.

We theoretically and numerically investigate the temperature-dependent properties of the biphotons generated from four isomorphs of periodically poled $\mathrm{KTiOPO_4}$ (PPKTP): i.e., PPRTP, PPKTA, PPRTA and PPCTA. It is discovered that the first type of group-velocity-matched (GVM) wavelength is decreased by 6.4, 1.2, 8.9, 25.6 and 6.3 nm, while the phase-matched wavelength is decreased by 4.4, -0.4, -1.2, 29.1 and 59.5 nm for PPKTP, PPRTP, PPKTA, PPRTA and PPCTA, respectively, when the temperature is increased from 20$\,^{\circ}\mathrm{C}$ to 120$\,^{\circ}\mathrm{C}$. Although the maximal spectral purity of the heralded single photons is not changed at different temperature, the Hong-Ou-Mandel (HOM) interference shows different patterns due to a shift of the joint spectral amplitude. These thermal effects are very important for precise control of the quantum state for the future applications in quantum information processing, for example, in quantum interference or spectroscopy.

Time-frequency duality, which enables control of optical waveforms by manipulating amplitudes and phases of electromagnetic fields, plays a pivotal role in a wide range of modern optics. The conventional one-dimensional (1D) time-frequency duality has been successfully applied to characterize the behavior of classical light, such as ultrafast optical pulses from a laser. However, the 1D treatment is not enough to characterize quantum mechanical correlations in the time-frequency behavior of multiple photons, such as the biphotons from parametric down conversion. The two-dimensional treatment is essentially required, but has not been fully demonstrated yet due to the technical problem. Here, we study the two-dimensional (2D) time-frequency duality duality of biphotons, by measuring two-photon distributions in both frequency and time domains. It was found that generated biphotons satisfy the Fourier limited condition quantum mechanically, but not classically, by analyzing the time-bandwidth products in the 2D Fourier transform. Our study provides an essential and deeper understanding of light beyond classical wave optics, and opens up new possibilities for optical synthesis in a high-dimensional frequency space in a quantum manner.

The classical Wiener-Khinchin theorem (WKT), which can extract spectral information by classical interferometers through Fourier transform, is a fundamental theorem used in many disciplines. However, there is still need for a quantum version of WKT, which could connect correlated biphoton spectral information by quantum interferometers. Here, we extend the classical WKT to its quantum counterpart, i.e., extended WKT (e-WKT), which is based on two-photon quantum interferometry. According to the e-WKT, the difference-frequency distribution of the biphoton wavefunctions can be extracted by applying a Fourier transform on the time-domain Hong-Ou-Mandel interference (HOMI) patterns, while the sum-frequency distribution can be extracted by applying a Fourier transform on the time-domain NOON state interference (NOONI) patterns. We also experimentally verified the WKT and e-WKT in a Mach-Zehnder interference (MZI), a HOMI and a NOONI. This theorem can be directly applied to quantum spectroscopy, where the spectral correlation information of biphotons can be obtained from time-domain quantum interferences by Fourier transform. This may open a new pathway for the study of light-matter interaction at the single photon level.

Multiparticle interference is a fundamental phenomenon in the study of quantum mechanics.It was discovered in a recent experiment [Ra, Y.-S. et al, Proc. Natl Acad. Sci. USA \textbf110, 1227(2013)] that spectrally uncorrelated biphotons exhibited a nonmonotonic quantum-to-classical transition in a four-photon Hong-Ou-Mandel (HOM) interference. In this work, we consider the same scheme with spectrally correlated photons.By theoretical calculation and numerical simulation, we found the transition not only can be nonmonotonic with negative-correlated or uncorrelated biphotons, but also can be monotonic with positive-correlated biphotons. The fundamental reason for this difference is that the HOM-type multi-photon interference is a differential-frequency interference. Our study may shed new light on understanding the role of frequency entanglement in multi-photon behavior.

We present a detailed numerical investigation of five nonlinear materials and their properties regarding photon-pair creation using parametric downconversion. Periodic poling of ferroelectric nonlinear materials is a convenient way to generate collinearly propagating photon pairs. Most applications and experiments use the well-known potassium titanyl phosphate (KTiOPO4, ppKTP) and lithium niobate (LiNbO3, ppLN) crystals for this purpose. In this article we provide a profound discussion on the family of KTP-isomorphic nonlinear materials, including KTP itself but also the much less common CTA (CsTiOAsO4), KTA (KTiOAsO4), RTA (RbTiOAsO4) and RTP (RbTiOPO4). We discuss in which way these crystals can be used for creation of spectrally pure downconversion states and generation of crystal-intrinsic polarisation- and frequency entanglement. The investigation of the new materials disclosed a whole new range of promising experimental setups, in some cases even outperforming the established materials ppLN and ppKTP.

Significant successes have recently been reported in the study of the generation of spectrally pure state in group-velocity-matched (GVM) nonlinear crystals. However, the GVM condition can only be realized in limited kinds of crystals and at limited wavelengths. Here, we investigate pure state generation in the isomorphs of PPKTP crystal: i.e., periodically poled RTP, KTA, RTA and CTA crystals. By numerical simulation, we find that these crystals from the KTP family can generate pure photons with high spectral purity (over 0.8), wide tunability (more than 400 nm), reasonable nonlinearity at a variety of wavelengths (from 1300 nm to 2100 nm). It is also discovered that the PPCTA crystal may achieve purity of 0.97 at 1506 nm. This study may provide more and better choices for quantum state engineering at telecom wavelengths.

NOON state interference (NOON-SI) is a powerful tool to improve the phase sensing precision, and can play an important role in quantum sensing and quantum imaging. However, most of the previous NOON-SI experiments only investigated the center part of the interference pattern, while the full range of the NOON-SI pattern has not yet been well explored.In this Letter, we experimentally and theoretically demonstrate up to six-photon NOON-SI and study the properties of the interference patterns over the full range.The multi-photons were generated at a wavelength of 1584 nm from a PPKTP crystal in a parametric down conversion process.It was found that the shape, the coherence time and the visibility of the interference patterns were strongly dependent on the detection schemes.This experiment can be used for applications which are based on the envelope of the NOON-SI pattern, such as quantum spectroscopy and quantum metrology.

Hong-Ou-Mandel (HOM) interference between independent photon sources (HOMI-IPS) is the fundamental block for quantum information processing, such as quantum gate, Shor's algorithm, Boson sampling, etc. All the previous HOMI-IPS experiments were carried out in time-domain, however, the spectral information during the interference was lost, due to technical difficulties. Here, we investigate the HOMI-IPS in spectral domain using the recently developed fast fiber spectrometer, and demonstrate the spectral distribution during the HOM interference between two heralded single-photon sources, and two thermal sources. This experiment can not only deepen our understanding of HOMI-IPS in the spectral domain, but also be utilized to improve the visibility by post-processing spectral filtering.

In spontaneous parametric down conversion (SPDC) based quantum information processing (QIP) experiments, there is a tradeoff between the coincide count rates (i.e. the pumping power of the SPDC), which limits the rate of the protocol, and the visibility of the quantum interference, which limits the quality of the protocol. This tradeoff is mainly caused by the multi-photon pair emissions from the SPDCs. In theory, the problem is how to model the experiments without truncating these multi-photon emissions while including practical imperfections. In this paper, we establish a method to theoretically simulate SPDC based QIPs which fully incorporates the effect of multi-photon emissions and various practical imperfections. The key ingredient in our method is the application of the characteristic function formalism which has been used in continuous variable QIPs. We apply our method to three examples, the Hong-Ou-Mandel interference and the Einstein-Podolsky-Rosen interference experiments, and the concatenated entanglement swapping protocol. For the first two examples, we show that our theoretical results quantitatively agree with the recent experimental results. Also we provide the closed expressions for these the interference visibilities with the full multi-photon components and various imperfections. For the last example, we provide the general theoretical form of the concatenated entanglement swapping protocol in our method and show the numerical results up to 5 concatenations. Our method requires only a small computation resource (few minutes by a commercially available computer) which was not possible by the previous theoretical approach. Our method will have applications in a wide range of SPDC based QIP protocols with high accuracy and a reasonable computation resource.

Entanglement swapping at telecom wavelengths is at the heart of quantum networking in optical fiber infrastructures. Although entanglement swapping has been demonstrated experimentally so far using various types of entangled photon sources both in near-infrared and telecom wavelength regions, the rate of swapping operation has been too low to be applied to practical quantum protocols, due to limited efficiency of entangled photon sources and photon detectors. Here we demonstrate drastic improvement of the efficiency at telecom wavelength by using two ultra-bright entangled photon sources and four highly efficient superconducting nanowire single photon detectors.We have attained a four-fold coincidence count rate of 108 counts per second, which is three orders higher than the previous experiments at telecom wavelengths. A raw (net) visibility in a Hong-Ou-Mandel interference between the two independent entangled sources was 73.3 $\pm$ 1.0% (85.1 $\pm$ 0.8%). We performed the teleportation and entanglement swapping, and obtained a fidelity of 76.3% in the swapping test.Our results on the coincidence count rates are comparable with the ones ever recorded in teleportation/swaping and multi-photon entanglement generation experiments at around 800\u2009nm wavelengths. Our setup opens the way to practical implementation of device-independent quantum key distribution and its distance extension by the entanglement swapping as well as multi-photon entangled state generation in telecom band infrastructures with both space and fiber links.

Efficient generation and detection of indistinguishable twin photons are at the core of quantum information and communications technology (Q-ICT). These photons are conventionally generated by spontaneous parametric down conversion (SPDC), which is a probabilistic process, and hence occurs at a limited rate, which restricts wider applications of Q-ICT. To increase the rate, one had to excite SPDC by higher pump power, while it inevitably produced more unwanted multi-photon components, harmfully degrading quantum interference visibility.Here we solve this problem by using recently developed 10 GHz repetition-rate-tunable comb laser, combined with a group-velocity-matched nonlinear crystal, and superconducting nanowire single photon detectors. They operate at telecom wavelengths more efficiently with less noises than conventional schemes, those typically operate at visible and near infrared wavelengths generated by a 76 MHz Ti Sapphire laser and detected by Si detectors. We could show high interference visibilities, which are free from the pump-power induced degradation. Our laser, nonlinear crystal, and detectors constitute a powerful tool box, which will pave a way to implementing quantum photonics circuits with variety of good and low-cost telecom components, and will eventually realize scalable Q-ICT in optical infra-structures.

We demonstrate pulsed polarization-entangled photons generated from a periodically poled $\mathrm{KTiOPO_4}$ (PPKTP) crystal in a Sagnac interferometer configuration at telecom wavelength. Since the group-velocity-matching (GVM) condition is satisfied, the intrinsic spectral purity of the photons is much higher than in the previous scheme at around 800 nm wavelength. The combination of a Sagnac interferometer and the GVM-PPKTP crystal makes our entangled source compact, stable, highly entangled, spectrally pure and ultra-bright. The photons were detected by two superconducting nanowire single photon detectors (SNSPDs) with detection efficiencies of 70% and 68% at dark counts of less than 1 kcps. We achieved fidelities of 0.981 $\pm$ 0.0002 for $\left| {\psi ^ -} \right\rangle$ and 0.980 $\pm$ 0.001 for $\left| {\psi ^ +} \right\rangle$ respectively. This GVM-PPKTP-Sagnac scheme is directly applicable to quantum communication experiments at telecom wavelength, especially in free space.

We investigate the detection of an ultra-bright single-photon source using highly efficient superconducting nanowire single-photon detectors (SNSPDs) at telecom wavelengths. Both the single-photon source and the detectors are characterized in detail. At a pump power of 100 mW (400 mW), the measured coincidence counts can achieve 400 kcps (1.17 Mcps), which is the highest ever reported at telecom wavelengths to the best of our knowledge. The multi-pair contributions at different pump powers are analyzed in detail. We compare the experimental and theoretical second order coherence functions $g^{(2)}(0)$ and find that the conventional experimentally measured $g^{(2)}(0)$ values are smaller than the theoretically expected ones. We also consider the saturation property of SNSPD and find that SNSPD can be easier to saturate with a thermal state rather than with a coherent state. The experimental data and theoretical analysis should be useful for the future experiments to detect ultra-bright down-conversion sources with high-efficiency detectors.

We theoretically and experimentally investigate the spectral tunability and purity of photon pairs generated from spontaneous parametric down conversion in periodically poled $\mathrm{KTiOPO_4}$ crystal with group-velocity matching condition. The numerical simulation predicts that the purity of joint spectral intensity ($P_{JSI}$) and the purity of joint spectral amplitude ($P_{JSA}$) can be kept higher than 0.98 and 0.81, respectively, when the wavelength is tuned from 1460 nm to 1675 nm, which covers the S-, C-, L-, and U-band in telecommunication wavelengths. We also directly measured the joint spectral intensity at 1565 nm, 1584 nm and 1565 nm, yielding $P_{JSI}$ of 0.989, 0.983 and 0.958, respectively. Such a photon source is useful for quantum information and communication systems.

We demonstrate a Hong-Ou-Mandel interference between two independent, intrinsically pure, heralded single photons from spontaneous parametric down conversion (SPDC) at telecom wavelength. A visibility of $85.5\pm8.3%$ was achieved without using any bandpass filter. Thanks to the group-velocity-matched SPDC and superconducting nanowire single photon detectors (SNSPDs), the 4-fold coincidence counts are one order higher than that in the previous experiments. The combination of bright single photon sources and SNSPDs is a crucial step for future practical quantum info-communication systems at telecom wavelength.

We report on the experimental generation of an entangled state with a spectrally pure heralded single-photon state and a weak coherent state. By choosing group-velocity matching in the nonlinear crystal, our system for producing entangled photons was 60 times brighter than that in the earlier experiment [Phys. Rev. Lett. 90, 240401 (2003)], with no need of bandpass filters. This entanglement system is useful for quantum information protocols that require indistinguishable photons from independent sources.

We propose a new quantum network scheme using orbital angular momentum states of photons to route the network and spin angular momentum states to encode the information. A four-user experimental scheme based on this efficient quantum network is analyzed in detail, which is particularly appealing for the free space quantum key distribution. Users can freely exchange quantum keys with each other.

We present an experiment of nonclassical interference between a pure heralded single-photon state and a weak coherent state. Our experiment is the first to demonstrate that spectrally pure single photons can have high interference visibility, 89.4 \pm 0.5%, with weak coherent photons. Our scheme lays the groundwork for future experiments requiring quantum interference between photons in nonclassical states and those in coherent states.