Utilizing nonlinear interferometers for sensing with undetected light enables new sensing and imaging techniques in spectral ranges that are difficult to detect. To enhance this method for future applications, it is advantageous to extract both amplitude and phase information of an object. This study introduces two approaches for synthetic quantum holography with undetected light, which allows for obtaining an object's amplitude and phase information in a nonlinear interferometer by capturing only a single image. One method is based on quasi-phase-shifting holography using superpixel structures displayed on a spatial light modulator. The other method relies on synthetic off-axis holography implemented through a linear phase gradient on a spatial light modulator. Both approaches are experimentally analyzed for applicability and compared against available multi-acquisition methods.
O. Anton, I. Bröckel, D. Derr, A. Fieguth, M. Franzke, M. Gärtner, E. Giese, J. S. Haase, J. Hamann, A. Heidt, S. Kanthak, C. Klempt, J. Kruse, M. Krutzik, S. Kubitza, C. Lotz, K. Müller, J. Pahl, E. M. Rasel, M. Schiemangk, et al (4) The INTENTAS project aims to develop an atomic sensor utilizing entangled Bose-Einstein condensates (BECs) in a microgravity environment. This key achievement is necessary to advance the capability for measurements that benefit from both entanglement-enhanced sensitivities and extended interrogation times. The project addresses significant challenges related to size, weight, and power management (SWaP) specific to the experimental platform at the Einstein-Elevator in Hannover. The design ensures a low-noise environment essential for the creation and detection of entanglement. Additionally, the apparatus features an innovative approach to the all-optical creation of BECs, providing a flexible system for various configurations and meeting the requirements for rapid turnaround times. Successful demonstration of this technology in the Einstein-Elevator will pave the way for a future deployment in space, where its potential applications will unlock high-precision quantum sensing.
If the quantum mechanical recoil of the electron due to its scattering from the undulator and laser fields dominates the dynamics, a regime of the free-electron laser emerges where quantum effects lead to a drastic change in the radiation properties. However, the large interaction length required for a single-pass quantum free-electron laser impedes the experimental realization. The quantum free-electron laser oscillator, proposed in the present article, is a possible scheme to resolve this issue. Here we show that this device features a photon statistics that is closer to a coherent state in comparison to existing classical free-electron lasers. The device can be even operated in such a way that a sub-Poissonian statistics is obtained. Beside the benefit of demonstrating this pure quantum effect, the narrowing of the photon distribution implies reduced intensity fluctuations of the emitted radiation, which in turn lead to decreased noise in imaging experiments or to an enhanced sensitivity in interferometric applications.
What time does a clock tell after quantum tunneling? Predictions and indirect measurements range from superluminal or instantaneous tunneling to finite durations, depending on the specific experiment and the precise definition of the elapsed time. Proposals and implementations utilize the atomic motion to define this delay, even though the inherent quantum nature of atoms implies a delocalization and is in sharp contrast to classical trajectories. Here, we rely on an operational approach: we prepare atoms in a coherent superposition of internal states and study the time read off via a Ramsey sequence after the tunneling process without the notion of classical trajectories or velocities. Our operational framework (a) unifies definitions of tunneling delay within one approach; (b) connects the time to a frequency standard given by a conventional atomic clock which can be boosted by differential light shifts; and (c) highlights that there exists no superluminal or instantaneous tunneling.
Jason R. Williams, Charles A. Sackett, Holger Ahlers, David C. Aveline, Patrick Boegel, Sofia Botsi, Eric Charron, Ethan R. Elliott, Naceur Gaaloul, Enno Giese, Waldemar Herr, James R. Kellogg, James M. Kohel, Norman E. Lay, Matthias Meister, Gabriel Müller, Holger Müller, Kamal Oudrhiri, Leah Phillips, Annie Pichery, et al (9) Ultracold atomic gases hold unique promise for space science by capitalizing on quantum advantages and extended freefall, afforded in a microgravity environment, to enable next-generation precision sensors. Atom interferometers are a class of quantum sensors which can use freely falling gases of atoms cooled to sub-photon-recoil temperatures to provide unprecedented sensitivities to accelerations, rotations, and gravitational forces, and are currently being developed for space-based applications in gravitational, earth, and planetary sciences, as well as to search for subtle forces that could signify physics beyond General Relativity and the Standard Model. NASA's Cold Atom Lab (CAL) operates onboard the International Space Station as a multi-user facility for studies of ultracold atoms and to mature quantum technologies, including atom interferometry, in persistent microgravity. In this paper, we report on path-finding experiments utilizing ultracold $^{87}$Rb atoms in the CAL atom interferometer, which was enabled by an on-orbit upgrade of the CAL science module: A three-pulse Mach-Zehnder interferometer was studied to understand limitations from the influence of ISS vibrations. Additionally, Ramsey shear-wave interferometry was used to manifest interference patterns in a single run that were observable for over 150 ms free-expansion time. Finally, the CAL atom interferometer was used to remotely measure the photon recoil from the atom interferometer laser as a demonstration of the first quantum sensor using matter-wave interferometry in space.
The Space Time Explorer and QUantum Equivalence principle Space Test (STE-QUEST) recently proposed, aims at performing a precision test of the weak equivalence principle (WEP), a fundamental cornerstone of General Relativity. Taking advantage of the ideal operation conditions for high-precision quantum sensing on board of a satellite, it aims to detect possible violations of WEP down to the $10^{-17}$ level. This level of performance leads to stringent environmental requirements on the control of the spacecraft. We assume an operation of a dual-species atom interferometer of rubidium and potassium isotopes in a double-diffraction configuration and derive the constraints to achieve an Eötvös parameter $\eta=10^{-17}$ in statistical and systematic uncertainties. We show that technical heritage of previous satellite missions, such as MICROSCOPE, satisfies the platform requirements to achieve the proposed objectives underlying the technical readiness of the STE-QUEST mission proposal.
Sven Abend, Baptiste Allard, Iván Alonso, John Antoniadis, Henrique Araujo, Gianluigi Arduini, Aidan Arnold, Tobias Aßmann, Nadja Augst, Leonardo Badurina, Antun Balaz, Hannah Banks, Michele Barone, Michele Barsanti, Angelo Bassi, Baptiste Battelier, Charles Baynham, Beaufils Quentin, Aleksandar Belic, Ankit Beniwal, et al (233) This document presents a summary of the 2023 Terrestrial Very-Long-Baseline Atom Interferometry Workshop hosted by CERN. The workshop brought together experts from around the world to discuss the exciting developments in large-scale atom interferometer (AI) prototypes and their potential for detecting ultralight dark matter and gravitational waves. The primary objective of the workshop was to lay the groundwork for an international TVLBAI proto-collaboration. This collaboration aims to unite researchers from different institutions to strategize and secure funding for terrestrial large-scale AI projects. The ultimate goal is to create a roadmap detailing the design and technology choices for one or more km-scale detectors, which will be operational in the mid-2030s. The key sections of this report present the physics case and technical challenges, together with a comprehensive overview of the discussions at the workshop together with the main conclusions.
Single-photon transitions are one of the key technologies for designing and operating very-long-baseline atom interferometers tailored for terrestrial gravitational-wave and dark-matter detection. Since such setups aim at the detection of relativistic and beyond-Standard-Model physics, the analysis of interferometric phases as well as of atomic diffraction must be performed to this precision and including these effects. In contrast, most treatments focused on idealized diffraction so far. Here, we study single-photon transitions, both magnetically-induced and direct ones, in gravity and Standard-Model extensions modeling dark matter as well as Einstein-equivalence-principle violations. We take into account relativistic effects like the coupling of internal to center-of-mass degrees of freedom, induced by the mass defect, as well as the gravitational redshift of the diffracting light pulse. To this end, we also include chirping of the light pulse required by terrestrial setups, as well as its associated modified momentum transfer for single-photon transitions.
Atomic high-precision measurements have become a competitive and essential technique for tests of fundamental physics, the Standard Model, and our theory of gravity. It is therefore self-evident that such measurements call for a consistent relativistic description of atoms that eventually originates from quantum field theories like quantum electrodynamics. Most quantum-metrological approaches even postulate effective field-theoretical treatments to describe a precision enhancement through techniques like squeezing. However, a consistent derivation of interacting atomic quantum gases from an elementary quantum field theory that includes both the internal structure as well as the center of mass of atoms, has not yet been addressed. We present such a subspace effective field theory for interacting, spin carrying, and possibly charged ensembles of atoms composed of nucleus and electron that form composite bosons called cobosons, where the interaction with light is included in a multipolar description. Relativistic corrections to the energy of a single coboson, light-matter interaction, and the scattering potential between cobosons arise in a consistent and natural manner. In particular, we obtain a relativistic coupling between the coboson's center-of-mass motion and internal structure encoded by the mass defect. We use these results to derive modified bound-state energies, including the motion of ions, modified scattering potentials, a relativistic extension of the Gross-Pitaevskii equation, and the mass defect applicable to atomic clocks or quantum clock interferometry.
Holger Ahlers, Leonardo Badurina, Angelo Bassi, Baptiste Battelier, Quentin Beaufils, Kai Bongs, Philippe Bouyer, Claus Braxmaier, Oliver Buchmueller, Matteo Carlesso, Eric Charron, Maria Luisa Chiofalo, Robin Corgier, Sandro Donadi, Fabien Droz, Robert Ecoffet, John Ellis, Frédéric Estève, Naceur Gaaloul, Domenico Gerardi, et al (33) An M-class mission proposal in response to the 2021 call in ESA's science programme with a broad range of objectives in fundamental physics, which include testing the Equivalence Principle and Lorentz Invariance, searching for Ultralight Dark Matter and probing Quantum Mechanics.
We examine the prospects of utilizing matter-wave Fabry-Pérot interferometers for enhanced inertial sensing applications. Our study explores such tunneling-based sensors for the measurement of accelerations in two configurations: (a) a transmission setup, where the initial wave packet is transmitted through the cavity and (b) an out-tunneling scheme with intra-cavity generated initial states lacking a classical counterpart. We perform numerical simulations of the complete dynamics of the quantum wave packet, investigate the tunneling through a matter-wave cavity formed by realistic optical potentials and determine the impact of interactions between atoms. As a consequence we estimate the prospective sensitivities to inertial forces for both proposed configurations and show their feasibility for serving as inertial sensors.
Metric descriptions of gravitation, among them general relativity as today's established theory, are founded on assumptions summarized by the Einstein equivalence principle (EEP). Its violation would hint at unknown physics and could be a leverage for the development of quantum gravity. Atomic clocks are excellent systems to probe aspects of EEP connected to (proper) time and have evolved into a working horse for tests of local position invariance (LPI). Even though the operational definition of time requires localized and idealized clocks, quantum systems like atoms allow for spatial superpositions that are inherently delocalized. While quantum experiments have tested other aspects of EEP, no competitive test of LPI has been performed or proposed allowing for an intrinsic delocalization. We extend the concepts for tests of the universality of clock rates (one facet of LPI) to atom interferometry generating delocalized quantum clocks. The proposed test depends on proper time with a favorable scaling and is, in contrast to fountain clocks, robust against initial conditions and recoil effects. It enables optical frequencies so that the projected sensitivity exceeds the one of state-of-the-art localized clocks. These results extend our notion of time, detached from classical and localized philosophies.
We present a detailed study of the effects of imperfect atom-optical manipulation in Bragg-based light-pulse atom interferometers. Off-resonant higher-order diffraction leads to population loss, spurious interferometer paths, and diffraction phases. In a path-dependent formalism, we study numerically various effects and analyze the interference signal caused by an external phase or gravity. We compare first-order single and double Bragg diffraction in retroreflective setups. In double Bragg diffraction, phase imperfections lead to a beating due to three-path interference. Some effects of diffraction phases can be avoided by adding the population of the outer exit ports of double diffraction.
The analogs of optical elements in light-pulse atom interferometers are generated from the interaction of matter waves with light fields. As such, these fields possess quantum properties, which fundamentally lead to a reduced visibility in the observed interference. This loss is a consequence of the encoded information about the atom's path. However, the quantum nature of the atom-optical elements also gives an additional degree of freedom to reduce such effects: We demonstrate that entanglement between all light fields can be used to erase information about the atom's path and by that to partially recover the visibility. Thus, our work highlights the role of complementarity on atom-interferometric experiments.
The far-field patterns of atoms diffracted from a classical light field, or from a quantum one in a photon-number state are identical. On the other hand, diffraction from a field in a coherent state, which shares many properties with classical light, displays a completely different behavior. We show that in contrast to the diffraction patterns, the interference signal of an atom interferometer with light-pulse beam splitters and mirrors in intense coherent states does approach the limit of classical fields. However, low photon numbers reveal the granular structure of light, leading to a reduced visibility since Welcher-Weg (which-way) information is encoded into the field. We discuss this effect for a single photon-number state as well as a superposition of two such states.
Atomic interference experiments can probe the gravitational redshift via the internal energy splitting of atoms and thus give direct access to test the universality of the coupling between matter-energy and gravity at different spacetime points. By including possible violations of the equivalence principle in a fully quantized treatment of all degrees of freedom, we characterize how the sensitivity to gravitational redshift violations arises in atomic clocks and atom interferometers, as well as their underlying limitations. Specifically, we show that: (i.) Contributions beyond linear order to trapping potentials lead to such a sensitivity of trapped atomic clocks. (ii.) While Bragg-type interferometers, even with a superposition of internal states, with state-independent, linear interaction potentials are at first insensitive to gravitational redshift tests, modified configurations, for example by relaunching the atoms, can mimic such tests tests under certain conditions. (iii.) Guided atom interferometers are comparable to atomic clocks. (iv.) Internal transitions lead to state-dependent interaction potentials through which light-pulse atom interferometers can become sensitive to gravitational redshift violations.
We solve the long-time dynamics of a high-gain free-electron laser in the quantum regime. In this regime each electron emits at most one photon on average, independently of the initial field. In contrast, the variance of the photon statistics shows a qualitatively different behavior for different initial states of the field. We find that the realization of a seeded Quantum FEL is more feasible than self-amplified spontaneous emission.
In a retroreflective scheme atomic Raman diffraction adopts some of the properties of Bragg diffraction due to additional couplings to off-resonant momenta. As a consequence, double Raman diffraction has to be performed in a Bragg-type regime. Taking advantage of this regime, double Raman allows for resonant higher-order diffraction. We study theoretically the case of third-order diffraction and compare it to first order as well as a sequence of first-order pulses giving rise to the same momentum transfer as the third-order pulse. In fact, third-order diffraction constitutes a competitive tool for the diffraction of ultracold atoms and interferometry based on large momentum transfer since it allows to reduce the complexity of the experiment as well as the total duration of the diffraction process compared to a sequence.
Light-pulse atom interferometers constitute powerful quantum sensors for inertial forces. They are based on delocalised spatial superpositions and the combination with internal transitions directly links them to atomic clocks. Since classical tests of the gravitational redshift are based on a comparison of two clocks localised at different positions under gravity, it is promising to explore whether the aforementioned interferometers constitute a competitive alternative for tests of general relativity. Here we present a specific geometry which together with state transitions leads to a scheme that is concurrently sensitive to both violations of the universality of free fall and gravitational redshift, two premises of general relativity. The proposed interferometer does not rely on a superposition of internal states, but merely on transitions between them, and therefore generalises the concept of physical atomic clocks and quantum-clock interferometry. An experimental realisation seems feasible with already demonstrated techniques in state-of-the-art facilities.
In a quantum mechanical description of the free-electron laser (FEL) the electrons jump on discrete momentum ladders, while they follow continuous trajectories according to the classical description. In order to observe the transition from quantum to classical dynamics, it is not sufficient that many momentum levels are involved. Only if additionally the initial momentum spread of the electron beam is larger than the quantum mechanical recoil, caused by the emission and absorption of photons, the quantum dynamics in phase space resembles the classical one. Beyond these criteria, quantum signatures of averaged quantities like the FEL gain might be washed out.
We provide a comprehensive study of atomic Raman and Bragg diffraction when coupling to a pair of counterpropagating light gratings (double diffraction) or to a single one (single diffraction) and discuss the transition from one case to the other in a retroreflective geometry as the Doppler detuning changes. In contrast to single diffraction, double Raman loses its advantage of high diffraction efficiency for short pulses and has to be performed in a Bragg-type regime. Moreover, the structure of double diffraction leads to further limitations for broad momentum distributions on the efficiency of mirror pulses, making the use of (ultra) cold ensembles essential for high diffraction efficiency.
Phase distortions, or aberrations, can negatively influence the performance of an optical imaging system. Through the use of position-momentum entangled photons, we nonlocally correct for aberrations in one photon's optical path by intentionally introducing the complementary aberrations in the optical path of the other photon. In particular, we demonstrate the simultaneous nonlocal cancellation of aberrations that are of both even and odd order in the photons' transverse degrees of freedom. We also demonstrate a potential application of this technique by nonlocally cancelling the effect of defocus in a quantum imaging experiment and thereby recover the original spatial resolution.
We derive an effective Dicke model in momentum space to describe collective effects in the quantum regime of a free-electron laser (FEL). The resulting exponential gain from a single passage of electrons allows the operation of a Quantum FEL in the high-gain mode and avoids the experimental challenges of an X-ray FEL oscillator. Moreover, we study the intensity fluctuations of the emitted radiation which turn out to be super-Poissonian.
Sina Loriani, Alexander Friedrich, Christian Ufrecht, Fabio Di Pumpo, Stephan Kleinert, Sven Abend, Naceur Gaaloul, Christian Meiners, Christian Schubert, Dorothee Tell, Étienne Wodey, Magdalena Zych, Wolfgang Ertmer, Albert Roura, Dennis Schlippert, Wolfgang P. Schleich, Ernst M. Rasel, Enno Giese The phase of matter waves depends on proper time and is therefore susceptible to special-relativistic (kinematic) and gravitational (redshift) time dilation. Hence, it is conceivable that atom interferometers measure general-relativistic time-dilation effects. In contrast to this intuition, we show: (i.) Closed light-pulse interferometers without clock transitions during the pulse sequence are not sensitive to gravitational time dilation in a linear potential. (ii.) They can constitute a quantum version of the special-relativistic twin paradox. (iii.) Our proposed experimental geometry for a quantum-clock interferometer isolates this effect.
High-dimensional encoding schemes have emerged as a novel way to perform quantum information tasks. For high dimensionality, temporal and transverse spatial modes of photons are the two paradigmatic degrees of freedom commonly used in such experiments. Nevertheless, general devices for multi-outcome measurements are still needed to take full advantage of the high-dimensional nature of encoding schemes. We propose a general full-field mode sorting scheme consisting only of up to two optimized phase elements based on evolutionary algorithms that allows for joint sorting of azimuthal and radial modes in a wide range of bases. We further study the performance of our scheme through simulations in the context of high-dimensional quantum cryptography, where high-fidelity measurement schemes are crucial.
Scattering processes have played a crucial role in the development of quantum theory. In the field of optics, scattering phase shifts have been utilized to unveil interesting forms of light-matter interactions. Here, we investigate the mode-coupling phase of single photons to surface plasmon polaritons in a quantum plasmonic tritter. We observe that the coupling process induces a phase jump that occurs when photons scatter into surface plasmons and vice versa. This interesting coupling phase dynamics is of particular relevance for quantum plasmonic experiments. Furthermore, it is demonstrated that this photon-plasmon interaction can be modeled through a quantum-mechanical tritter. We show that the visibility of a double-slit and a triple-slit interference patterns are convenient observables to characterize the interaction at a slit and determine the coupling phase. Our accurate and simple model of the interaction, validated by simulations and experiments, has important implications not only for quantum plasmonic interference effects, but is also advantageous to classical applications.
We compare a conventional Mach-Zehnder light-pulse atom interferometer based on diffractive mirrors with one that uses specular reflection. In contrast to diffractive mirrors that generate a symmetric configuration, specular mirrors realized, for example, by evanescent fields lead under the influence of gravity to an asymmetric geometry. In such an arrangement the interferometer phase contains nonrelativistic signatures of proper time.
The phase uncertainty of an unseeded nonlinear interferometer, where the output of one nonlinear crystal is transmitted to the input of a second crystal that analyzes it, is commonly said to be below the shot-noise level but highly dependent on detection and internal loss. Unbalancing the gains of the first (source) and second (analyzer) crystals leads to a configuration that is tolerant against detection loss. However, in terms of sensitivity, there is no advantage in choosing a stronger analyzer over a stronger source, and hence the comparison to a shot-noise level is not straightforward. Internal loss breaks this symmetry and shows that it is crucial whether the source or analyzer is dominating. Based on these results, claiming a Heisenberg scaling of the sensitivity is more subtle than in a balanced setup.
Induced coherence in parametric down-conversion between two coherently pumped nonlinear crystals that share a common idler mode can be used as an imaging technique. Based on the interference between the two signal modes of the crystals, an image can be reconstructed. By obtaining an expression for the interference pattern that is valid in both the low- and the high-gain regimes of parametric down-conversion, we show how the coherence of the light emitted by the two crystals can be controlled. With our comprehensive analysis we provide deeper insight into recent discussions about the application of induced coherence to imaging in different regimes. Moreover, we propose a scheme for optimizing the visibility of the interference pattern so that it directly corresponds to the degree of coherence of the light generated in the two crystals. We find that this scheme leads in the high-gain regime to a visibility arbitrarily close to unity.
We show that standard approximations in nonlinear optics are violated for situations involving a small value of the linear refractive index. Consequently, the conventional equation for the intensity-dependent refractive index, $n(I) = n_0 + n_2 I$, becomes inapplicable in epsilon-near-zero and low-index media, even in the presence of only third-order effects. For the particular case of indium tin oxide, we find that the $\chi^{(3)}$, $\chi^{(5)}$ and $\chi^{(7)}$ contributions to refraction eclipse the linear term; thus, the nonlinear response can no longer be interpreted as a perturbation in these materials. Although the response is non-perturbative, we find no evidence that the power series expansion of the material polarization diverges.
Bragg diffraction of an atomic wave packet in a retroreflective geometry with two counterpropagating optical lattices exhibits a light shift induced phase. We show that the temporal shape of the light pulse determines the behavior of this phase shift: In contrast to Raman diffraction, Bragg diffraction with Gaussian pulses leads to a significant suppression of the intrinsic phase shift due to a scaling with the third power of the inverse Doppler frequency. However, for box-shaped laser pulses, the corresponding shift is twice as large as for Raman diffraction. Our results are based on approximate, but analytical expressions as well as a numerical integration of the corresponding Schrödinger equation.
We provide an introduction into the formulation of non-relativistic quantum mechanics using the Wigner phase-space distribution function and apply this concept to two physical situations at the interface of quantum theory and general relativity: (i) the motion of an ensemble of cold atoms relevant to tests of the weak equivalence principle, and (ii) the Kasevich-Chu interferometer. In order to lay the foundations for this analysis we first present a representation-free description of the Kasevich-Chu interferometer based on unitary operators.
The use of retro-reflection in light-pulse atom interferometry under microgravity conditions naturally leads to a double-diffraction scheme. The two pairs of counterpropagating beams induce simultaneously transitions with opposite momentum transfer that, when acting on atoms initially at rest, give rise to symmetric interferometer configurations where the total momentum transfer is automatically doubled and where a number of noise sources and systematic effects cancel out. Here we extend earlier implementations for Raman transitions to the case of Bragg diffraction. In contrast with the single-diffraction case, the existence of additional off-resonant transitions between resonantly connected states precludes the use of the adiabatic elimination technique. Nevertheless, we have been able to obtain analytic results even beyond the deep Bragg regime by employing the so-called "method of averaging," which can be applied to more general situations of this kind. Our results have been validated by comparison to numerical solutions of the basic equations describing the double-diffraction process.
H. Müntinga, H. Ahlers, M. Krutzik, A. Wenzlawski, S. Arnold, D. Becker, K. Bongs, H. Dittus, H. Duncker, N. Gaaloul, C. Gherasim, E. Giese, C. Grzeschik, T. W. Hänsch, O. Hellmig, W. Herr, S. Herrmann, E. Kajari, S. Kleinert, C. Lämmerzahl, et al (24) Atom interferometers covering macroscopic domains of space-time are a spectacular manifestation of the wave nature of matter. Due to their unique coherence properties, Bose-Einstein condensates are ideal sources for an atom interferometer in extended free fall. In this paper we report on the realization of an asymmetric Mach-Zehnder interferometer operated with a Bose-Einstein condensate in microgravity. The resulting interference pattern is similar to the one in the far-field of a double-slit and shows a linear scaling with the time the wave packets expand. We employ delta-kick cooling in order to enhance the signal and extend our atom interferometer. Our experiments demonstrate the high potential of interferometers operated with quantum gases for probing the fundamental concepts of quantum mechanics and general relativity.
Braneshop, and
the US National Science Foundation.
SciRate