The ability to discover new materials with desirable properties is critical for numerous applications from helping mitigate climate change to advances in next generation computing hardware. AI has the potential to accelerate materials discovery and design by more effectively exploring the chemical space compared to other computational methods or by trial-and-error. While substantial progress has been made on AI for materials data, benchmarks, and models, a barrier that has emerged is the lack of publicly available training data and open pre-trained models. To address this, we present a Meta FAIR release of the Open Materials 2024 (OMat24) large-scale open dataset and an accompanying set of pre-trained models. OMat24 contains over 110 million density functional theory (DFT) calculations focused on structural and compositional diversity. Our EquiformerV2 models achieve state-of-the-art performance on the Matbench Discovery leaderboard and are capable of predicting ground-state stability and formation energies to an F1 score above 0.9 and an accuracy of 20 meV/atom, respectively. We explore the impact of model size, auxiliary denoising objectives, and fine-tuning on performance across a range of datasets including OMat24, MPtraj, and Alexandria. The open release of the OMat24 dataset and models enables the research community to build upon our efforts and drive further advancements in AI-assisted materials science.
Autonomous implantable bioelectronics rely on wireless connectivity, necessitating highly efficient electromagnetic (EM) radiation systems. However, limitations in power, safety, and data transmission currently impede the advancement of innovative wireless medical devices, such as tetherless neural interfaces, electroceuticals, and surgical microrobots. To overcome these challenges and ensure sufficient link and power budgets for wireless implantable systems, this study explores the mechanisms behind EM radiation and losses, offering strategies to enhance radiation efficiency in wireless implantable bioelectronics. Using analytical modeling, the EM waves emitted by the implant are expanded as a series of spherical harmonics, enabling a detailed analysis of the radiation mechanisms. This framework is then extended to approximate absorption losses caused by the lossy and dispersive properties of tissues through derived analytical expressions. The radiation efficiency and in-body path loss are quantified and compared in terms of three primary loss mechanisms. The impact of various parameters on the EM efficiency of implantable devices is analyzed and quantified, including operating frequency, implant size, body-air interface curvature, and implantation location. Additionally, a rapid estimation technique is introduced to determine the optimal operating frequency for specific scenarios, along with a set of design principles aimed at improving radiation performance. The design strategies derived in this work - validated through numerical and experimental demonstrations on realistic implants - reveal a potential improvement in implant radiation efficiency or gain by a factor of five to ten, leading to a corresponding increase in overall link efficiency compared to conventional designs.
Entanglement entropy characterizes the correlation of multi-particles and unveils the crucial features of open quantum systems. However, the experimental realization of exploring entanglement in non-Hermitian systems remains a challenge. In parallel, quantum walks have offered the possibility of studying the underlying mechanisms of non-Hermitian physics, which includes exceptional points, the non-Hermitian skin effect, and non-Bloch phase transitions. Unfortunately, these studies have only involved and prevailingly focused on the behavior of a single particle. Here, we propose and experimentally realize quantum walks of two indistinguishable photons in engineered non-Hermitian photonic lattices. We have successfully observed the unidirectional behavior of quantum walks in the bulk far from the edges induced by the skin effect. Moreover, we experimentally reveal the suppression of entanglement that is caused by the skin effect in non-Hermitian systems. Our study may facilitate a deep understanding of entanglement in open quantum many-body systems that are far from thermal equilibrium.
On-chip micro-ring resonators (MRRs) have been proposed for constructing delay reservoir computing (RC) systems, offering a highly scalable, high-density computational architecture that is easy to manufacture. However, most proposed RC schemes have utilized passive integrated optical components based on silicon-on-insulator (SOI), and RC systems based on lithium niobate on insulator (LNOI) have not yet been reported. The nonlinear optical effects exhibited by lithium niobate microphotonic devices introduce new possibilities for RC design. In this work, we design an RC scheme based on a series-coupled MRR array, leveraging the unique interplay between thermo-optic nonlinearity and photorefractive effects in lithium niobate. We first demonstrate the existence of three regions defined by wavelength detuning between the primary LNOI micro-ring resonator and the coupled micro-ring array, where one region achieves an optimal balance between nonlinearity and high memory capacity at extremely low input energy, leading to superior computational performance. We then discuss in detail the impact of each ring's nonlinearity and the system's symbol duration on performance. Finally, we design a wavelength-division multiplexing (WDM) based multi-task parallel computing scheme, showing that the computational performance for multiple tasks matches that of single-task computations.
Meng-Yu Xie, Su-Jian Niu, Zhao-Qi-Zhi Han, Yin-Hai Li, Ren-Hui Chen, Xiao-Hua Wang, Ming-Yuan Gao, Li Chen, Yue-Wei Song, Zhi-Yuan Zhou, Bao-Sen Shi Polarimetric imaging, a technique that captures the invisible polarization-related properties of given materials, has broad applications from fundamental physics to advanced fields such as target recognition, stress detection, biomedical diagnosis and remote sensing. The introduction of quantum sources into classical imaging systems has demonstrated distinct advantages, yet few studies have explored their combination with polarimetric imaging. In this study, we present a quantum polarimetric imaging system that integrates polarization-entangled photon pairs into a polarizer-sample-compensator-analyzer (PSRA)-type polarimeter. Our system visualizes the birefringence properties of a periodical-distributed anisotropic material under decreasing illumination levels and diverse disturbing light sources. Compared to the classical system, the quantum approach reveals the superior sensitivity and robustness in low-light conditions, particularly useful in biomedical studies where the low illumination and non-destructive detection are urgently needed. The study also highlights the nonlocality of entangled photons in birefringence measurement, indicating the potential of quantum polarimetric system in the remote sensing domain.
Direct numerical simulations (DNS) of microscale fluid-structure interactions (mFSI) in multicomponent multiphase flows pose many challenges such as the thermodynamic consistency of multiphysics couplings, the tracking of moving interfaces, and the dynamics of moving triple-phase contact lines. We propose and validate a generic DNS approach: Diffuse-Resistance-Domain (DRD). It overcomes the above challenges by employing Onsager's principle to formulate dynamic models and combining traditional diffuse-interface models for fluid-fluid interfacial dynamics with a novel implementation of complex fluid-solid interfacial conditions via smooth interpolations of dynamic-resistance coefficients across interfaces. After careful validation by benchmark simulations, we simulated three challenging mFSI problems taken from different fields.
An innovative method is developed for accurate determination of thermodynamic properties as a function of temperature by revisiting the density functional theory (DFT) based quasiharmonic approach (QHA). The present methodology individually evaluates the contributions from static total energy, phonon, and thermal electron to free energy for increased efficiency and accuracy. The Akaike information criterion with a correction (AICc) is used to select models and model parameters for fitting each contribution as a function of volume. Using the additively manufactured Inconel alloy 625 (IN625) as an example, predicted temperature-dependent linear coefficient of thermal expansion (CTE) agrees well with dilatometer measurements and values in the literature. Sensitivity and uncertainty are also analyzed for the predicted IN625 CTE due to different structural configurations used by DFT, and hence different equilibrium properties determined.
Shanshan Shan, Yang Gao, David E. J. Waddington, Hongli Chen, Brendan Whelan, Paul Z. Y. Liu, Yaohui Wang, Chunyi Liu, Hongping Gan, Mingyuan Gao, Feng Liu MRI-Linac systems require fast image reconstruction with high geometric fidelity to localize and track tumours for radiotherapy treatments. However, B0 field inhomogeneity distortions and slow MR acquisition potentially limit the quality of the image guidance and tumour treatments. In this study, we develop an interpretable unrolled network, referred to as RebinNet, to reconstruct distortion-free images from B0 inhomogeneity-corrupted k-space for fast MRI-guided radiotherapy applications. RebinNet includes convolutional neural network (CNN) blocks to perform image regularizations and nonuniform fast Fourier Transform (NUFFT) modules to incorporate B0 inhomogeneity information. The RebinNet was trained on a publicly available MR dataset from eleven healthy volunteers for both fully sampled and subsampled acquisitions. Grid phantom and human brain images acquired from an open-bore 1T MRI-Linac scanner were used to evaluate the performance of the proposed network. The RebinNet was compared with the conventional regularization algorithm and our recently developed UnUNet method in terms of root mean squared error (RMSE), structural similarity (SSIM), residual distortions, and computation time. Imaging results demonstrated that the RebinNet reconstructed images with lowest RMSE (<0.05) and highest SSIM (>0.92) at four-time acceleration for simulated brain images. The RebinNet could better preserve structural details and substantially improve the computational efficiency (ten-fold faster) compared to the conventional regularization methods, and had better generalization ability than the UnUNet method. The proposed RebinNet can achieve rapid image reconstruction and overcome the B0 inhomogeneity distortions simultaneously, which would facilitate accurate and fast image guidance in radiotherapy treatments.
Li Chen, Zheng Ge, Su-Jian Niu, Yin-Hai Li, Zhao-Qi-Zhi Han, Yue-Wei Song, Wu-Zhen Li, Ren-Hui Chen, Ming-Yuan Gao, Meng-Yu Xie, Zhi-Yuan Zhou, Bao-Sen Shi Four wave mixing (FWM) is an important way to generate supercontinuum and frequency combs in the mid-infrared band. Here, we obtain simultaneous synthetic FWM in the visible and mid-infrared bands by cascading quadratic nonlinear processes in a periodically poled lithium niobate crystal (PPLN), which has a 110dB(at 3000nm) higher conversion efficiency than the FWM directly generated by third-order susceptibilities in bulk PPLN crystals. A general model of this process is developed that is in full agreement with the experimental verifications. The frequency difference between the new frequency components can be freely tuned by changing the frequency difference of the dual pump lasers. Furthermore, by increasing the conversion bandwidth and efficiency of the cascaded processes, it is feasible to generate frequency combs in three bands the visible, near-infrared and mid-infrared bands simultaneously through high-order cascaded processes. This work opens up a new avenue toward free-tuning multiband frequency comb generation with multi-octaves frequency spanning, which will have significant applications in fields such as mid-infrared gas sensing, lidar and precision spectroscopy.
Entanglement enables many promising applications in quantum technology. Devising new generation methods and harnessing entanglement are prerequisites for practical applications. Here we realize a distinct polarization-entangled source by simultaneously achieving type-0 and type-I backward quasi-phase matching (BQPM) through spontaneous parametric down-conversion in a single bulk crystal, which is different from all previous entangled-source configurations. Pumping the crystal with a single polarized beam generates a non-maximally polarization-entangled state, which can be further projected to a maximal Bell state with a pair of Brewster windows. Hong-Ou-Mandel interference experiments are done on polarization-degenerate photon pairs for both type-0 and type-I BQPM processes for the first time. The emitted photons in both processes have a bandwidth as narrow as 15.7 GHz. The high quality of this source is characterized by various methods. The rather simple configuration, narrow bandwidth, and high entanglement quality make the source very promising for many quantum information tasks.
An ellipsometer is a vital precision tool used for measuring optical parameters with wide applications in many fields, including accurate measurements in film thickness, optical constants, structural profiles, etc. However, the precise measurement of photosensitive materials meets huge obstacles because of the excessive input photons, therefore the requirement of enhancing detection accuracy under low incident light intensity is an essential topic in the precision measurement. In this work, by combining a polarization-entangled photon source with a classical transmission-type ellipsometer, the quantum ellipsometer with the PSA (Polarizer-Sample-Analyzer) and the Senarmount method is constructed firstly to measure the phase retardation of the birefringent materials. The experimental results show that the accuracy can reach to nanometer scale at extremely low input intensity, and the stability are within 1% for all specimens tested with a compensator involved. Our work paves the way for precision measurement at low incident light intensity, with potential applications in measuring photosensitive materials, active-biological samples and other remote monitoring scenarios.
Pei-Yi Feng, Zheng-Hua An, Da-Li Zhang, Chen-Wei Wang, Chao Zheng, Sheng Yang, Shao-Lin Xiong, Jia-Cong Liu, Xin-Qiao Li, Ke Gong, Xiao-Jing Liu, Min Gao, Xiang-Yang Wen, Ya-Qing liu, Xiao-Yun Zhao, Fan Zhang, Xi-Lei Sun, Hong Lu Gamma-ray Transient Monitor (GTM) is an all-sky monitor onboard the Distant Retrograde Orbit-A (DRO-A) satellite with the scientific objective of detecting gamma-ray transients ranging from 20 keV to 1 MeV. GTM is equipped with 5 Gamma-ray Transient Probe (GTP) detector modules, utilizing the NaI(Tl) scintillator coupled with a SiPM array. To reduce the SiPM noise, GTP makes use of a dedicated dual-channel coincident readout design. In this work, we firstly studied the impact of different coincidence times on detection efficiency and ultimately selected the 500 ns time coincidence window for offline data processing. To test the performance of GTPs and validate the Monte Carlo simulated energy response, we conducted comprehensive ground calibration tests using Hard X-ray Calibration Facility (HXCF) and radioactive sources, including energy response, detection efficiency, spatial response, bias-voltage response, and temperature dependence. We extensively presented the ground calibration results, and validated the design and mass model of GTP detector. These work paved the road for the in-flight observation and science data analysis.
Pei-Yi Feng, Xi-Lei Sun, Zheng-Hua An, Yong Deng, Cheng-Er Wang, Huang Jiang, Jun-Jie Li, Da-Li Zhang, Xin-Qiao Li, Shao-Lin Xiong, Chao Zheng, Ke Gong, Sheng Yang, Xiao-Jing Liu, Min Gao, Xiang-Yang Wen, Ya-Qing Liu, Yan-Bing Xu, Xiao-Yun Zhao, Jia-Cong Liu, et al (2) The GECAM series of satellites utilize LaBr3(Ce), LaBr3(Ce,Sr), and NaI(Tl) crystals as sensitive materials for gamma-ray detectors (GRDs). To investigate the non-linearity in the detection of low-energy gamma rays and address errors in the E-C relationship calibration, comprehensive tests and comparative studies of the non-linearity of these three crystals were conducted using Compton electrons, radioactive sources, and mono-energetic X-rays. The non-linearity test results for Compton electrons and X-rays displayed substantial differences, with all three crystals showing higher non-linearity for X-rays and gamma-rays than for Compton electrons. Despite LaBr3(Ce) and LaBr3(Ce,Sr) crystals having higher absolute light yields, they exhibited a noticeable non-linear decrease in light yield, especially at energies below 400 keV. The NaI(Tl) crystal demonstrated excess light output in the 6~200 keV range, reaching a maximum excess of 9.2% at 30 keV in X-ray testing and up to 15.5% at 14 keV during Compton electron testing, indicating a significant advantage in the detection of low-energy gamma rays. Furthermore, this paper explores the underlying causes of the observed non-linearity in these crystals. This study not only elucidates the detector responses of GECAM, but also marks the inaugural comprehensive investigation into the non-linearity of domestically produced lanthanum bromide and sodium iodide crystals.
Implantable wireless bioelectronic devices enable communication and/or power transfer through RF wireless connections with external nodes. These devices encounter notable design challenges due to the lossy nature of the host body, which significantly diminishes the radiation efficiency of the implanted antenna and tightens the wireless link budget. Prior research has yielded closed-form approximate expressions for estimating losses occurring within the lossy host body, known as the in-body path loss. To assess the total path loss between the implanted transmitter and external receiver, this paper focuses on the free-space path loss of the implanted antenna, from the body-air interface to the external node. This is not trivial, as in addition to the inherent radial spreading of spherical electromagnetic waves common to all antennas, implanted antennas confront additional losses arising from electromagnetic scattering at the interface between the host body and air. Employing analytical modeling, we propose closed-form approximate expressions for estimating this free-space path loss. The approximation is formulated as a function of the free-space distance, the curvature radius of the body-air interface, the depth of the implanted antenna, and the permittivity of the lossy medium. This proposed method undergoes thorough validation through numerical calculations, simulations, and measurements for different implanted antenna scenarios. This study contributes to a comprehensive understanding of the path loss in implanted antennas and provides a reliable analytical framework for their efficient design and performance evaluation.
$B_1^+$ and $B_0$ field-inhomogeneities can significantly reduce accuracy and robustness of MRF's quantitative parameter estimates. Additional $B_1^+$ and $B_0$ calibration scans can mitigate this but add scan time and cannot be applied retrospectively to previously collected data. Here, we proposed a calibration-free sequence-adaptive deep-learning framework, to estimate and correct for $B_1^+$ and $B_0$ effects of any MRF sequence. We demonstrate its capability on arbitrary MRF sequences at 3T, where no training data were previously obtained. Such approach can be applied to any previously-acquired and future MRF-scans. The flexibility in directly applying this framework to other quantitative sequences is also highlighted.
The development of X-ray Free Electron Lasers (XFELs) has opened numerous opportunities to probe atomic structure and ultrafast dynamics of various materials. Single Particle Imaging (SPI) with XFELs enables the investigation of biological particles in their natural physiological states with unparalleled temporal resolution, while circumventing the need for cryogenic conditions or crystallization. However, reconstructing real-space structures from reciprocal-space x-ray diffraction data is highly challenging due to the absence of phase and orientation information, which is further complicated by weak scattering signals and considerable fluctuations in the number of photons per pulse. In this work, we present an end-to-end, self-supervised machine learning approach to recover particle orientations and estimate reciprocal space intensities from diffraction images only. Our method demonstrates great robustness under demanding experimental conditions with significantly enhanced reconstruction capabilities compared with conventional algorithms, and signifies a paradigm shift in SPI as currently practiced at XFELs.
This paper presents a method for the fast and accurate estimation of the gain pattern and maximum gain of an implanted antenna including the effect of the host body, under the assumption that the latter is electrically large. The estimation procedure is based on the radiation of an elementary dipole source placed in a planar body model. The derivation of closed-form expressions is based on spherical wave analysis and the Green's functions for layered media. The validity of this approximation for practical cases is shown on different implanted antennas, where the results are compared to full wave simulations and measurements.
S. Fatigoni, P.A.R. Ade, Z. Ahmed, M. Amiri, D. Barkats, R. Basu Thakur, C.A. Bischoff, D. Beck, J.J. Bock, V. Buza, J. Cheshire, J. Connors, J. Cornelison, M. Crumrine, A.J. Cukierman, E.V. Denison, M.I. Dierickx, L. Duband, M. Eiben, J.P. Filippini, et al (67) Time-Division Multiplexing is the readout architecture of choice for many ground and space experiments, as it is a very mature technology with proven outstanding low-frequency noise stability, which represents a central challenge in multiplexing. Once fully populated, each of the two BICEP Array high frequency receivers, observing at 150GHz and 220/270GHz, will have 7776 TES detectors tiled on the focal plane. The constraints set by these two receivers required a redesign of the warm readout electronics. The new version of the standard Multi Channel Electronics, developed and built at the University of British Columbia, is presented here for the first time. BICEP Array operates Time Division Multiplexing readout technology to the limits of its capabilities in terms of multiplexing rate, noise and crosstalk, and applies them in rigorously demanding scientific application requiring extreme noise performance and systematic error control. Future experiments like CMB-S4 plan to use TES bolometers with Time Division/SQUID-based readout for an even larger number of detectors.
Hurricanes present major challenges in the U.S. due to their devastating impacts. Mitigating these risks is important, and the insurance industry is central in this effort, using intricate statistical models for risk assessment. However, these models often neglect key temporal and spatial hurricane patterns and are limited by data scarcity. This study introduces a refined approach combining the ARIMA model and K-MEANS to better capture hurricane trends, and an Autoencoder for enhanced hurricane simulations. Our experiments show that this hybrid methodology effectively simulate historical hurricane behaviors while providing detailed projections of potential future trajectories and intensities. Moreover, by leveraging a comprehensive yet selective dataset, our simulations enrich the current understanding of hurricane patterns and offer actionable insights for risk management strategies.
In this study, we introduce a unique approach that employs time-resolved Schlieren imaging to capture and visualize the dynamic changes of a thin liquid (mixture of water, soap and glycerin) film in ultrasonic wave field with high spatial and temporal resolution. By placing a soap film spanning a wire frame vertically in the path of light, we harnessed the vibrations induced by the ultrasonic waves, resulting in remarkable Schlieren imaging patterns. The investigation not only uncovers an unexpected branch flow phenomenon within the film, challenging existing assumptions, but also reveals a fascinating interplay between vortex flow and branch flow. The experiments have revealed a captivating spectrum of dynamic phenomena within the thin liquid films. The observation of small-scale capillary waves, large-scale standing waves, traveling waves, and the intricate fusion of capillary-gravity wave patterns underscores the rich complexity inherent in the interaction between the films and the holographic ultrasonic wave field. These diverse states of film dynamics provide a comprehensive understanding of the intricate interplay between various wave modes and fluid behavior, further enhancing comprehension of this fascinating phenomenon. The ability to visualize the pressure field opens up new avenues for optimizing acoustic levitation techniques, investigating particle behavior, and exploring potential applications in materials science and bioengineering.
On-chip microring resonators (MRRs) have been proposed to construct the time-delayed reservoir computing (RC), which offers promising configurations available for computation with high scalability, high-density computing, and easy fabrication. A single MRR, however, is inadequate to supply enough memory for the computational task with diverse memory requirements. Large memory needs are met by the MRR with optical feedback waveguide, but at the expense of its large footprint. In the structure, the ultra-long optical feedback waveguide substantially limits the scalable photonic RC integrated designs. In this paper, a time-delayed RC is proposed by utilizing a silicon-based nonlinear MRR in conjunction with an array of linear MRRs. These linear MRRs possess a high quality factor, providing sufficient memory capacity for the entire system. We quantitatively analyze and assess the proposed RC structure's performance on three classical tasks with diverse memory requirements, i.e., the Narma 10, Mackey-Glass, and Santa Fe chaotic timeseries prediction tasks. The proposed system exhibits comparable performance to the MRR with an ultra-long optical feedback waveguide-based system when it comes to handling the Narma 10 task, which requires a significant memory capacity. Nevertheless, the overall length of these linear MRRs is significantly smaller, by three orders of magnitude, compared to the ultra-long feedback waveguide in the MRR with optical feedback waveguide-based system. The compactness of this structure has significant implications for the scalability and seamless integration of photonic RC.
Performance limitations for implanted antennas, taking radiation efficiency as the metric, are presented. The performance limitations use a convex optimization procedure with the current density inside the implant acting as its degree of freedom. The knowledge of the limitations provides useful information in design procedure and physical insight. Ohmic losses in the antenna and surrounding tissue are both considered and quantitatively compared. The interaction of all parts of the system is taken into account in a full-wave manner via the hybrid computation method. The optimization framework is thoroughly tested on a realistic implanted antenna design that is treated both experimentally and as a model in a commercial electromagnetic solver. Good agreement is reported. To demonstrate the feasibility of developed performance limitations, they are compared to the performance of a loop and a dipole antenna showing the importance of various loss mechanisms during the design process. The trade-off between tissue loss and antenna ohmic loss indicates critical points at which the optimal solution drastically changes and the chosen topology for a specific design should be changed.
Stagnant weather condition is one of the major contributors to air pollution as it is favorable for the formation and accumulation of pollutants. To measure the atmosphere's ability to dilute air pollutants, Air Stagnation Index (ASI) has been introduced as an important meteorological index. Therefore, making long-lead ASI forecasts is vital to make plans in advance for air quality management. In this study, we found that autumn Niño indices derived from sea surface temperature (SST) anomalies show a negative correlation with wintertime ASI in southern China, offering prospects for a prewinter forecast. We developed an LSTM-based model to predict the future wintertime ASI. Results demonstrated that multivariate inputs (past ASI and Niño indices) achieve better forecast performance than univariate input (only past ASI). The model achieves a correlation coefficient of 0.778 between the actual and predicted ASI, exhibiting a high degree of consistency.
Ying Gao, Xuekai Ma, Xiaokun Zhai, Chunzi Xing, Meini Gao, Haitao Dai, Hao Wu, Tong Liu, Yuan Ren, Xiao Wang, Anlian Pan, Wei Hu, Stefan Schumacher, Tingge Gao In planar microcavities, the transverse-electric and transverse-magnetic (TE-TM) mode splitting of cavity photons arises due to their different penetration into the Bragg mirrors and can result in optical spin-orbit coupling (SOC). In this work, we find that in a liquid crystal (LC) microcavity filled with perovskite microplates, the pronounced TE-TM splitting gives rise to a strong SOC that leads to the spatial instability of microcavity polariton condensates under single-shot excitation. Spatially varying hole burning and mode competition occurs between polarization components leading to different condensate profiles from shot to shot. The single-shot polariton condensates become stable when the SOC vanishes as the TE and TM modes are spectrally well separated from each other, which can be achieved by application of an electric field to our LC microcavity with electrically tunable anisotropy. Our findings are well reproduced and traced back to their physical origin by our detailed numerical simulations. With the electrical manipulation our work reveals how the shot-to-shot spatial instability of spatial polariton profiles can be engineered in anisotropic microcavities at room temperature, which will benefit the development of stable polariton-based optoeletronic and light-emitting devices.
Thermal silica is a common dielectric used in all silicon-photonic circuits. And bound hydroxyl ions (Si-OH) can provide a significant component of optical loss in this material on account of the wet nature of the thermal oxidation process. A convenient way to quantify this loss relative to other mechanisms is through OH-absorption at 1380 nm. Here, using ultra-high-Q thermal-silica wedge microresonators, the OH absorption loss peak is measured and distinguished from the scattering loss base line over a wavelength range from 680 nm to 1550 nm. Record-high on-chip resonator Q factors are observed for near-visible and visible wavelengths, and the absorption limited Q factor is as high as 8 billion in the telecom band. OH ion content level around 2.4 ppm (weight) is inferred from both Q measurements and by Secondary Ion Mass Spectroscopy (SIMS) depth profiling.
Chao Zheng, Zheng-Hua An, Wen-Xi Peng, Da-Li Zhang, Shao-Lin Xiong, Rui. Qiao, Yan-Qiu Zhang, Wang-Chen Xue, Jia-Cong Liu, Pei-Yi Feng, Ce. Cai, Min Gao, Ke Gong, Dong-Ya Guo, Dong-Jie Hou, Gang Li, Xin-Qiao Li, Yan-Guo Li, Mao-Shun Li, Xiao-Hua Liang, et al (18) As a new member of GECAM mission, GECAM-C (also named High Energy Burst Searcher, HEBS) was launched onboard the SATech-01 satellite on July 27th, 2022, which is capable to monitor gamma-ray transients from $\sim$ 6 keV to 6 MeV. As the main detector, there are 12 gamma-ray detectors (GRDs) equipped for GECAM-C. In order to verify the GECAM-C GRD detector performance and to validate the Monte Carlo simulations of detector response, comprehensive on-ground calibration experiments have been performed using X-ray beam and radioactive sources, including Energy-Channel relation, energy resolution, detection efficiency, SiPM voltage-gain relation and the non-uniformity of positional response. In this paper, the detailed calibration campaigns and data analysis results for GECAM-C GRDs are presented, demonstrating the excellent performance of GECAM-C GRD detectors.
Dali Zhang, Chao Zheng, Jiacong Liu, Zhenghua An, Chenwei Wang, Xiangyang Wen, Xinqiao Li, Xilei Sun, Ke Gong, Yaqing Liu, Xiaojing Liu, Sheng Yang, Wenxi Peng, Rui Qiao, Dongya Guo, Peiyi Feng, Yanqiu Zhang, Wangchen Xue, Wenjun Tan, Ce Cai, et al (25) As a new member of GECAM mission, the GECAM-C (also called High Energy Burst Searcher, HEBS) is a gamma-ray all-sky monitor onboard SATech-01 satellite, which was launched on July 27th, 2022 to detect gamma-ray transients from 6 keV to 6 MeV, such as Gamma-Ray Bursts (GRBs), high energy counterpart of Gravitational Waves (GWs) and Fast Radio Bursts (FRBs), and Soft Gamma-ray Repeaters (SGRs). Together with GECAM-A and GECAM-B launched in December 2020, GECAM-C will greatly improve the monitoring coverage, localization, as well as temporal and spectral measurements of gamma-ray transients. GECAM-C employs 12 SiPM-based Gamma-Ray Detectors (GRDs) to detect gamma-ray transients . In this paper, we firstly give a brief description of the design of GECAM-C GRDs, and then focus on the on-ground tests and in-flight performance of GRDs. We also did the comparison study of the SiPM in-flight performance between GECAM-C and GECAM-B. The results show GECAM-C GRD works as expected and is ready to make scientific observations.
Qing-Xin Ji, Warren Jin, Lue Wu, Yan Yu, Zhiquan Yuan, Wei Zhang, Maodong Gao, Bohan Li, Heming Wang, Chao Xiang, Joel Guo, Avi Feshali, Mario Paniccia, Vladimir S. Ilchenko, Andrey B. Matsko, John Bowers, Kerry Vahala Normal group velocity dispersion (GVD) microcombs offer high comb line power and high pumping efficiency compared to bright pulse microcombs. The recent demonstration of normal GVD microcombs using CMOS-foundry-produced microresonators is an important step towards scalable production. However, the chromatic dispersion of CMOS devices is large and impairs generation of broadband microcombs. Here, we report the development of a microresonator in which GVD is reduced due to a couple-ring resonator configuration. Operating in the turnkey self-injection-locking mode, the resonator is hybridly integrated with a semiconductor laser pump to produce high-power-efficiency combs spanning a bandwidth of 9.9 nm (1.22 THz) centered at 1560 nm, corresponding to 62 comb lines. Fast, linear optical sampling of the comb waveform is used to observe the rich set of near-zero GVD comb behaviors, including soliton molecules, switching waves (platicons) and their hybrids. Tuning of the 20 GHz repetition rate by electrical actuation enables servo locking to a microwave reference, which simultaneously stabilizes the comb repetition rate, offset frequency and temporal waveform. This hybridly integrated system could be used in coherent communications or for ultra-stable microwave signal generation by two-point optical frequency division.
Soliton microcombs are helping to advance the miniaturization of a range of comb systems. These combs mode lock through the formation of short temporal pulses in anomalous dispersion resonators. Here, a new microcomb is demonstrated that mode locks through the formation of pulse pairs in normal-dispersion coupled-ring resonators. Unlike conventional microcombs, pulses in this system cannot exist alone, and instead must phase lock in pairs to form a bright soliton comb. Also, the pulses can form at recurring spectral windows and the pulses in each pair feature different optical spectra. This pairwise mode-locking modality extends to higher dimensions and we demonstrate 3-ring systems in which 3 pulses mode lock through alternating pairwise pulse coupling. The results are demonstrated using the new CMOS-foundry platform that has not previously produced bright solitons on account of its inherent normal dispersion. The ability to generate multi-color pulse pairs over multiple rings is an important new feature for microcombs. It can extend the concept of all-optical soliton buffers and memories to multiple storage rings that multiplex pulses with respect to soliton color and that are spatially addressable. The results also suggest a new platform for the study of quantum combs and topological photonics.
Two-dimensional (2D) magnetic materials have attracted tremendous research interest because of the promising application in the next-generation microelectronic devices. Here, by the first-principles calculations, we propose a two-dimensional ferromagnetic material with high Curie temperature, manganese tetranitride MnN$_4$ monolayer, which is a square-planar lattice made up of only one layer of atoms. The structure is demonstrated to be stable by the phonon spectra and the molecular dynamic simulations, and the stability is ascribed to the $\pi$-d conjugation between $\pi$ orbital of N=N bond and Mn $d$ orbital. More interestingly, the MnN$_4$ monolayer displays robust 2D ferromagnetism, which originates from the strong exchange couplings between Mn atoms due to the $\pi$-d conjugation. The high critical temperature of 247 K is determined by solving the Heisenberg model with the Monte Carlo method.
Manipulating bosonic condensates with electric fields is very challenging as the electric fields do not directly interact with the neutral particles of the condensate. Here we demonstrate a simple electric method to tune the vorticity of exciton polariton condensates in a strong coupling liquid crystal (LC) microcavity with CsPbBr$_3$ microplates as active material at room temperature. In such a microcavity, the LC molecular director can be electrically modulated giving control over the polariton condensation in different modes. For isotropic non-resonant optical pumping we demonstrate the spontaneous formation of vortices with topological charges of +1, +2, -2, and -1. The topological vortex charge is controlled by a voltage in the range of 1 to 10 V applied to the microcavity sample. This control is achieved by the interplay of a built-in potential gradient, the anisotropy of the optically active perovskite microplates, and the electrically controllable LC molecular director in our system with intentionally broken rotational symmetry. Besides the fundamental interest in the achieved electric polariton vortex control at room temperature, our work paves the way to micron-sized emitters with electric control over the emitted light's phase profile and quantized orbital angular momentum for information processing and integration into photonic circuits.
Nemanja Jovanovic, Pradip Gatkine, Boqiang Shen, Maodong Gao, Nick Cvetojevic, Katarzyna Lawniczuk, Ronald Broeke, Charles Beichman, Stephanie Leifer, Jeffery Jewell, Gautam Vasisht, Dimitri Mawet Spectral shaping is critical to many fields of science. In astronomy for example, the detection of exoplanets via the Doppler effect hinges on the ability to calibrate a high resolution spectrograph. Laser frequency combs can be used for this, but the wildly varying intensity across the spectrum can make it impossible to optimally utilize the entire comb, leading to a reduced overall precision of calibration. To circumvent this, astronomical applications of laser frequency combs rely on a bulk optic setup which can flatten the output spectrum before sending it to the spectrograph. Such flatteners require complex and expensive optical elements like spatial light modulators and have non-negligible bench top footprints. Here we present an alternative in the form of an all-photonic spectral shaper that can be used to flatten the spectrum of a laser frequency comb. The device consists of a circuit etched into a silicon nitride wafer that supports an arrayed-waveguide grating to disperse the light over hundreds of nanometers in wavelength, followed by Mach-Zehnder interferometers to control the amplitude of each channel, thermo-optic phase modulators to phase the channels and a second arrayed-waveguide grating to recombine the spectrum. The demonstrator device operates from 1400 to 1800 nm (covering the astronomical H band), with twenty 20 nm wide channels. The device allows for nearly 40 dBs of dynamic modulation of the spectrum via the Mach-Zehnders , which is greater than that offered by most spatial light modulators. With a superluminescent diode, we reduced the static spectral variation to ~3 dB, limited by the properties of the components used in the circuit and on a laser frequency comb we managed to reduce the modulation to 5 dBs, sufficient for astronomical applications.
Nemanja Jovanovic, Pradip Gatkine, Boqiang Shen, Maodong Gao, Nick Cvetojevic, Katarzyna Ławniczuk, Ronald Broeke, Charles Beichman, Stephanie Leifer, Jeffery Jewell, Gautam Vasisht, Dimitri Mawet Laser frequency combs are fast becoming critical to reaching the highest radial velocity precisions. One shortcoming is the highly variable brightness of the comb lines across the spectrum (up to 4-5 orders of magnitude). This can result in some lines saturating while others are at low signal and lost in the noise. Losing lines to either of these effects reduces the precision and hence effectiveness of the comb. In addition, the brightness of the comb lines can vary with time which could drive comb lines with initially reasonable SNR's into the two regimes described above. To mitigate these two effects, laser frequency combs use optical flattener's. Flattener's are typically bulk optic setups that disperse the comb light with a grating, and then use a spatial light modulator to control the amplitude across the spectrum before recombining the light into another single mode fiber and sending it to the spectrograph. These setups can be large (small bench top), expensive (several hundred thousand dollars) and have limited stability. To address these issues, we have developed an all-photonic spectrum flattener on a chip. The device is constructed from optical waveguides on a SiN chip. The light from the laser frequency comb's output optical fiber can be directly connected to the chip, where the light is first dispersed using an arrayed waveguide grating. To control the brightness of each channel, the light is passed through a Mach-Zehnder interferometer before being recombined with a second arrayed waveguide grating. Thermo-optic phase modulators are used in each channel before recombination to path length match the channels as needed. Here we present the results from our first generation prototype. The device operates from 1400-1800 nm (covering the H band), with 20, 20 nm wide channels.
DAMPE Collaboration, F. Alemanno, C. Altomare, Q. An, P. Azzarello, F. C. T. Barbato, P. Bernardini, X. J. Bi, M. S. Cai, E. Casilli, E. Catanzani, J. Chang, D. Y. Chen, J. L. Chen, Z. F. Chen, M. Y. Cui, T. S. Cui, Y. X. Cui, H. T. Dai, A. De-Benedittis, et al (131) More than a century after the performance of the oil drop experiment, the possible existence of fractionally charged particles FCP still remains unsettled. The search for FCPs is crucial for some extensions of the Standard Model in particle physics. Most of the previously conducted searches for FCPs in cosmic rays were based on experiments underground or at high altitudes. However, there have been few searches for FCPs in cosmic rays carried out in orbit other than AMS-01 flown by a space shuttle and BESS by a balloon at the top of the atmosphere. In this study, we conduct an FCP search in space based on on-orbit data obtained using the DArk Matter Particle Explorer (DAMPE) satellite over a period of five years. Unlike underground experiments, which require an FCP energy of the order of hundreds of GeV, our FCP search starts at only a few GeV. An upper limit of $6.2\times 10^{-10}~~\mathrm{cm^{-2}sr^{-1} s^{-1}}$ is obtained for the flux. Our results demonstrate that DAMPE exhibits higher sensitivity than experiments of similar types by three orders of magnitude that more stringently restricts the conditions for the existence of FCP in primary cosmic rays.
In optics, we can generate vortex beams using specific methods such as spiral phase plates or computer generated holograms. While, in nature, it is worth noting that water can produce vortices by a circularly symmetrical hole. So, if a light beam can generate vortex when it is diffracted by an aperture? Here, we show that the light field in the Fresnel region of the diffracted circularly polarized beam carries orbital angular momentum, which can transfer to the trapped particles and make orbital rotation.
Implantable bioelectronics often relies on an RF-wireless link for communication and/or remote powering. Propagation through biological media is very lossy, and previous work has shown that these losses can be separated into three parts: the losses incurred by the propagating fields, the reflections at media interfaces, and the coupling of the reactive near field and the lossy body. The first two are unavoidable, but a clever antenna design can minimize the near-field losses. A good physical understanding of this particular loss phenomenon is thus very desirable. Unfortunately, previous work does not take the implantation depth into account and is thus valid only for deep implants. In this contribution, we propose approximate expressions to the near field losses of antennas implanted in biological hosts considering the encapsulation size, the frequency, the characteristics of the host medium, and the implantation depth. They are obtained using a spherical wave expansion, and are useful for realistic implantation scenarios. This is demonstrated by first comparing the results obtained using these expressions with rigorous computations for two canonical phantoms: a spherical phantom and a planar phantom. Finally, the usefulness of the obtained expressions is illustrated in the practical realization of a capsule-shaped implanted antenna.
The wireless power transfer efficiency to implanted bioelectronic devices is constrained by several frequency-dependent physical mechanisms. Recent works have developed several mathematical formulations to understand these mechanisms and predict the optimal operating conditions. However, existing approaches rely on simplified body models, which are unable to capture important aspects of wireless power transfer. Therefore, this paper proposes the efficiency analysis approach in anatomical models that can provide insightful information on achieving the optimum operation conditions. First, this approach is validated with a theoretical spherical wave expansion analysis, and the results for a simplified spherical model and a human pectoral model are compared. The results show that although a magnetic receiver outperforms an electric one for near-field operation and both sources could be equally employed in far-field range, it is in mid-field that the maximum efficiency is achieved with an optimum frequency between 1-5 GHz depending on the implantation depth. The receiver orientation is another factor that affects the efficiency, with a maximum difference between the best and worst-case scenarios around five times for the electric source and over 13 times for the magnetic one. This approach is used to analyze the case of a deep-implanted pacemaker wirelessly powered by an on-body transmitter and subjected to stochastic misalignments. We evaluate the efficiency and exposure, and we demonstrate how a buffered transmitter can be tailored to achieve maximum powering efficiency. Finally, design guidelines that lead to optimal implantable wireless power transfer systems are established from the results obtained with the proposed approach.
Single-atom-thick two-dimensional materials such as graphene usually have a hexagonal lattice while the square-planar lattice is uncommon in the family of two-dimensional materials. Here, we demonstrate that single-atom-thick transition metal nitride CrN$_4$ monolayer is a stable free-standing layer with a square-planar network. The stability of square-planar geometry is ascribed to the combination of N=N double bond, Cr-N coordination bond, and $\pi$-d conjugation, in which the double $\pi$-d conjugation is rarely reported in previous studies. This mechanism is entirely different from that of the reported two-dimensional materials, leading to lower formation energy and more robust stability compared to the synthesized g-C$_3$N$_4$ monolayer. On the other hand, CrN$_4$ layer has a ferromagnetic ground state, in which the ferromagnetic coupling between two Cr atoms is mediated by electrons of the half-filled large $\pi$ orbitals from $\pi$-d conjugation. The high-temperature ferromagnetism in CrN$_4$ monolayer is confirmed by solving the Heisenberg model with Monte Carlo method.
Magnetic two-dimensional materials have potential application in next-generation electronic devices and have stimulated extensive interest in condensed matter physics and material fields. However, how to realize high-temperature ferromagnetism in two-dimensional materials remains a great challenge in physics. Herein, we propose an effective approach that the dimerization of magnetic ions in two-dimensional materials can enhance the exchange coupling and stabilize the ferromagnetism. Manganese carbonitride Mn$_2$N$_6$C$_6$ with a planar monolayer structure is taken as an example to clarify the method, in which two Mn atoms are gathered together to form a ferromagnetic dimer of Mn atoms and further these dimers are coupled together to form the overall ferromagnetism of the two-dimensional material. In Mn$_2$N$_6$C$_6$ monolayer, the near-room-temperature ferromagnetism with the Curie temperature of 272.3 K is determined by solving Heisenberg model using Monte Carlo simulations method.
Di Xia, Zelin Yang, Pingyang Zeng, Bin Zhang, Jiayue Wu, Zifu Wang, Jiaxin Zhao, Mingqi Gao, Yufei Huang, Jianteng Huang, Liyang Luo, Dong Liu, Shuixian Yang, Hairun Guo, Zhaohui Li Photonic integrated microcombs have enabled advanced applications in optical communication, microwave synthesis, and optical metrology, which in nature unveil an optical dissipative soliton pattern under cavity-enhanced nonlinear processes. The most decisive factor of microcombs lies in the photonic material platforms, where materials with high nonlinearity and in capacity of high-quality chip integration are highly demanded. In this work, we present a home-developed chalcogenide glasses-Ge25Sb10S65 (GeSbS) for the nonlinear photonic integration and for the dissipative soliton microcomb generation. Compared with the current integrated nonlinear platforms, the GeSbS features wider transparency from the visible to 11 um region, stronger nonlinearity, and lower thermo-refractive coefficient, and is CMOS compatible in fabrication. In this platform, we achieve chip-integrated optical microresonators with a quality (Q) factor above 2 x 10^6, and carry out lithographically controlled dispersion engineering. In particular, we demonstrate that both a bright soliton-based microcomb and a dark-pulsed comb are generated in a single microresonator, in its separated fundamental polarized mode families under different dispersion regimes. The overall pumping power is on the ten-milliwatt level, determined by both the high Q-factor and the high material nonlinearity of the microresonator. Our results may contribute to the field of nonlinear photonics with an alternative material platform for highly compact and high-intensity nonlinear interactions, while on the application aspect, contribute to the development of soliton microcombs at low operation power, which is potentially required for monolithically integrated optical frequency combs.
Qiangbing Guo, Xiao-Zhuo Qi, Meng Gao, Sanlue Hu, Lishu Zhang, Wenju Zhou, Wenjie Zang, Xiaoxu Zhao, Junyong Wang, Bingmin Yan, Mingquan Xu, Yun-Kun Wu, Goki Eda, Zewen Xiao, Huiyang Gou, Yuan Ping Feng, Guang-Can Guo, Wu Zhou, Xi-Feng Ren, Cheng-Wei Qiu, et al (2) Interlayer electronic coupling in two-dimensional (2D) materials enables tunable and emergent properties by stacking engineering. However, it also brings significant evolution of electronic structures and attenuation of excitonic effects in 2D semiconductors as exemplified by quickly degrading excitonic photoluminescence and optical nonlinearities in transition metal dichalcogenides when monolayers are stacked into van der Waals structures. Here we report a novel van der Waals crystal, niobium oxide dichloride, featuring a vanishing interlayer electronic coupling and scalable second harmonic generation intensity of up to three orders higher than that of exciton-resonant monolayer WS2. Importantly, the strong second-order nonlinearity enables correlated parametric photon pair generation, via a spontaneous parametric down-conversion (SPDC) process, in flakes as thin as ~46 nm. To our knowledge, this is the first SPDC source unambiguously demonstrated in 2D layered materials, and the thinnest SPDC source ever reported. Our work opens an avenue towards developing van der Waals material-based ultracompact on-chip SPDC sources, and high-performance photon modulators in both classical and quantum optical technologies.
Y.B. Xu, X.L. Sun, S. Yang, X.Q. Li, W.X. Peng, K. Gong, X.H. Liang, Y.Q. Liu, D.Y. Guo, H. Wang, C.Y. Li, Z.H.An, J.J. He, X.J. Liu, S.L. Xiong, X.Y. Wen, Fan Zhang, D.L. Zhang, X.Y. Zhao, C.Y. Zhang, et al (30) The Gravitational Wave highly energetic Electromagnetic Counterpart All-sky Monitor (GECAM) is dedicated to detecting gravitational wave gamma-ray bursts. It is capable of all-sky monitoring over and discovering gamma-ray bursts and new radiation phenomena. GECAM consists of two microsatellites, each equipped with 8 charged particle detectors (CPDs) and 25 gamma-ray detectors (GRDs). The CPD is used to measure charged particles in the space environment, monitor energy and flow intensity changes, and identify between gamma-ray bursts and space charged particle events in conjunction with GRD. CPD uses plastic scintillator as the sensitive material for detection, silicon photomultiplier (SiPM) array as the optically readable device, and the inlaid Am-241 radioactive source as the onboard calibration means. In this paper, we will present the working principle, physical design, functional implementation and preliminary performance test results of the CPD.
X. Q. Li, X. Y. Wen, S. L. Xiong, K. Gong, D. L. Zhang, Z. H. An, Y. B. Xu, Y. Q. Liu, C. Cai, Z. Chang, G. Chen, C. Chen, Y. Y. Du, M. Gao, R. Gao, D. Y. Guo, J. J. He, D. J. Hou, Y. G. Li, C. Li, et al (39) The GECAM mission consists of two identical microsatellites (GECAM-A and GECAM-B). Each satellite is equipped with 25 gamma-ray detectors (GRD) and 8 charged particle detectors (CPD). The main scientific objective of the GECAM mission is to detect gamma-ray bursts (GRBs) associated with the gravitational wave events produced by the merging of binary compact stars. After the launch on Dec. 10, 2020 , we carried out a series of on orbit tests. This paper introduces the test results of the GECAM-B satellite. According to the in-flight performance, the energy band for gamma-ray detection of GECAM-B is from about 7 keV to 3.5 MeV. GECAM-B can achieve prompt localization of GRBs. For the first time, GECAM-B realized a quasi-real-time transmission of trigger information using Beidou-3 RDSS. Keywords GECAM, gamma-ray burst, gravitational wave, GRD, CPD
We propose an unsupervised convolutional neural network (CNN) for relaxation parameter estimation. This network incorporates signal relaxation and Bloch simulations while taking advantage of residual learning and spatial relations across neighboring voxels. Quantification accuracy and robustness to noise is shown to be significantly improved compared to standard parameter estimation methods in numerical simulations and in vivo data for multi-echo T2 and T2* mapping. The combination of the proposed network with subspace modeling and MR fingerprinting (MRF) from highly undersampled data permits high quality T1 and T2 mapping.
Maodong Gao, Qi-Fan Yang, Qing-Xin Ji, Heming Wang, Lue Wu, Boqiang Shen, Junqiu Liu, Guanhao Huang, Lin Chang, Weiqiang Xie, Su-Peng Yu, Scott B. Papp, John E. Bowers, Tobias J. Kippenberg, Kerry J. Vahala Optical microresonators with high quality ($Q$) factors are essential to a wide range of integrated photonic devices. Steady efforts have been directed towards increasing microresonator $Q$ factors across a variety of platforms. With success in reducing microfabrication process-related optical loss as a limitation of $Q$, the ultimate attainable $Q$, as determined solely by the constituent microresonator material absorption, has come into focus. Here, we report measurements of the material-limited $Q$ factors in several photonic material platforms. High-$Q$ microresonators are fabricated from thin films of SiO$_2$, Si$_3$N$_4$, Al$_{0.2}$Ga$_{0.8}$As and Ta$_2$O$_5$. By using cavity-enhanced photothermal spectroscopy, the material-limited $Q$ is determined. The method simultaneously measures the Kerr nonlinearity in each material and reveals how material nonlinearity and ultimate $Q$ vary in a complementary fashion across photonic materials. Besides guiding microresonator design and material development in four material platforms, the results help establish performance limits in future photonic integrated systems.
D.L. Zhang, M. Gao, X.L. Sun, X.Q. Li, Z.H. An, X.Y. Wen, C. Cai, Z. Chang, G. Chen, C. Chen, Y.Y. Du, R. Gao, K. Gong, D.Y. Guo, J.J. He, D.J. Hou, Y.G. Li, C.Y. Li, G. Li, L. Li, et al (28) The Gravitational wave high-energy Electromagnetic Counterpart All-sky Monitor (GECAM) satellite consists of two small satellites. Each GECAM payload contains 25 gamma ray detectors (GRD) and 8 charged particle detectors (CPD). GRD is the main detector which can detect gamma-rays and particles and localize the Gamma-Ray Bursts (GRB),while CPD is used to help GRD to discriminate gamma-ray bursts and charged particle bursts. The GRD makes use of lanthanum bromide (LaBr3) crystal readout by SiPM. As the all available SiPM devices belong to commercial grade, quality assurance tests need to be performed in accordance with the aerospace specifications. In this paper, we present the results of quality assurance tests, especially a detailed mechanism analysis of failed devices during the development of GECAM. This paper also summarizes the application experience of commercial-grade SiPM devices in aerospace payloads, and provides suggestions for forthcoming SiPM space applications.
Xiangyan Sun, Ke Liu, Yuquan Lin, Lingjie Wu, Haoming Xing, Minghong Gao, Ji Liu, Suocheng Tan, Zekun Ni, Qi Han, Junqiu Wu, Jie Fan We have developed an end-to-end, retrosynthesis system, named ChemiRise, that can propose complete retrosynthesis routes for organic compounds rapidly and reliably. The system was trained on a processed patent database of over 3 million organic reactions. Experimental reactions were atom-mapped, clustered, and extracted into reaction templates. We then trained a graph convolutional neural network-based one-step reaction proposer using template embeddings and developed a guiding algorithm on the directed acyclic graph (DAG) of chemical compounds to find the best candidate to explore. The atom-mapping algorithm and the one-step reaction proposer were benchmarked against previous studies and showed better results. The final product was demonstrated by retrosynthesis routes reviewed and rated by human experts, showing satisfying functionality and a potential productivity boost in real-life use cases.
Recently microcavities with anisotropic materials are shown to be able to create novel bands with non-zero local Berry curvature. The anisotropic refractive index of the cavity layer is believed to be critical in opening an energy gap at the tilted Dirac points. In this work, we show that an anticrossing between a cavity mode and a Bragg mode can also form within an empty microcavity without any birefringent materials. Flat bands are observed within the energy gap due to the particular refractive index distribution of the sample. The intrinsic TE-TM splitting and XY splitting induce the squeezing of the cavity modes in momentum space, so that the flat bands are spin-dependently tilted. Our results pave the way to investigate the spin orbit coupling of photons in a simple microcavity without anisotropic cavity layers.
Li Na Quan, Yoonjae Park, Peijun Guo, Mengyu Gao, Jianbo Jin, Jianmei Huang, Jason K. Copper, Adam Schwartzberg, Richard Schaller, David T. Limmer, Peidong Yang Organic-inorganic layered perovskites are two-dimensional quantum wells with layers of lead-halide octahedra stacked between organic ligand barriers. The combination of their dielectric confinement and ionic sublattice results in excitonic excitations with substantial binding energies that are strongly coupled to the surrounding soft, polar lattice. However, the ligand environment in layered perovskites can significantly alter their optical properties due to the complex dynamic disorder of soft perovskite lattice. Here, we observe the dynamic disorder through phonon dephasing lifetimes initiated by ultrafast photoexcitation employing high-resolution resonant impulsive stimulated Raman spectroscopy of a variety of ligand substitutions. We demonstrate that vibrational relaxation in layered perovskite formed from flexible alkyl-amines as organic barriers is fast and relatively independent of the lattice temperature. Relaxation in aromatic amine based layered perovskite is slower, though still fast relative to pure inorganic lead bromide lattices, with a rate that is temperature dependent. Using molecular dynamics simulations, we explain the fast rates of relaxation by quantifying the large anharmonic coupling of the optical modes with the ligand layers and rationalize the temperature independence due to their amorphous packing. This work provides a molecular and time-domain depiction of the relaxation of nascent optical excitations and opens opportunities to understand how they couple to the complex layered perovskite lattice, elucidating design principles for optoelectronic devices.
Zhiquan Yuan, Heming Wang, Peng Liu, Bohan Li, Boqiang Shen, Maodong Gao, Lin Chang, Warren Jin, Avi Feshali, Mario Paniccia, John Bowers, Kerry Vahala Narrow-linewidth lasers are important to many applications spanning precision metrology to sensing systems. Characterization of these lasers requires precise measurements of their frequency noise spectra. Here we demonstrate a correlated self-heterodyne (COSH) method capable of measuring frequency noise as low as 0.01 Hz$^2$/Hz at 1 MHz offset frequency. The measurement setup is characterized by both commercial and lab-built lasers, and features low optical power requirements, fast acquisition time and high intensity noise rejection.
Liquid crystals formed by acute-angle bent-core (ABC) molecules with a 1,7 naphthalene central core show an intriguing phase behavior with the nematic phase accompanied by poorly understood additional phases. In this work, we characterize the physical properties of an ABC material, such as birefringence, dielectric permittivities, elastic constants, and surface alignment, and present X-ray diffraction and transmission electron microscopy studies of their ordering. The ABC molecular shape resembling the letter $\lambda$ yields a very small splay elastic constant in the uniaxial nematic phase and results in the formation of a tetragonal positionally ordered columnar phase consisting of molecular columns with a uniform uniaxial director that can be bent but not splayed.
Halide perovskites have attracted increasing research attention regarding their outstanding optoelectronic applications. Owing to its low activation energy, ion migration is implicated in the long-term stability and many unusual transport behaviors of halide perovskite devices. However, precise control of the ionic transport in halide perovskite crystals remains challenging. Here we visualized and quantified the electric-field-induced halide ion migration in an axial CsPbBr$_3$-CsPbCl$_3$ nanowire heterostructure and demonstrated a solid-state ionic rectification, which is due to the non-uniform distribution of the ionic vacancies in the nanowire that results from a competition between electrical screening and their creation and destruction at the electrode interface. The asymmetric heterostructure characteristics add an additional knob to the ion-movement manipulation in the design of advanced ionic circuits with halide perovskites as building blocks.
Purpose: To investigate the feasibility of myelin water content quantification using fast dual-echo steady-state (DESS) scans and machine learning with kernels. Methods: We optimized combinations of steady-state (SS) scans for precisely estimating the fast-relaxing signal fraction ff of a two-compartment signal model, subject to a scan time constraint. We estimated ff from the optimized DESS acquisition using a recently developed method for rapid parameter estimation via regression with kernels (PERK). We compared DESS PERK ff estimates to conventional myelin water fraction (MWF) estimates from a longer multi-echo spin-echo (MESE) acquisition in simulation, in vivo, and ex vivo studies. Results: Simulations demonstrate that DESS PERK ff estimators and MESE MWF estimators achieve comparable error levels. In vivo and ex vivo experiments demonstrate that MESE MWF and DESS PERK ff estimates are quantitatively comparable measures of WM myelin water content. To our knowledge, these experiments are the first to demonstrate myelin water images from a SS acquisition that are quantitatively similar to conventional MESE MWF images. Conclusion: Combinations of fast DESS scans can be designed to enable precise ff estimation. PERK is well-suited for ff estimation. DESS PERK ff and MESE MWF estimates are quantitatively similar measures of WM myelin water content.
A. Tykhonov, G. Ambrosi, R. Asfandiyarov, P. Azzarello, P. Bernardini, B. Bertucci, A. Bolognini, F. Cadoux, A. D'Amone, A. De Benedittis, I. De Mitri, M. Di Santo, Y. F. Dong, M. Duranti, D. D'Urso, R. R. Fan, P. Fusco, V. Gallo, M. Gao, F. Gargano, et al (22) DAMPE (DArk Matter Particle Explorer) is a spaceborne high-energy cosmic ray and gamma-ray detector, successfully launched in December 2015. It is designed to probe astroparticle physics in the broad energy range from few GeV to 100 TeV. The scientific goals of DAMPE include the identification of possible signatures of Dark Matter annihilation or decay, the study of the origin and propagation mechanisms of cosmic-ray particles, and gamma-ray astronomy. DAMPE consists of four sub-detectors: a plastic scintillator strip detector, a Silicon-Tungsten tracKer-converter (STK), a BGO calorimeter and a neutron detector. The STK is composed of six double layers of single-sided silicon micro-strip detectors interleaved with three layers of tungsten for photon conversions into electron-positron pairs. The STK is a crucial component of DAMPE, allowing to determine the direction of incoming photons, to reconstruct tracks of cosmic rays and to estimate their absolute charge (Z). We present the in-flight performance of the STK based on two years of in-flight DAMPE data, which includes the noise behavior, signal response, thermal and mechanical stability, alignment and position resolution.
The temperature of the semiconductor diode increases under strong light illumination whether thermoelectric cooler is installed or not, which changes the output wavelength of the laser (Lee M. S. et al., 2017). However, other characteristics also vary as temperature increases. These variations may help the eavesdropper in practical quantum key distribution systems. We study the effects of temperature increase on gain-switched semiconductor lasers by simulating temperature dependent rate equations. The results show that temperature increase may cause large intensity fluctuation, decrease the output intensity and lead the signal state and decoy state distinguishable. We also propose a modified photon number splitting attack by exploiting the effects of temperature increase. Countermeasures are also proposed.
A. Tykhonov, G. Ambrosi, R. Asfandiyarov, P. Azzarello, P. Bernardini, B. Bertucci, A. Bolognini, F. Cadoux, A. D'Amone, A. De Benedittis, I. De Mitri, M. Di Santo, Y. F. Dong, M. Duranti, D. D'Urso, R. R. Fan, P. Fusco, V. Gallo, M. Gao, F. Gargano, et al (23) The DArk Matter Particle Explorer (DAMPE) is a space-borne particle detector designed to probe electrons and gamma-rays in the few GeV to 10 TeV energy range, as well as cosmic-ray proton and nuclei components between 10 GeV and 100 TeV. The silicon-tungsten tracker-converter is a crucial component of DAMPE. It allows the direction of incoming photons converting into electron-positron pairs to be estimated, and the trajectory and charge (Z) of cosmic-ray particles to be identified. It consists of 768 silicon micro-strip sensors assembled in 6 double layers with a total active area of 6.6 m$^2$. Silicon planes are interleaved with three layers of tungsten plates, resulting in about one radiation length of material in the tracker. Internal alignment parameters of the tracker have been determined on orbit, with non-showering protons and helium nuclei. We describe the alignment procedure and present the position resolution and alignment stability measurements.
Baoshan Cui, Dong Li, Shiwei Chen, Jijun Yun, Yalu Zuo, Xiaobin Guo, Kai Wu, Xu Zhang, Yupei Wang, Dezheng Yang, Meizhen Gao, Li Xi Magnetic trilayers having large perpendicular magnetic anisotropy (PMA) and high spin-orbit torques (SOTs) efficiency are the key to fabricate nonvolatile magnetic memory and logic devices. In this work, PMA and SOTs are systematically studied in Pt/Co/Cr stacks as a function of Cr thickness. An enhanced perpendicular anisotropy field around 10189 Oe is obtained and is related to the interface between Co and Cr layers. In addition, an effective spin Hall angle up to 0.19 is observed due to the improved antidamping-like torque by employing dissimilar metals Pt and Cr with opposite signs of spin Hall angles on opposite sides of Co layer. Finally, we observed a nearly linear dependence between spin Hall angle and longitudinal resistivity from their temperature dependent properties, suggesting that the spin Hall effect may arise from extrinsic skew scattering mechanism. Our results indicate that 3d transition metal Cr with a large negative spin Hall angle could be used to engineer the interfaces of trilayers to enhance PMA and SOTs.
J. Chang, G. Ambrosi, Q. An, R. Asfandiyarov, P. Azzarello, P. Bernardini, B. Bertucci, M. S. Cai, M. Caragiulo, D. Y. Chen, H. F. Chen, J. L. Chen, W. Chen, M. Y. Cui, T. S. Cui, A. D'Amone, A. De Benedittis, I. De Mitri, M. Di Santo, J. N. Dong, et al (144) The DArk Matter Particle Explorer (DAMPE), one of the four scientific space science missions within the framework of the Strategic Pioneer Program on Space Science of the Chinese Academy of Sciences, is a general purpose high energy cosmic-ray and gamma-ray observatory, which was successfully launched on December 17th, 2015 from the Jiuquan Satellite Launch Center. The DAMPE scientific objectives include the study of galactic cosmic rays up to $\sim 10$ TeV and hundreds of TeV for electrons/gammas and nuclei respectively, and the search for dark matter signatures in their spectra. In this paper we illustrate the layout of the DAMPE instrument, and discuss the results of beam tests and calibrations performed on ground. Finally we present the expected performance in space and give an overview of the mission key scientific goals.
Dongya Guo, Huanyu Wang, Wenxi Peng, Xingzhu Cui, Chengmo Zhang, Yaqing Liu, Xiaohua Liang, Yifan Dong, Jinzhou Wang, Min Gao, Jiawei Yang, Jiayu Zhang, Chunlai Li, Yongliao Zou, Guangliang Zhang, Liyan Zhang, Xiaohui Fu The Active Particle-induced X-ray Spectrometer (APXS) is one of the payloads on board the Yutu rover of Chang'E-3 mission. In order to assess the instrumental performance of APXS, a ground verification test was done for two unknown samples (basaltic rock, mixed powder sample). In this paper, the details of the experiment configurations and data analysis method are presented. The results show that the elemental abundance of major elements can be well determined by the APXS with relative deviations < 15 wt. % (detection distance = 30 mm, acquisition time = 30 min). The derived detection limit of each major element is inversely proportional to acquisition time and directly proportional to detection distance, suggesting that the appropriate distance should be < 50mm.
The supercritical state is currently viewed as uniform and homogeneous on the pressure-temperature phase diagram in terms of physical properties. Here, we study structural properties of the supercritical carbon dioxide, and discover the existence of persistent medium-range order correlations which make supercritical carbon dioxide non-uniform and heterogeneous on an intermediate length scale, a result not hitherto anticipated. We report on the carbon dioxide heterogeneity shell structure where, in the first shell, both carbon and oxygen atoms experience gas-like type inter- actions with short range order correlations, while within the second shell oxygen atoms essentially exhibit liquid-like type of interactions with medium range order correlations due to localisation of transverse-like phonon packets. We show that the local order heterogeneity remains in the three phase-like equilibrium within very wide temperature range. Importantly, we highlight a catalytic role of atoms inside the nearest neighbor heterogeneity shell in providing a mechanism for diffusion in the supercritical carbon dioxide on an intermediate length scale. Finally, we discuss important implications for answering the intriguing question whether Venus may have had carbon dioxide oceans and urge for an experimental detection of this persistent local order heterogeneity.
We experimentally demonstrate microwave control of the motional state of a trapped ion placed in a state-dependent potential generated by a running optical lattice. Both the optical lattice depth and the running lattice frequency provide tunability of the spin-motion coupling strength. The spin-motional coupling is exploited to demonstrate sideband cooling of a Yb171 ion to the ground state of motion.
In search for novel nematic materials, a laterally linked H-shaped liquid crystal dimer have been synthesized and characterized. The distinct feature of the material is a very broad temperature range (about 50 oC) of the nematic phase, which is in contrast with other reported H-dimers that show predominantly smectic phases. The material exhibits interesting textural features at the scale of nanometers (presence of smectic clusters) and at the macroscopic scales. Namely, at a certain temperature, the flat samples of the material show occurrence of domain walls. These domain walls are caused by the surface anchoring transition and separate regions with differently tilted director. Both above and below this transition temperature the material represents a uniaxial nematic, as confirmed by the studies of defects in flat samples and samples with colloidal inclusions, freely suspended drops, X-ray diffraction and transmission electron microscopy.
R.R.Fan, F.Zhang, W.X.Peng, Y.F.Dong, K.Gong, S.Yang, D.Y.Guo, J.Z.Wang, M.Gao, X.H.Liang, J.Y.Zhang, X.Z.Cui, Y.Q.Liu, H.Y.Wang A new generation detector for the high energy cosmic ray - the DAMPE(DArk Matter Particle Explorer) is a satellite based project. Its main object is the measurement of energy spectrum of cosmic ray nuclei from 100GeV to 100TeV, the high energy electrons and gamma ray from 5GeV to 10TeV. A silicon matrix detector described in this paper, is employed for the sea level cosmic ray energy and position detection while the prototype testing of the DAMPE. This matrix is composed by the 180 silicon PIN detectors, which covers an area of 32*20 cm2. The primary testing results are shown including MIPs energy spectrum and the position sensitive map.
Volodymyr Borshch, Young-Ki Kim, Jie Xiang, Min Gao, Antal Jákli, Vitaly P. Panov, Jagdish K. Vij, Corrie T. Imrie, Maria-Gabriela Tamba, Georg H. Mehl, Oleg D. Lavrentovich A state of matter in which molecules show a long-range orientational order and no positional order is called a nematic liquid crystal. The best known and most widely used (for example, in modern displays) is the uniaxial nematic, with the rod-like molecules aligned along a single axis, called the director. When the molecules are chiral, the director twists in space, drawing a right-angle helicoid and remaining perpendicular to the helix axis; the structure is called a chiral nematic. In this work, using transmission electron and optical microscopy, we experimentally demonstrate a new nematic order, formed by achiral molecules, in which the director follows an oblique helicoid, maintaining a constant oblique angle with the helix axis and experiencing twist and bend. The oblique helicoids have a nanoscale pitch. The new twist-bend nematic represents a structural link between the uniaxial nematic (no tilt) and a chiral nematic (helicoids with right-angle tilt).
The total impedance of a ladder-shape network consisting of inductors and capacitors does not converge to a certain value when the steps of the network increased. In this paper, we analyze this effect in frequency domain. We find that in some band the impedance converge to a limit value while in other band it doesn't. Based on this property in frequency, we propose a filter that exhibits excellent performance both in amplitude and phase response. As a validation of our result, the simulation of this filter was carried out on the EDA software Multisim with respect to a practical circuit.